Ion-trap Quantum Computing Laboratory

We propose an ion-trap implementation of the Vaccaro, Barnett and Wright et al. spin-heat engine (SHE); a hypothetical engine that operates between energy and spin thermal reservoirs rather than two energy reservoirs. The SHE operates in two steps: first, in the work extraction stage, heat from a thermal energy reservoir is converted into optical work via a two photon Raman transition resonant with close-to energy degenerate spin states; second, the internal spin states are brought back to their initial state via non-energetic information erasure using a spin reservoir. The latter incurs no energy cost, but rather the reset occurs at the cost of angular momentum from a spin bath that acts as the thermal spin reservoir. The SHE represents an important first step toward demonstrating heat engines that operate beyond the conventional paradigm of requiring two thermal reservoirs, paving the way to harness quantum coherence in arbitrary conserved quantities via similar machines.

Experimental realizations of two qubit entangling gates with trapped ions typically rely on addressing spectroscopically resolved motional sidebands, limiting gate speed to the secular frequency. Fast entangling gates using ultrafast pulsed lasers overcome this speed limit. This approach is based on state-dependent photon recoil kicks from a sequence of counter-propagating, resonant, ultrafast pulse pairs, which can allow sub-microsecond gate speeds. Here we demonstrate a key component of the ultrafast gate protocol, the coherent excitation of a 171Yb+ ion across the 2S1/2-2P1/2 transition with a single near-resonant short optical pulse at 369.53 nm. We achieve a maximum population transfer of 94.3(6)% using a picosecond pulsed laser that can be tuned across the 2S1/2-2P1/2 transition, and 42.53(13)% with 190(7) GHz detuning.

Efficiently scaling quantum networks to long ranges requires local processing nodes to perform basic computation and communication tasks. Trapped ions have demonstrated all the properties required for the construction of such a node, storing quantum information for up to 12 minutes, implementing deterministic high fidelity logic operations on one and two qubits, and ion-photon coupling. While most ions suitable for quantum computing emit photons in visible to near ultraviolet (UV) frequency ranges poorly suited to long-distance fibre optical based networking, recent experiments in frequency conversion provide a technological solution by shifting the photons to frequencies in the telecom band with lower attenuation for fused silica fibres. Encoding qubits in frequency rather than polarization makes them more robust against decoherence from thermal or mechanical noise due to the conservation of energy. To date, ion-photonic frequency qubit entanglement has not been directly shown. Here we demonstrate a frequency encoding ion-photon entanglement protocol in $^{171}$Yb$^+$ with correlations equivalent to 92.4(8)% fidelity using a purpose-built UV hyperfine spectrometer. The same robustness against decoherence precludes our passive optical setup from rotating photonic qubits to unconditionally demonstrate entanglement, however it is sufficient to allow us to benchmark the quality of ion-UV photon correlations prior to frequency conversion to the telecom band.

Surface ion traps are among the most promising technologies for scaling up quantum computing machines, but their complicated multi-electrode geometry can make some tasks, including compensation for stray electric fields, challenging both at the level of modeling and of practical implementation. Here we demonstrate the compensation of stray electric fields using a gradient descent algorithm and a machine learning technique, which trained a deep learning network. We show automated dynamical compensation tested against induced electric charging from UV laser light hitting the chip trap surface. The results show improvement in compensation using gradient descent and the machine learner over manual compensation. This improvement is inferred from an increase of the fluorescence rate of 78% and 96% respectively, for a trapped $^{171}$Yb$^+$ ion driven by a laser tuned to -7.8 MHz of the $^2$S$_{1/2}\leftrightarrow^2$P$_{1/2}$ Doppler cooling transition at 369.5 nm.

Isotope selective optical excitation of atoms is important for experiments with neutral atoms, metrology, and work with trapped ions, including quantum information processing. Polarization-enhanced absorption spectroscopy is used to frequency stabilise a tunable external cavity laser diode system at 398.9 nm for isotope selective photoionization of neutral Yb atoms. This spectroscopy technique is used to measure isotope resolved dispersive features from transitions within a see through configuration Ytterbium hollow-cathode discharge lamp. This Doppler-free dichroic polarization spectroscopy is realised by retro-reflecting a laser beam through the discharge and analysing the polarization dependent absorption with balanced detection. The spectroscopy signal is recovered using lock-in detection of frequency modulation induced by current modulation of the external cavity laser diode. Here, we show the use of polarization-enhanced absorption spectroscopy for isotope selectively loading of $^{171}$Yb$^+$, $^{172}$Yb$^+$, or $^{174}$Yb$^+$ ions into an RF Paul trap.

