John J. Bollinger

Penning ion traps as quantum platforms have primarily utilized global control and symmetric Dicke states for quantum simulation and sensing experiments. The introduction of local control greatly increases the power of the platform as a quantum simulator but is technically challenging due to the rapid rotation of the ion crystals. Here we use an ultraviolet-compatible spatial light modulator (SLM) to imprint programmable AC Stark shift patterns with different azimuthal symmetries and gradients that co-rotate with the ion crystals, demonstrating localized coherent control of single plane crystals with greater than 100 ions. Comparisons of the measured ion qubit populations with calculations from independent measurements of the applied AC Stark shift patterns show good agreement, validating the technique and providing a path, with a higher format SLM, for parallelizable, coherent individual ion addressing in Penning traps.

Large, 3D trapped ion crystals offer improved sensitivity in quantum sensing protocols, and are expected to be implemented as platforms in near-future experiments. However, numerical techniques used to study the laser cooling of such crystals are inefficient as the number of ions, $N$, in the crystal increases. Here we develop a powerful numerical framework to simulate laser cooling of up to $10^5$ ions stored in a Penning trap. We apply this framework to characterize and optimize the cooling of ellipsoidal 3D crystals. We document new pathways to enhanced cooling based on the addition of an axial component to the potential energy-dominated $\boldsymbol{E}\times\boldsymbol{B}$ modes. Furthermore, we observe greatly enhanced cooling of the perpendicular kinetic energy to below 1 mK in prolate ion crystals, enabling a simplified cooling beam setup for such crystals. We propose specific values of trap and laser beam parameters which lead to optimal cooling in a variety of examples. This work illustrates the feasibility of preparing large 3D crystals for high-sensitivity quantum science protocols, motivating their use in future experiments.

Quantum many-body systems driven far from equilibrium can exhibit chaos, entanglement, and non-classical correlations, yet directly observing these phenomena in large, closed quantum systems remains challenging. Here we realize the Dicke model -- a fundamental description of light-matter interactions -- in a two-dimensional crystal of approximately 100 trapped ions. The ions' internal state is optically coupled to the center of mass vibrational mode via an optical spin-dependent force, enabling unitary many-body dynamics beyond the mean-field and few-body limits. In the integrable regime, where the phonons can be adiabatically eliminated, we observe a dynamical phase transition between ferromagnetic to paramagnetic spin phases. In contrast, when the spins and phonons are strongly coupled, we observe clear signatures of non-integrable chaotic dynamics, including erratic phase-space trajectories and the exponential growth of excitations and entanglement quantified by the one-body Rényi entropy. By quenching from an unstable fixed point in the near-integrable regime, quantum noise can generate correlated spin-phonon excitations. Our numerical calculations, in clear agreement with experiment, reveal the generation of two-mode spin-phonon squeezing, 2.6 dB below the standard quantum limit (4.6 dB relative to the initial thermal state), followed by generalized vacuum Rabi collapses and revivals. Our results establish large ion crystals as scalable analog quantum simulators of non-equilibrium light-matter dynamics and provide a controlled platform for experimental studies of information scrambling and entanglement in closed many-body systems.

We develop a unified many-body theory of two-photon dark-state laser cooling, the workhorse for preparing trapped ions close to their motional quantum ground state. For ions with a $Λ$ level structure, driven by Raman lasers, we identify an ion-number-dependent crossover between weak and strong coupling where both the cooling rate and final temperature are simultaneously optimized. We obtain simple analytic results in both extremes: In the weak coupling limit, we show a Lorentzian spin-absorption spectrum determines the cooling rate and final occupation of the motional state, which are both independent of the number of ions. We also highlight the benefit of including an additional spin dependent force in this case. In the strong coupling regime, our theory reveals the role of collective dynamics arising from phonon exchange between dark and bright states, allowing us to explain the enhancement of the cooling rate with increasing ion number. Our analytic results agree closely with exact numerical simulations and provide experimentally accessible guidelines for optimizing cooling in large ion crystals, a key step toward scalable, high-fidelity trapped-ion quantum technologies.

