Mukaiyama Laboratory

We developed a surface-electrode ion trap with a square hole measuring $40\,\mathrm{μm}$ for atomic loading. The hole was fabricated using anisotropic etching of a silicon substrate and was designed to minimize potential distortion in the trapping region. By introducing the atomic beam through the hole, we achieved enhanced isotope selectivity and experimentally demonstrated the selective trapping of calcium isotope ions using an atomic oven. We successfully prepared isotope ion pairs directly from the oven via sympathetic cooling at a rate comparable to that achieved using ablation loading. The sympathetic cooling process occurred on the order of a few seconds. We demonstrated the direct generation of an ion chain above the through-hole. This approach can be applied for trapping a wide range of ion species using a remarkably simple experimental setup, making it desirable for several applications such as quantum-charge-coupled-device (QCCD) architectures and precision measurements of isotope shifts.

The quantum charge-coupled device (QCCD) is one of the notable architectures to achieve large-scale trapped-ion quantum computers. To realize QCCD architecture, ions must be transported quickly while minimizing motional excitation. High-voltage sources are necessary to achieve such high-quality ion transport through a high secular frequency. In this study, we report the development of a field programmable gate array (FPGA)-based digital-to-analog converter (DAC) system with an output voltage range of +/-50 V and demonstrate its effectiveness in ion transport operations. The device provides 16-channel analog output, maximum update rate of 16 mega updates per second (MUPS), slew rate of 20 V/us, and bandwidth of > 200 kHz. By optimizing the voltage sets with quadratic programming, we experimentally confirmed that this DAC system can achieve more than twice the secular frequency attainable when its output range is restricted to +/-10 V, which is consistent with the fact that scaling all electrode voltages by a factor of 5 will scale the secular frequency by the square root of 5. Since the output range of many commercially available DACs is commonly limited to +/-10 V, this increase is effective for ion shuttling operations, such as transport, split and merge. The developed DAC system has potential to increase the speed of ion transport thereby reducing processing times in QCCD-based quantum computers.

In some types of mass spectrometers, such as Time of Flight mass spectrometers (TOF-MSs), it is necessary to control pulsed beams of ions. This can be easily accomplished by applying a pulsed voltage to the pusher electrode while the ionizer is continuously flowing ions. This method is preferred for its simplicity, although the ion utilization efficiency is not optimized. Here we employed another pulse-control method with a higher ion utilization rate, which is to bunch ions and kick them out instead of letting them stream. The benefit of this method is that higher sensitivity can be achieved; since the start of new ions cannot be allowed during TOF separation, it is highly advantageous to bunch ions that would otherwise be unusable. In this study, we used analytical and numerical methods to design a new bunching ionizer with reduced resources, adopting the principle of electrostatic ion beam trap. The test model experimentally demonstrated the bunching performance with respect to sample gas density and ion bunching time using gas samples and electron impact ionization. We also conducted an experiment in connection with a miniature TOF-MS, and showed that the sensitivity was improved by more than one order of magnitude using the newly developed ionizer. Since the device is capable of bunching ions with lower voltage and lower power consumption (~100 V, ~0.8 W) compared with conventional RF ion trap bunchers (several kilovolts, ~10 W), it will be possible to find applications in portable mass spectrometer with reduced resources.

We systematically investigate local phonon hopping in the radial direction of a linear trapped-ion string. We measure the decay of hopping as a function of key trap parameters and analyze the results in terms of the decay time and the number of oscillations. We attribute the loss of coherence to nonlinear coupling between different modes. Despite quantitative differences, the overall trends in our numerical simulations are similar to those of the experimental results. This work establishes a method for evaluating phonon hopping coherence and provides insight into the underlying decoherence mechanisms.

