I. Lesanovsky

Trapped ions are a versatile platform for the investigation of quantum many-body phenomena, in particular for the study of scenarios where long-range interactions are mediated by phonons. Recent experiments have shown that the trapped ion platform can be augmented by exciting high-lying Rydberg states. This introduces controllable state-dependent interactions that are independent from the phonon structure. However, the many-body physics in this newly accessible regime is largely unexplored. We show that this system grants access to generalized Dicke model physics, where dipolar interactions between ions in Rydberg states drastically alter the collective non-equilibrium behavior. We analyze and classify the emerging dynamical phases and identify a host of non-equilibrium signatures such as multi-phase coexistence regions and phonon-lasing regimes. We moreover show how they can be detected and characterized through the fluorescence signal of scattered photons. Our study thus highlights new capabilities of trapped Rydberg ion systems for creating and detecting quantum non-equilibrium phases.

We provide a detailed theoretical and conceptual study of a planned experiment to excite Rydberg states of ions trapped in a Paul trap. The ultimate goal is to exploit the strong state dependent interactions between Rydberg ions to implement quantum information processing protocols and to simulate the dynamics of strongly interacting spin systems. We highlight the promises of this approach when combining the high degree of control and readout of quantum states in trapped ion crystals with the novel and fast gate schemes based on interacting giant Rydberg atomic dipole moments. We discuss anticipated theoretical and experimental challenges on the way towards its realization.

We study two ions confined in a Penning trap. We show that electronically highly excited states exist in which an electron is delocalized among the two ions forming a giant molecule of several micrometer size. At energies close to the top of the Coulomb barrier these molecular states can be regarded as superpositions of Rydberg states of individual ions. We illuminate the possibility to observe coherent charge transfer between the ions. Beyond a critical principal quantum number the electron can coherently tunnel through the Coulomb barrier to an adjacent doubly charged ion. The tunneling occurs on timescales on which the dynamics of the nuclei can be considered frozen and radiative decay can be neglected.

We study the dynamics of Rydberg ions trapped in a linear Paul trap, and discuss the properties of ionic Rydberg states in the presence of the static and time-dependent electric fields constituting the trap. The interactions in a system of many ions are investigated and coupled equations of the internal electronic states and the external oscillator modes of a linear ion chain are derived. We show that strong dipole-dipole interactions among the ions can be achieved by microwave dressing fields. Using low-angular momentum states with large quantum defect the internal dynamics can be mapped onto an effective spin model of a pair of dressed Rydberg states that describes the dynamics of Rydberg excitations in the ion crystal. We demonstrate that excitation transfer through the ion chain can be achieved on a nanosecond timescale and discuss the implementation of a fast two-qubit gate in the ion chain.