Three-dimensional (3D) crystals offer a route to scale up trapped ion systems for quantum sensing and quantum simulation applications. However, engineering coherent spin-motion couplings and effective spin-spin interactions in large crystals poses technical challenges associated with decoherence and prolonged timescales to generate appreciable entanglement. Here, we explore the possibility to speed up these interactions in 3D crystals via parametric amplification. We derive a general Hamiltonian for the parametric amplification of spin-motion coupling that is applicable to crystals of any dimension in both rf Paul traps and Penning traps. Unlike in lower dimensional crystals, we find that the ability to faithfully (uniformly) amplify the spin-spin interactions in 3D crystals depends on the physical implementation of the spin-motion coupling. We consider the light-shift (LS) gate, and the so-called phase-insensitive and phase-sensitive Mølmer-Sørensen (MS) gates, and find that only the latter gate can be faithfully amplified in general 3D crystals. We discuss a situation where non-uniform amplification can be advantageous. We also reconsider the impact of counter-rotating terms on parametric amplification and find that they are not as detrimental as previous studies suggest.

Two-dimensional planar ion crystals in a Penning trap are a platform for quantum information science experiments. However, the low-frequency planar modes of these crystals are not efficiently cooled by laser cooling, which can limit the utility of the drumhead modes for quantum information processing. Recently, it has been shown that nonlinear mode coupling can enhance the cooling of the low-frequency planar modes. Here, we demonstrate in numerical simulations that this coupling can be dynamically tuned by adiabatically changing the rotation frequency of the ion crystal during experiments. Furthermore, we show that this technique can, in addition, produce lower temperatures for the low-frequency planar modes via an adiabatic cooling process. This result allows cooling of the planar modes to sub-millikelvin temperatures, resulting in improved spectral resolution of the drumhead modes at experimentally relevant rotation frequencies, which is crucial for quantum information processing applications.

We simulate the dynamics, including laser cooling, of 3D ion crystals confined in a Penning trap using a newly developed molecular dynamics-like code. The numerical integration of the ions' equations of motion is accelerated using the fast multipole method to calculate the Coulomb interaction between ions, which allows us to efficiently study large ion crystals with thousands of ions. In particular, we show that the simulation time scales linearly with ion number, rather than with the square of the ion number. By treating the ions' absorption of photons as a Poisson process, we simulate individual photon scattering events to study laser cooling of 3D ellipsoidal ion crystals. Initial simulations suggest that these crystals can be efficiently cooled to ultracold temperatures, aided by the mixing of the easily cooled axial motional modes with the low frequency planar modes. In our simulations of a spherical crystal of 1,000 ions, the planar kinetic energy is cooled to several millikelvin in a few milliseconds while the axial kinetic energy and total potential energy are cooled even further. This suggests that 3D ion crystals could be well-suited as platforms for future quantum science experiments.

Trapped ion systems are a leading platform for quantum information processing, but they are currently limited to 1D and 2D arrays, which imposes restrictions on both their scalability and their range of applications. Here, we propose a path to overcome this limitation by demonstrating that Penning traps can be used to realize remarkably clean bilayer crystals, wherein hundreds of ions self-organize into two well-defined layers. These bilayer crystals are made possible by the inclusion of an anharmonic trapping potential, which is readily implementable with current technology. We study the normal modes of this system and discover salient differences compared to the modes of single-plane crystals. The bilayer geometry and the unique properties of the normal modes open new opportunities, in particular in quantum sensing and quantum simulation, that are not straightforward in single-plane crystals. Furthermore, we illustrate that it may be possible to extend the ideas presented here to realize multilayer crystals with more than two layers. Our work increases the dimensionality of trapped ion systems by efficiently utilizing all three spatial dimensions and lays the foundation for a new generation of quantum information processing experiments with multilayer 3D crystals of trapped ions.

Improving coherence is a fundamental challenge in quantum simulation and sensing experiments with trapped ions. Here we discuss, experimentally demonstrate, and estimate the potential impacts of two different protocols that enhance, through motional parametric excitation, the coherent spin-motion coupling of ions obtained with a spin-dependent force. The experiments are performed on 2D crystal arrays of approximately one hundred $^9$Be$^+$ ions confined in a Penning trap. By modulating the trapping potential at close to twice the center-of-mass mode frequency, we squeeze the motional mode and enhance the spin-motion coupling while maintaining spin coherence. With a stroboscopic protocol, we measure $5.4 \pm 0.9$ dB of motional squeezing below the ground-state motion, from which theory predicts a $10$ dB enhancement in the sensitivity for measuring small displacements using a recently demonstrated protocol [Science $\textbf{373}$, 673 (2021)]. With a continuous squeezing protocol, we measure and accurately calibrate the parametric coupling strength. Theory suggests this protocol can be used to improve quantum spin squeezing, limited in our system by off-resonant light scatter. We illustrate numerically the trade-offs between strong parametric amplification and motional dephasing in the form of center-of-mass frequency fluctuations for improving quantum spin squeezing in our set-up.