Compact and robust ion traps for thorium are enabling technology for the next generation of atomic clocks based on a low-energy isomeric transition in the thorium-229 nucleus. We aim at a laser ablation loading of single triply ionized thorium in a radio-frequency electromagnetic linear Paul trap. Detection of ions is based on a modified mass spectrometer and a channeltron with single-ion sensitivity. In this study, we successfully created and detected 232Th+ and 232Th2+ ions from plasma plumes, studied their yield evolution, and compared the loading to a quadrupole ion trap with Yb. We explore the feasibility of laser ablation loading for future low-cost 229Th3+ trapping. The thorium ablation yield shows a strong depletion, suggesting that we have ablated oxide layers from the surface and the ions were a result of the plasma plume evolution and collisions. Our results are in good agreement with similar experiments for other elements and their oxides.

Here we present a cost effective multi-channel opto-mechanical switch and software PID system for locking multiple lasers to a single channel commercial wavemeter. The switch is based on a rotating cylinder that selectively transmits one laser beam at a time to the wavemeter, the wavelength is read by the computer and an error signal is output to the lasers to correct wavelength drifts every millisecond. We use this system to stabilise 740 nm (subsequently frequency doubled to 370 nm), 399 nm and 935 nm lasers for trapping and cooling different isotopes of Yb+ ion. We characterize the frequency stability of the three lasers by using a second, more precise, commercial wavemeter. We also characterise the absolute frequency stability of the 740 nm laser using the fluorescence drift rate of a trapped 174Yb+ ion. For the 740 nm laser we demonstrate an Allan deviation, df/f, of 3 x 10^-10 (at 20 s integration time), equivalent to sub-200 KHz stability.

Obtaining quantitative ground-state behavior for geometrically-frustrated quantum magnets with long-range interactions is challenging for numerical methods. Here, we demonstrate that the ground states of these systems on two-dimensional lattices can be efficiently obtained using state-of-the-art translation-invariant variants of matrix product states and density-matrix renormalization-group algorithms. We use these methods to calculate the fully-quantitative ground-state phase diagram of the long-range interacting triangular Ising model with a transverse field on 6-leg infinite-length cylinders, and scrutinize the properties of the detected phases. We compare these results with those of the corresponding nearest neighbor model. Our results suggest that, for such long-range Hamiltonians, the long-range quantum fluctuations always lead to long-range correlations, where correlators exhibit power-law decays instead of the conventional exponential drops observed for short-range correlated gapped phases. Our results are relevant for comparisons with recent ion-trap quantum simulator experiments that demonstrate highly-controllable long-range spin couplings for several hundred ions.

All physical interactions are mediated by forces. Ultra-sensitive force measurements are therefore a crucial tool for investigating the fundamental physics of magnetic, atomic, quantum, and surface phenomena. Laser cooled trapped atomic ions are a well controlled quantum system and a standard platform for precision metrology. Their low mass, strong Coulomb interaction, and readily detectable fluorescence signal make trapped ions favourable for performing high-sensitivity force measurements. Here we demonstrate a three-dimensional sub-attonewton sensitivity force sensor based on super-resolution imaging of the fluorescence from a single laser cooled $^{174}$Yb$^+$ ion in a Paul trap. The force is detected by measuring the net ion displacement with nanometer precision, and does not rely on mechanical oscillation. Observed sensitivities were 372$\pm$9$_\mbox{stat}$, 347$\pm$12$_\mbox{sys}\pm$14$_\mbox{stat}$, and 808$\pm$29$_\mbox{sys}\pm$42$_\mbox{stat}$ zN/$\sqrt{\mbox{Hz}}$ in the three dimensions, corresponding to 24x, 87x, and 21x of the quantum limit. We independently verified the accuracy of this apparatus by measuring a light pressure force of 95 zN on the ion, an important systematic effect in any optically based force sensor. This technique can be applied for sensing DC or low frequency forces external to the trap or internally from a co-trapped biomolecule or nanoparticle.