Quantum approximate optimization algorithm (QAOA) has attracted much attention as an algorithm that has the potential to efficiently solve combinatorial optimization problems. Among them, a fermionic QAOA (FQAOA) for solving constrained optimization problems has been developed [Yoshioka, Sasada, Nakano, and Fujii, Phys. Rev. Research vol. 5, 023071, 2023]. In this algorithm, the constraints are essentially imposed as fermion number conservation at arbitrary approximation level. We take the portfolio optimization problem as an application example and propose a new driver Hamiltonian on an one-dimensional cyclic lattice. Our FQAOA with the new driver Hamiltonian reduce the number of gate operations in quantum circuits. Experiments on a trapped-ion quantum computer using 16 qubits on Amazon Braket demonstrates that the proposed driver Hamiltonian effectively suppresses noise effects compared to the previous FQAOA.

We demonstrate the site-dependent control of polaritons in the Jaynes Cummings Hubbard (JCH) model with trapped ions. In a linear ion crystal under illumination by optical beams nearly resonant to the red-sideband (RSB) transition for the radial vibrational direction, quasiparticles called polaritonic excitations or polaritons, each being a superposition of one internal excitation and one vibrational quantum (phonon), can exist as conserved particles. Polaritons can freely hop between ion sites in a homogeneous configuration, while their motion can be externally controlled by modifying the parameters for the optical beams site-dependently. We demonstrate the blockade of polariton hopping in a system of two ions by the individual control of the frequency of the optical beams illuminating each ion. A JCH system consisting of polaritons in a large number of ion sites can be considered an artificial many-body system of interacting particles and the technique introduced here can be used to exert fine local control over such a system, enabling detailed studies of both its quasi-static and dynamic properties.

In this paper, we present a dynamical decoupling (DD) technique to coherently control the dynamics of a single local phonon in trapped ions. A 2$π$ rotation at a motional sideband transition flips the sign of the relevant local phonon state, resulting in cancellation of the phonon dynamics. In this work, we implement DD using single and multiple blue-sideband pulses to control a single local phonon in two $^{40}{\rm Ca}^{+}$ ions in a linear Paul trap. Our proposed DD technique can be used to engineer coupling between local phonon modes.

We propose and demonstrate a scalable scheme for the simultaneous determination of internal and motional states in trapped ions with single-site resolution. The scheme is applied to the study of polaritonic excitations in the Jaynes- Cummings Hubbard model with trapped ions, in which the internal and motional states of the ions are strongly correlated. We observe quantum phase transitions of polaritonic excitations in two ions by directly evaluating their variances per ion site. Our work establishes an essential technological method for large-scale quantum simulations of polaritonic systems.

We demonstrate the generation of a trapped ion oscillator having large oscillation amplitude of $16.9~{\rm μm}$. Applying an offset voltage to the ion trap electrode helped achieve a displacement of the trap center within the time scale of 5 ns. The fluorescence dynamics of the ion were analyzed after the displacement to estimate the oscillation amplitude. The realized trap displacement is one order magnitude larger than that achieved in the previous work. Thus, this result is an important step toward the realization of a gyroscope using a single trapped ion.

We have experimentally observed the dynamics of a single polariton and two polaritons in a two-ion chain. By driving two trapped ions at a motional blue-sideband transition, we realize the anti-Jaynes-Cummings-Hubbard model. When a single polariton exists in a trapped-ion chain, the polariton hops between the ion sites. On the other hand, when there are single polaritons at each ion site, the hopping of the polaritons is suppressed because of the polariton-polariton interaction induced by the nonlinearity of the anti-Jaynes-Cummings interaction, thereby realizing the blockade of polariton hopping in the anti-Jaynes-Cummings-Hubbard model with trapped ions. Our work is a step towards the development of a trapped-ion based quantum simulator for strongly interacting polaritonic systems.