Penning traps have been used for performing quantum simulations and sensing with hundreds of ions and provide a promising route toward scaling up trapped ion quantum platforms because of the ability to trap and control up to thousands of ions in 2D and 3D crystals. A leading source of decoherence in laser-based multiqubit operations on trapped ions is off-resonant spontaneous emission. While many trapped ion quantum computers or simulators utilize clock qubits, other systems rely on Zeeman qubits, which require a more complex calculation of this decoherence. We examine theoretically the impacts of spontaneous emission on quantum gates performed with trapped ions in a high magnetic field. We consider two types of gates -- light-shift and Molmer-Sorensen gates -- and compare the decoherence errors in each. We also compare different detunings, polarizations, and required intensities of the laser beams used to drive the gates. We show that both gates can have similar performance at their optimal operating conditions and examine the experimental feasibility of various operating points. By examining the magnetic field dependence of each gate, we demonstrate that when the $P$ state fine structure splitting is large compared to the Zeeman splittings, the theoretical performance of the Molmer-Sorensen gate is significantly better than that of the light-shift gate. Additionally, for the light-shift gate, we make an approximate comparison between the fidelities that can be achieved at high fields with the fidelities of state-of-the-art two-qubit trapped ion quantum gates. We show that, with regard to spontaneous emission, the achievable infidelity of our current configuration is about an order of magnitude larger than that of the best low-field gates, but we also discuss alternative configurations with potential error rates that are comparable with state-of-the-art trapped ion gates.

Two-dimensional $p+ i p$ superconductors and superfluids are systems that feature chiral behavior emerging from the Cooper pairing of electrons or neutral fermionic atoms with non-zero angular momentum. Their realization has been a longstanding goal because they offer great potential utility for quantum computation and memory. However, they have so far eluded experimental observation both in solid state systems as well as in ultracold quantum gases. Here, we propose to leverage the tremendous control offered by rotating two-dimensional trapped-ion crystals in a Penning trap to simulate the dynamical phases of two-dimensional $p+ip$ superfluids. This is accomplished by mapping the presence or absence of a Cooper pair into an effective spin-1/2 system encoded in the ions' electronic levels. We show how to infer the topological properties of the dynamical phases, and discuss the role of beyond mean-field corrections. More broadly, our work opens the door to use trapped ion systems to explore exotic models of topological superconductivity and also paves the way to generate and manipulate skyrmionic spin textures in these platforms.

Trapped ions boast long coherence times and excellent gate fidelities, making them a useful platform for quantum information processing. Scaling to larger numbers of ion qubits in RF Paul traps demands great effort. Another technique for trapping ions is via a Penning trap where a 2D crystal of hundreds of ions is formed by controlling the rotation of the ions in the presence of a strong magnetic field. However, the rotation of the ion crystal makes single ion addressability a significant challenge. We propose a protocol that takes advantage of a deformable mirror to introduce AC Stark shift patterns that are static in the rotating frame of the crystal. Through numerical simulations we validate the potential of this protocol to perform high-fidelity single-ion gates in crystalline arrays of hundreds of ions.

We propose protocols for the creation of useful entangled states in a system of spins collectively coupled to a bosonic mode, directly applicable to trapped-ion and cavity QED setups. The protocols use coherent manipulations of the spin-boson interactions naturally arising in these systems to prepare spin squeezed states exponentially fast in time. We demonstrate the robustness of the protocols by analyzing the effects of natural sources of decoherence in these systems and show their advantage compared to more standard slower approaches where entanglement is generated algebraically with time.

Planar thermal equilibration is studied using direct numerical simulations of ultracold two-dimensional (2D) ion crystals in a Penning trap with a rotating wall. The large magnetic field of the trap splits the modes that describe in-plane motion of the ions into two branches: High frequency cyclotron modes dominated by kinetic energy and low frequency $\mathbf{E \times B}$ modes dominated by potential energy associated with thermal position displacements. Using an eigenmode analysis we extract the equilibration rate between these two branches as a function of the ratio of the frequencies that characterize the two branches and observe this equilibration rate to be exponentially suppressed as the ratio increases. Under experimental conditions relevant for current work at NIST, the predicted equilibration time is orders of magnitude longer than any relevant experimental timescales. We also study the coupling rate dependence on the thermal temperature and the number of ions. Besides, we show how increasing the rotating wall strength improves crystal stability. These details of in-plane mode dynamics help set the stage for developing strategies to efficiently cool the in-plane modes and improve the performance of single-plane ion crystals for quantum information processing.