Quantum networking links quantum processors through remote entanglement for distributed quantum information processing (QIP) and secure long-range communication. Trapped ions are a leading QIP platform, having demonstrated universal small-scale processors and roadmaps for large-scale implementation. Overall rates of ion-photon entanglement generation, essential for remote trapped ion entanglement, are limited by coupling efficiency into single mode fibres5 and scaling to many ions. Here we show a microfabricated trap with integrated diffractive mirrors that couples 4.1(6)% of the fluorescence from a $^{174}$Yb$^+$ ion into a single mode fibre, nearly triple the demonstrated bulk optics efficiency. The integrated optic collects 5.8(8)% of the π transition fluorescence, images the ion with sub-wavelength resolution, and couples 71(5)% of the collected light into the fibre. Our technology is suitable for entangling multiple ions in parallel and overcomes mode quality limitations of existing integrated optical interconnects. In addition, the efficiencies are sufficient for fault tolerant QIP.

Trapped ions are one of the most promising approaches for the realization of a universal quantum computer. Faster quantum logic gates could dramatically improve the performance of trapped-ion quantum computers, and require the development of suitable high repetition rate pulsed lasers. Here we report on a robust frequency upconverted fiber laser based source, able to deliver 2.5 ps ultraviolet (UV) pulses at a stabilized repetition rate of 300.00000 MHz with an average power of 190 mW. The laser wavelength is resonant with the strong transition in Ytterbium (Yb+) at 369.53 nm and its repetition rate can be scaled up using high harmonic mode locking. We show that our source can produce arbitrary pulse patterns using a programmable pulse pattern generator and fast modulating components. Finally, simulations demonstrate that our laser is capable of performing resonant, temperature-insensitive, two-qubit quantum logic gates on trapped Yb$^+$ ions faster than the trap period and with fidelity above 99%.

We study and demonstrate the frequency conversion of UV radiation, resonant with 369.5 nm transition in Yb+ ions to the C-band wavelength 1580.3 nm and vice-versa using a reverse proton-exchanged waveguide in periodically poled lithium niobate. Our integrated device can interface trapped Yb+ ions with telecom infrastructure for the realization of an Yb+ based quantum repeater protocol and to efficiently distribute entanglement over long distances. We analyse the single photon frequency conversion efficiency from the 369.525 nm to the telecom wavelength and its dependence on pump power, device length and temperature. The single-photon noise generated by spontaneous Raman scattering of the pump is also measured. From this analysis we estimate a single photon conversion efficiency of 9% is achievable with our technology with almost complete suppression of the Raman noise.

Full quantum state tomography (FQST) plays a unique role in the estimation of the state of a quantum system without \emph{a priori} knowledge or assumptions. Unfortunately, since FQST requires informationally (over)complete measurements, both the number of measurement bases and the computational complexity of data processing suffer an exponential growth with the size of the quantum system. A 14-qubit entangled state has already been experimentally prepared in an ion trap, and the data processing capability for FQST of a 14-qubit state seems to be far away from practical applications. In this paper, the computational capability of FQST is pushed forward to reconstruct a 14-qubit state with a run time of only 3.35 hours using the linear regression estimation (LRE) algorithm, even when informationally overcomplete Pauli measurements are employed. The computational complexity of the LRE algorithm is first reduced from $O(10^{19})$ to $O(10^{15})$ for a 14-qubit state, by dropping all the zero elements, and its computational efficiency is further sped up by fully exploiting the parallelism of the LRE algorithm with parallel Graphic Processing Unit (GPU) programming. Our result can play an important role in quantum information technologies with large quantum systems.

Driven dissipative steady state entanglement schemes take advantage of coupling to the environment to robustly prepare highly entangled states. We present a scheme for two trapped ions to generate a maximally entangled steady state with fidelity above 0.99, appropriate for use in quantum protocols. Furthermore, we extend the scheme by introducing detection of our dissipation process, significantly enhancing the fidelity. Our scheme is robust to anomalous heating and requires no sympathetic cooling.

We present a fast phase gate scheme that is experimentally achievable and has an operation time more than two orders of magnitude faster than current experimental schemes for low numbers of pulses. The gate time improves with the number of pulses following an inverse power law. Unlike implemented schemes which excite precise motional sidebands, thus limiting the gate timescale, our scheme excites multiple motional states using discrete ultra-fast pulses. We use beam-splitters to divide pulses into smaller components to overcome limitations due to the finite laser pulse repetition rate. This provides gate times faster than proposed theoretical schemes when we optimise a practical setup.

The conformational dynamics of biomolecules drives the chemistry of life. We propose trapping large biomolecular ions in a Paul trap to probe their dynamics and that of their surrounding solvent cage.