We demonstrate a method of micromotion minimization of a trapped ion in a linear Paul trap based on the precision measurement of the ion trapping position displacement due to a stray electric field in the radial plane by ion fluorescence imaging. The amount of displacement in the radial plane is proportional to the strength of a stray electric field. Therefore, we evaluated the micromotion compensation condition by measuring the ion displacements from the ion equilibrium position using two different radial trap frequencies with various combinations of the compensation voltage. The residual electric field uncertainty of this technique reached a few volts per meter. This compensation technique does not depend on the orientation of the incident cooling laser or the detuning and imaging direction. Therefore, this method is suitable for a planar ion trap, a stylus ion trap, which limits the propagation angle of lasers, or miniaturized ion trap systems for sensing and metrological applications.

We demonstrate a microfabricated surface-electrode ion trap that is applicable as a nanofriction emulator and studies of many-body dynamics of interacting systems. The trap enables both single-well and double-well trapping potentials in the radial direction, where the distance between the two potential wells can be adjusted by the applied RF voltage. In the double-well configuration, parallel ion strings can be formed, which is a suitable system for the emulation of the Frenkel-Kontorova (FK) model. We derive the condition under which the trap functions as a FK model emulator. The trap is designed so that the Coulomb interaction between two ion strings becomes significant. We report on the microfabrication process for such downsized trap electrodes and experimental results of single-well and double-well operation with calcium ions. With the trap demonstrated in this work we can create atomically accessible, self-assembled Coulomb systems with a wide tuning range of the corrugation parameter in the FK model. This makes it a promising system for quantum simulations, but also for the study of nanofriction in one and higher dimensional systems.

We report on a demonstration of Ramsey interferometry by three-dimensional motion with a trapped $^{171}Yb^+$ ion. We applied a momentum kick to the ion in a direction diagonal to the trap axes to initiate three-dimensional motion using a mode-locked pulse laser. The interference signal was analyzed theoretically to demonstrate three-dimensional matter-wave interference. This work paves the way to realizing matter-wave interferometry using trapped ions.

Driving an ion at a motional sideband transition induces the Jaynes--Cummings (JC) interaction. This JC interaction creates an anharmonic ladder of JC eigenstates, resulting in the suppression of phonon hopping due to energy conservation. Here, we realize phonon blockade in the presence of multiple local phonons in a trapped-ion chain. Our work establishes a key technological component for quantum simulation with multiple bosonic particles, which can simulate classically intractable problems.

Incorporating optical cavities in ion traps is becoming increasingly important in the development of photonic quantum networks. However, the presence of the cavity can hamper efficient laser cooling of ions because of geometric constraints that the cavity imposes and an unfavourable Purcell effect that can modify the cooling dynamics substantially. On the other hand the coupling of the ion to the cavity can also be exploited to provide a mechanism to efficiently cool the ion. In this paper we demonstrate experimentally how cavity cooling can be implemented to improve the localisation of the ion and thus its coupling to the cavity. By using cavity cooling we obtain an enhanced ion-cavity coupling of $2π\times (16.7\pm 0.1)$ MHz, compared with $2π\times (15.2\pm 0.1)$ MHz when using only Doppler cooling.

We propose and demonstrate phonon-number-resolving detection of the multiple local phonon modes in a trapped-ion chain. To mitigate the effect of phonon hopping during the detection process, the probability amplitude of each local phonon mode is mapped to the auxiliary long-lived motional ground states. Sequential state-dependent fluorescence detection is then performed. In the experiment, we have successfully observed the time evolution of two local phonon modes in two ions, including the phonon-number correlation between the two modes.

The excitation efficiency and external luminescence quantum efficiency of trivalent Eu3+ ions doped into gallium nitride (GaN) was studied under optical and electrical excitation. For small pump fluences it was found that the excitation of Eu3+ ions is limited by an efficient carrier trap that competes in the energy transfer from the host material. For large pump fluences the limited number of high-efficiency Eu3+ sites, and the small excitation cross-section of the majority Eu3+ site, limit the quantum efficiency. At low temperatures under optimal excitation conditions, the external luminescence quantum efficiency reached a value of 46%. These results show the high potential for this material as an efficient light emitter, and demonstrates the importance of the excitation conditions on the light output efficiency.