Developing the isolation and control of ultracold atomic systems to the level of single quanta has led to significant advances in quantum sensing, yet demonstrating a quantum advantage in real world applications by harnessing entanglement remains a core task. Here, we realize a many-body quantum-enhanced sensor to detect weak displacements and electric fields using a large crystal of $\sim 150$ trapped ions. The center of mass vibrational mode of the crystal serves as high-Q mechanical oscillator and the collective electronic spin as the measurement device. By entangling the oscillator and the collective spin before the displacement is applied and by controlling the coherent dynamics via a many-body echo we are able to utilize the delicate spin-motion entanglement to map the displacement into a spin rotation such that we avoid quantum back-action and cancel detrimental thermal noise. We report quantum enhanced sensitivity to displacements of $8.8 \pm 0.4~$dB below the standard quantum limit and a sensitivity for measuring electric fields of $240\pm10~\mathrm{nV}\mathrm{m}^{-1}$ in $1$ second ($240~\mathrm{nV}\mathrm{m}^{-1}/\sqrt{\mathrm{Hz}}$).

Two-dimensional crystals of ions stored in Penning traps are a leading platform for quantum simulation and sensing experiments. For small amplitudes, the out-of-plane motion of such crystals can be described by a discrete set of normal modes called the drumhead modes, which can be used to implement a range of quantum information protocols. However, experimental observations of crystals with Doppler-cooled and even near-ground-state-cooled drumhead modes reveal an unresolved drumhead mode spectrum. In this work, we establish in-plane thermal fluctuations in ion positions as a major contributor to the broadening of the drumhead mode spectrum. In the process, we demonstrate how the confining magnetic field leads to unconventional in-plane normal modes, whose average potential and kinetic energies are not equal. This property, in turn, has implications for the sampling procedure required to choose the in-plane initial conditions for molecular dynamics simulations. For current operating conditions of the NIST Penning trap, our study suggests that the two dimensional crystals produced in this trap undergo in-plane potential energy fluctuations of the order of $10$ mK. Our study therefore motivates the need for designing improved techniques to cool the in-plane degrees of freedom.

In trapped-ion quantum information processing, interactions between spins (qubits) are mediated by collective modes of motion of an ion crystal. While there are many different experimental strategies to design such interactions, they all face both technical and fundamental limitations to the achievable coherent interaction strength. In general, obtaining strong interactions and fast gates is an ongoing challenge. Here, we extend previous work [Phys. Rev. Lett. 112, 030501 (2019)] and present a general strategy for enhancing the interaction strengths in trapped-ion systems via parametric amplification of the ions' motion. Specifically, we propose a stroboscopic protocol using alternating applications of parametric amplification and spin-motion coupling. In comparison with the previous work, we show that the current protocol can lead to larger enhancements in the coherent interaction that increase exponentially with the gate time.

A direct numerical simulation of many interacting ions in a Penning trap with a rotating wall is presented. The ion dynamics is modelled classically. Both axial and planar Doppler laser cooling are modeled using stochastic momentum impulses based on two-level atomic scattering rates. The plasmas being modeled are ultra-cold two-dimensional crystals made up of 100's of ions. We compare Doppler cooled results directly to a previous linear eigenmodes analysis. Agreement in both frequency and mode structure are obtained. Additionally, when Doppler laser cooling is applied, the laser cooled steady state plasma axial temperature agrees with the Doppler cooling limit. Numerical simulations using the approach described and benchmarked here will provide insights into the dynamics of large trapped-ion crystals, improving their performance as a platform for quantum simulation and sensing.

We study, both experimentally and theoretically, electromagnetically induced transparency cooling of the drumhead modes of planar 2-dimensional arrays with up to $N\approx 190$ Be${}^+$ ions stored in a Penning trap. Substantial sub-Doppler cooling is observed for all $N$ drumhead modes. Quantitative measurements for the center-of-mass mode show near ground state cooling with motional quantum numbers of $\bar{n} = 0.3\pm0.2$ obtained within $200~μs$. The measured cooling rate is faster than that predicted by single particle theory, consistent with a quantum many-body calculation. For the lower frequency drumhead modes, quantitative temperature measurements are limited by apparent damping and frequency instabilities, but near ground state cooling of the full bandwidth is strongly suggested. This advancement will greatly improve the performance of large trapped ion crystals in quantum information and quantum metrology applications.