Fundamental optics such as lenses and prisms work by applying phase shifts to incoming light via the refractive index. In these macroscopic devices, many particles each contribute a miniscule phase shift, working together to impose a total phase shift of many radians. In principle, even a single isolated particle can apply a radian-level phase shift, but observing this phenomenon has proven challenging. We have used a single trapped atomic ion to induce and measure a large optical phase shift of $1.3 \pm 0.1$ radians in light scattered by the atom. Spatial interferometry between the scattered light and unscattered illumination light enables us to isolate the phase shift in the scattered component. The phase shift achieves the maximum value allowed by atomic theory over the accessible range of laser frequencies, validating the microscopic model that underpins the macroscopic phenomenon of the refractive index. Single-atom phase shifts of this magnitude open up new quantum information protocols, including long-range quantum phase-shift-keying cryptography [1,2] and quantum nondemolition measurement [3,4].

Absorption imaging has played a key role in the advancement of science from van Leeuwenhoek's discovery of red blood cells to modern observations of dust clouds in stellar nebulas and Bose-Einstein condensates. Here we show the first absorption imaging of a single atom isolated in vacuum. The optical properties of atoms are thoroughly understood, so a single atom is an ideal system for testing the limits of absorption imaging. A single atomic ion was confined in an RF Paul trap and the absorption imaged at near wavelength resolution with a phase Fresnel lens. The observed image contrast of 3.1(3)% is the maximum theoretically allowed for the imaging resolution of our setup. The absorption of photons by single atoms is of immediate interest for quantum information processing (QIP). Our results also point out new opportunities in imaging of light-sensitive samples both in the optical and x-ray regimes.

We demonstrate millikelvin thermometry of laser cooled trapped ions with high-resolution imaging. This equilibrium approach is independent of the cooling dynamics and has lower systematic error than Doppler thermometry, with \pm5 mK accuracy and \pm1 mK precision. We used it to observe highly anisotropic dynamics of a single ion, finding temperatures of < 60 mK and > 15 K simultaneously along different directions. This thermometry technique can offer new insights into quantum systems sympathetically cooled by ions, including atoms, molecules, nanomechanical oscillators, and electric circuits.

A microfabricated phase Fresnel lens was used to image ytterbium ions trapped in a radio frequency Paul trap. The ions were laser cooled close to the Doppler limit on the 369.5 nm transition, reducing the ion motion so that each ion formed a near point source. By detecting the ion fluorescence on the same transition, near diffraction limited imaging with spot sizes of below 440 nm (FWHM) was achieved. This is the first demonstration of imaging trapped ions with a resolution on the order of the transition wavelength.

Trapped ions are a leading system for realizing quantum information processing (QIP). Most of the technologies required for implementing large-scale trapped-ion QIP have been demonstrated, with one key exception: a massively parallel ion-photon interconnect. Arrays of microfabricated phase Fresnel lenses (PFL) are a promising interconnect solution that is readily integrated with ion trap arrays for large-scale QIP. Here we show the first imaging of trapped ions with a microfabricated in-vacuum PFL, demonstrating performance suitable for scalable QIP. A single ion fluorescence collection efficiency of 4.2 +/- 1.5% was observed, in agreement with the previously measured optical performance of the PFL. The contrast ratio between the ion signal and the background scatter was 23 +/- 4. The depth of focus for the imaging system was 19.4 +/- 2.4 μm and the field of view was 140 +/- 20 μm. Our approach also provides an integrated solution for high-efficiency optical coupling in neutral atom and solid state QIP architectures.

We stabilize an ultraviolet diode laser system at 369.5 nm to the optical absorption signal from Yb+ ions in a hollow-cathode discharge lamp. The error signal for stabilization is obtained by Zeeman spectroscopy of the 3 GHz-wide absorption feature. The frequency stability is independently measured by comparison against the fluorescence signal from a laser-cooled crystal of 174Yb+ ions in a linear Paul trap. We measure a frequency fluctuation of 1.7 MHz RMS over 1000 s, and a frequency drift of 20 MHz over 7 days. Our method is suitable for use in quantum information processing experiments with trapped ion crystals.

Following on from previous work [J. A. Larsson, Phys. Rev. A 67, 022108 (2003)], Bell inequalities based on correlations between binary digits are considered for a particular entangled state involving 2N trapped ions. These inequalities involve applying displacement operations to half of the ions and then measuring correlations between pairs of corresponding bits in the binary representations of the number of centre-of-mass phonons of N particular ions. It is shown that the state violates the inequalities and thus displays nonclassical correlations. It is also demonstrated that it violates a Bell inequality when the displacements are replaced by squeezing operations.