Jean-Pierre Likforman

Laser-cooled trapped ions are at the heart of modern quantum technologies and their cooling dynamics often deviate from the simplified two-level atom model. Doppler cooling of the $^{88}$Sr$^{+}$ ion involves several electronic levels and repumping channels that strongly influence fluorescence. In this work, we study a repumping scheme for the $^{88}$Sr$^{+}$ ion by combining precision single-ion spectroscopy with comprehensive numerical modeling based on optical Bloch equations including 18 Zeeman sublevels. We show that, although the observed fluorescence spectra retain a Lorentzian lineshape, their width and amplitude cannot be explained by a two-level atom description. Moreover, we find the optimal repumping conditions for maximizing the photon scattering rate.

We describe and experimentally implement a single-ion local thermometry technique with absolute sensitivity adaptable to all laser-cooled atomic ion species. The technique is based on the velocity-dependent spectral shape of a quasi-dark resonance tailored in a J $\rightarrow$ J transition such that the two driving fields can be derived from the same laser source leading to a negligible relative phase shift. We validated the method and tested its performances in an experiment on a single 88 Sr + ion cooled in a surface radio-frequency trap. We first applied the technique to characterise the heating-rate of the surface trap. We then measured the stationary temperature of the ion as a function of cooling laser detuning in the Doppler regime. The results agree with theoretical calculations, with an absolute error smaller than 100 $μ$K at 500 $μ$K, in a temperature range between 0.5 and 3 mK and in the absence of adjustable parameters. This simple-to-implement and reliable method opens the way to fast absolute measurements of single-ion temperatures in future experiments dealing with heat transport in ion chains or thermodynamics at the single-ion level.

We measured the branching fractions for the decay of the 5p 2 P 1/2 state of 88 Sr + by applying a recently demonstrated photon-counting sequential method (M. Ramm et al., Phys. Rev. Lett. 111, 023004) to a single ion laser-cooled in a micro fabricated surface trap. The branching fraction for the decay into the 5s 2 S 1/2 ground level was found to be p = 0.9453 +0.0007 --0.0005. This result is in good agreement with recent theoretical calculations but disagrees with previous experimental measurements, however affected by a one order of magnitude larger uncertainty. This experiment also demonstrates the reliability and the performances of ion micro trap technology in the domain of precision measurements and spectroscopy. PACS numbers: 32.70.Cs, 06.30.Ft, 37.10.Ty

We measured by laser spectroscopy the isotope shifts between naturally-occurring even-isotopes of strontium ions for both the $5s\,\,^2S_{1/2}\to 5p\,\,^2P_{1/2}$ (violet) and the $4d\,\,^2D_{3/2}\to 5p\,\,^2P_{1/2}$ (infrared) dipole-allowed optical transitions. Fluorescence spectra were taken by simultaneous measurements on a two-component Coulomb crystal in a linear Paul trap containing $10^3$--$10^4$ laser-cooled Sr$^+$ ions. The isotope shifts are extracted from the experimental spectra by fitting the data with the analytical solution of the optical Bloch equations describing a three-level atom in interaction with two laser beams. This technique allowed us to increase the precision with respect to previously reported data obtained by optogalvanic spectroscopy or fast atomic-beam techniques. The results for the $5s\,\,^2S_{1/2}\to 5p\,\,^2P_{1/2}$ transition are $ν_{88}-ν_{84}=+378(4)$ MHz and $ν_{88}-ν_{86}=+170(3)$ MHz, in agreement with previously reported measurements. In the case of the previously unexplored $4d\,\,^2D_{3/2}\to 5p\,\,^2P_{1/2}$ transition we find $ν_{88}-ν_{84}=-828(4)$ MHz and $ν_{88}-ν_{86}=-402(2)$ MHz. These results provide more data for stringent tests of theoretical calculations of the isotope shifts of alkali-metal-like atoms. Moreover, they simplify the identification and the addressing of Sr$^+$ isotopes for ion frequency standards or quantum-information-processing applications in the case of multi-isotope ion strings.

This paper reports on photoionisation loading based on ultrafast pulses of singly-ionised strontium ions in a linear Paul trap. We take advantage of an autoionising resonance of Sr neutral atoms to form Sr+ by two-photon absorption of femtosecond pulses at a wavelength of 431nm. We compare this technique to electron-bombardment ionisation and observe several advantages of photoionisation. It actually allows the loading of a pure Sr+ ion cloud in a low radio-frequency voltage amplitude regime. In these conditions up to 4x10^4 laser-cooled Sr+ ions were trapped.