Dipti

Extreme Ultraviolet Spectroscopy of Highly Charged Lu and Yb Ions for Nuclear Charge Radius Determination

Hunter Staiger, Endre Takacs, Steven A. Blundell, Naoki Kimura, Hiroyuki A. Sakaue, Ronald F. Garcia Ruiz, Witold Nazarewicz, Paul-Gerhard Reinhard, Chowdhury A. Faiyaz, Chihiro Suzuki, Dipti [1,7,8,9,10,2,11,12], István Angeli, Yuri Ralchenko, Izumi Murakami, Daiji Kato, Yuki Nagai, Ryuji Takaoka, Yoshiki Miya, Nobuyuki Nakamura

Abstract

We report a high-precision determination of the natural-abundance-averaged nuclear charge-radius difference between Yb and Lu using extreme ultraviolet (EUV) spectroscopy of highly charged ions (HCIs). By measuring the $D_1$ transition energies in Na- and Mg-like charge states of Lu and Yb confined in the Tokyo electron-beam ion trap, we extract meV-level energy shifts that are directly sensitive to nuclear-size effects. Transition-energy differences obtained from these spectra are compared with state-of-the-art relativistic many-body perturbation theory, including a new treatment of Mg-like ions. We develop a generalized framework to propagate uncertainties arising from nuclear deformation and surface diffuseness and evaluate corresponding nuclear-sensitivity coefficients. Combining Na- and Mg-like results yields mutually consistent radius differences, demonstrating the robustness of both the experimental calibration and the theoretical predictions. To determine absolute isotopic radii, we perform a generalized least-squares optimization incorporating our HCI constraints together with optical-isotope-shift data and muonic-atom results. This analysis establishes that the $^{175}$Lu charge radius is smaller than that of $^{174}$Yb, restoring the expected odd-even staggering across the $N=94$ isotonic chain. Our recommended value, $R(^{175}\text{Lu}) = 5.291(11)$ fm, reduces the uncertainty of the Lu radius by a factor of three compared with the previous electron-scattering result and resolves a long-standing anomaly in rare-earth nuclear systematics. This work demonstrates that EUV spectroscopy of HCIs provides a powerful and broadly applicable method for precision nuclear-structure studies in heavy, deformed nuclei. The techniques developed here enable future investigations of isotonic and isoelectronic sequences, including radioactive nuclides and higher-$Z$ systems.

Dielectronic resonances of LMn and LNn (n $\geq$ 4) series in highly-charged M-shell tungsten ions

Dipti [1], A. Borovik [1], R. Silwal [1,2], J. M. Dreiling, A. C. Gall, E. Takacs [1,2], Yu. Ralchenko [1]

Abstract

We present spectroscopic measurements and detailed theoretical analysis of inner-shell LMn and LNn (n $\geq$ 4) dielectronic resonances in highly-charged M-shell ions of tungsten. The x-ray emission from W$^{49+}$ through W$^{64+}$ was recorded at the electron beam ion trap (EBIT) facility at the National Institute of Standards and Technology (NIST) with a high-purity Ge detector for electron beam energies between 6.8 keV and 10.8 keV. The measured spectra clearly show the presence of strong resonance features as well as direct excitation spectral lines. The analysis of the recorded spectra with large-scale collisional-radiative (CR) modeling of the EBIT plasma allowed us to unambiguously identify numerous dielectronic resonances associated with excitations of the inner-shell 2s$_{1/2}$, 2p$_{1/2}$, and 2p$_{3/2}$ electrons.

Measuring the Variation in Nuclear Charge Radius of Xe Isotopes by EUV Spectroscopy of Highly-Charged Na-like Ions

R. Silwal [1,2], A. Lapierre [3,2,4,5], J. D. Gillaspy, J. M. Dreiling, S. A. Blundell, Dipti [2], A. Borovik [2], G. Gwinner [6,3], A. C. C. Villari, Yu. Ralchenko [2], E. Takacs [1,2]

Abstract

The variation in mean-square nuclear charge radius of xenon isotopes was measured utilizing a new method based on extreme ultraviolet spectroscopy of highly charged Na-like ions. The isotope shift of the Na-like D1 (3s $^{2}$S$_{1/2}$ - 3p $^2$P$_{1/2}$) transition between the $^{124}$Xe and $^{136}$Xe isotopes was experimentally determined using the electron beam ion trap facility at the National Institute of Standards and Technology. The mass shift and the field shift coefficients were calculated with enhanced precision by relativistic many-body perturbation theory and multi-configuration Dirac-Hartree-Fock method. The mean-square nuclear charge radius difference was found to be $δ<r^2>^{136, 124}$ = 0.269(0.042) fm$^2$. Our result has smaller uncertainty than previous experimental results and agrees with the recommended value by Angeli and Marinova [I. Angeli and K. P. Marinova, At. Data and Nucl. Data Tables {\bf 99}, 69-95 (2013)].