Propagation and interference of quantum-mechanical particles comprise an important part of elementary processes in quantum physics, and their essence can be modeled using a quantum walk, a mathematical concept that describes the motion of a quantum-mechanical particle among discretized spatial regions. Here we report the observation of the quantum walks of a phonon, a vibrational quantum, in a trapped-ion crystal. By employing the capability of preparing and observing a localized wave packet of a phonon, the propagation of a single radial local phonon in a four-ion linear crystal is observed with single-site resolution. The results show an agreement with numerical calculations, indicating the predictability and reproducibility of the phonon system. These characteristics may contribute advantageously in advanced experimental studies of quantum walks with large numbers of nodes, as well as realization of boson sampling and quantum simulation using phonons as computational resources.

A trapped-ion quantum tunneling rotor (QTR) is in a quantum superposition of two different Wigner crystal orientations. In a QTR system, quantum tunneling drives the coherent transition between the two different Wigner crystal orientations. We theoretically study the quantum dynamics of a QTR, particularly when the spin state of one of the ions is flipped. We show that the quantum dynamics of an $\it{N}$-ion QTR can be described by continuous-time cyclic quantum walks. We also investigate the quantum dynamics of the QTR in a magnetic field. Flipping the spin state breaks the rotational symmetry of the QTR, making the quantum-tunneling-induced rotation distinguishable. This symmetry breaking creates coupling between the spin state of the ions and the rotational motion of the QTR, resulting in different quantum tunneling dynamics.

Trapped atomic ions are ideal single photon emitters with long lived internal states which can be entangled with emitted photons. Coupling the ion to an optical cavity enables efficient emission of single photons into a single spatial mode and grants control over their temporal shape. These features are key for quantum information processing and quantum communication. However, the photons emitted by these systems are unsuitable for long-distance transmission due to their wavelengths. Here we report the transmission of single photons from a single $^{40}\text{Ca}^{+}$ ion coupled to an optical cavity over a 10 km optical fibre via frequency conversion from 866 nm to the telecom C-band at 1,530 nm. We observe non-classical photon statistics of the direct cavity emission, the converted photons and the 10 km transmitted photons, as well as the preservation of the photons' temporal shape throughout. This telecommunication ready system can be a key component for long-distance quantum communication as well as future cloud quantum computation.

We demonstrated sympathetic cooling of a single ion in a buffer gas of ultracold atoms with small mass. Efficient collisional cooling was realized by suppressing collision-induced heating. We attempt to explain the experimental results with a simple rate equation model and provide a quantitative discussion of the cooling efficiency per collision. The knowledge we obtained in this work is an important ingredient for advancing the technique of sympathetic cooling of ions with neutral atoms.

We report on a surface-electrode trap with SmCo magnets arranged in a quadrupole configuration underneath the trap electrode. Because the distance between the magnets and the trapped ions can be as little as several hundred micrometers, a large magnetic field is produced without any heat management. The magnetic-field gradient was measured using the Zeeman splitting of a single trapped $^{40}$Ca$^+$ ion at several positions, and a field gradient of 36 T/m was obtained. Such a field gradient is useful for the generation of a state-dependent force, which is important for quantum simulation and/or quantum gate operation using radio-frequency or microwave radiation.

We present a novel method of machining optical fiber surfaces with a CO${}_2$ laser for use in Fiber-based Fabry-Perot Cavities (FFPCs). Previously FFPCs were prone to large birefringence and limited to relatively short cavity lengths ($\le$ 200 $μ$m). These characteristics hinder their use in some applications such as cavity quantum electrodynamics with trapped ions. We optimized the laser machining process to produce large, uniform surface structures. This enables the cavities to achieve high finesse even for long cavity lengths. By rotating the fibers around their axis during the laser machining process the asymmetry resulting from the laser's transverse mode profile is eliminated. Consequently we are able to fabricate fiber mirrors with a high degree of rotational symmetry, leading to remarkably low birefringence. Through measurements of the cavity finesse over a range of cavity lengths and the polarization dependence of the cavity linewidth, we confirmed the quality of the produced fiber mirrors for use in low-birefringence FFPCs.

We report an experimental realization of the Jaynes-Cummings-Hubbard (JCH) model using the internal and radial phonon states of two trapped ions. An adiabatic transfer corresponding to a quantum phase transition from a localized insulator ground state to a delocalized superfluid (SF) ground state is demonstrated. The SF phase of polaritonic excitations characteristic of the interconnected Jaynes-Cummings (JC) system is experimentally explored, where a polaritonic excitation refers to a combination of an atomic excitation and a phonon interchanged via a JC coupling.

We determine the minimal number of qubits that it is necessary to have access to in order to transform Dicke states into other Dicke states. In general, the number of qubits in Dicke states cannot be increased via transformation gates by accessing only a single qubit, in direct contrast to other multipartite entangled states such as GHZ, W and cluster states. We construct a universal optimal gate which adds spin-up qubits or spin-down qubits to any Dicke state by minimal access. We also show the existence of a universal gate which transforms any size of Dicke state as long as it has access to at least the required number of qubits. Our results have important consequences for the generation of Dicke states in physical systems such as ion traps, all-optical setups and cavity-QED settings where they can be used for a variety of quantum information processing tasks.

Universal single-qubit operations based on purely geometric phase factors in adiabatic processes are demonstrated by utilizing a four-level system in a trapped single $^{40}$Ca$^+$ ion connected by three oscillating fields. Robustness against parameter variations is studied. The scheme demonstrated here can be employed as a building block for large-scale holonomic quantum computations, which may be useful for large qubit systems with statistical variations in system parameters.

We propose a method for generating a spin-squeezed state that is a symmetric Dicke state, with trapped ions using only global access. The eigenstates of the ions under a strong dressing field become symmetric Dicke states and the M$ø$lmer--S$ø$rensen interaction selectively couples one of them to an initially populated auxiliary state. A $\mid D_{2n}^n>$ state, which is maximally spin squeezed, can be generated with high fidelity using only square pulses. Using an adiabatic technique, the ideal maximally spin-squeezed state is generated.

We propose the generation of entangled states with trapped calcium ions using a combination of an rf dressed state and a spin dependent force. Using this method, a decoherence-free entangled state of rf qubits can be directly generated and ideally its fidelity is close to unity. We demonstrate an rf entangled state with a fidelity of 0.68, which has a coherence time of more than 200 ms by virtue of the fact that it is an eigenstate with energy gaps between adjacent levels.Using the same technique, we also produce a qutrit-qutrit entangled state with a fidelity of 0.77, which exceeds the threshold value for separability of 2/3.

A two-qubit quantum gate is realized using electronic excited states in a single ion with an energy separation on the order of a terahertz times the Planck constant as a qubit. Two phase locked lasers are used to excite a stimulated Raman transition between two metastable states $D_{3/2}$ and $D_{5/2}$ separated by 1.82 THz in a single trapped $^{40}$Ca$^+$ ion to construct a qubit, which is used as the target bit for the Cirac-Zoller two-qubit controlled NOT gate. Quantum dynamics conditioned on a motional qubit is clearly observed as a fringe reversal in Ramsey interferometry.

We introduce three compact graph states that can be used to perform a measurement-based Toffoli gate. Given a weighted graph of six, seven or eight qubits, we show that success probabilities of 1/4, 1/2 and 1 respectively can be achieved. Our study puts a measurement-based version of this important quantum logic gate within the reach of current experiments. As the graphs are setup-independent, they could be realized in a variety of systems, including linear optics and ion-traps.