Penning traps, with their ability to control planar crystals of tens to hundreds of ions, are versatile quantum simulators. Thermal occupations of the motional drumhead modes, transverse to the plane of the ion crystal, degrade the quality of quantum simulations. Laser cooling using electromagnetically induced transparency (EIT cooling) is attractive as an efficient way to quickly initialize the drumhead modes to near ground-state occupations. We numerically investigate the efficiency of EIT cooling of planar ion crystals in a Penning trap, accounting for complications arising from the nature of the trap and from the simultaneous cooling of multiple ions. We show that, in spite of challenges, the large bandwidth of drumhead modes (hundreds of kilohertz) can be rapidly cooled to near ground-state occupations within a few hundred microseconds. Our predictions for the center-of-mass mode include a cooling time constant of tens of microseconds and an enhancement of the cooling rate with increasing number of ions. Successful experimental demonstrations of EIT cooling in the NIST Penning trap [E. Jordan, K. A. Gilmore, A. Shankar, A. Safavi-Naini, M. J. Holland, and J. J. Bollinger, "Near ground-state cooling of two-dimensional trapped-ion crystals with more than 100 ions", (2018), submitted.] validate our predictions.

Ultranarrow-linewidth atoms coupled to a lossy optical cavity mode synchronize, i.e. develop correlations, and exhibit steady-state superradiance when continuously repumped. This type of system displays rich collective physics and promises metrological applications. These features inspire us to investigate if analogous spin synchronization is possible in a different platform that is one of the most robust and controllable experimental testbeds currently available: ion-trap systems. We design a system with a primary and secondary species of ions that share a common set of normal modes of vibration. In analogy to the lossy optical mode, we propose to use a lossy normal mode, obtained by sympathetic cooling with the secondary species of ions, to mediate spin synchronization in the primary species of ions. Our numerical study shows that spin-spin correlations develop, leading to a macroscopic collective spin in steady-state. We propose an experimental method based on Ramsey interferometry to detect signatures of this collective spin; we predict that correlations prolong the visibility of Ramsey fringes, and that population statistics at the end of the Ramsey sequence can be used to directly infer spin-spin correlations.

Controllable arrays of ions and ultra-cold atoms can simulate complex many-body phenomena and may provide insights into unsolved problems in modern science. To this end, experimentally feasible protocols for quantifying the buildup of quantum correlations and coherence are needed, as performing full state tomography does not scale favorably with the number of particles. Here we develop and experimentally demonstrate such a protocol, which uses time reversal of the many-body dynamics to measure out-of-time-order correlation functions (OTOCs) in a long-range Ising spin quantum simulator with more than 100 ions in a Penning trap. By measuring a family of OTOCs as a function of a tunable parameter we obtain fine-grained information about the state of the system encoded in the multiple quantum coherence spectrum, extract the quantum state purity, and demonstrate the buildup of up to 8-body correlations. Future applications of this protocol could enable studies of many-body localization, quantum phase transitions, and tests of the holographic duality between quantum and gravitational systems.

We investigate the impact of a rotating wall potential on perpendicular laser cooling in a Penning ion trap. By including energy exchange with the rotating wall, we extend previous Doppler laser cooling theory and show that low perpendicular temperatures are more readily achieved with a rotating wall than without. Detailed numerical studies determine optimal operating parameters for producing low temperature, stable 2-dimensional crystals, important for quantum information processing experiments employing Penning traps.

Quantum simulation of spin models can provide insight into complex problems that are difficult or impossible to study with classical computers. Trapped ions are an established platform for quantum simulation, but only systems with fewer than 20 ions have demonstrated quantum correlations. Here we study non-equilibrium, quantum spin dynamics arising from an engineered, homogeneous Ising interaction in a two-dimensional array of $^9$Be$^+$ ions in a Penning trap. We verify entanglement in the form of spin-squeezed states for up to 219 ions, directly observing 4.0$\pm$0.9 dB of spectroscopic enhancement. We also observe evidence of non-Gaussian, over-squeezed states in the full counting statistics. We find good agreement with ab-initio theory that includes competition between entanglement and decoherence, laying the groundwork for simulations of the transverse-field Ising model with variable-range interactions, for which numerical solutions are, in general, classically intractable.

We demonstrate photodissociation of BeH$^+$ ions within a Coulomb crystal of thousands of $^9$Be$^+$ ions confined in a Penning trap. Because BeH$^+$ ions are created via exothermic reactions between trapped, laser-cooled Be$^+$($^2\text{P}_{3/2}$) and background H$_2$ within the vacuum chamber, they represent a major contaminant species responsible for infidelities in large-scale trapped-ion quantum information experiments. The rotational-state-insensitive dissociation scheme described here makes use of 157 nm photons to produce Be$^+$ and H as products, thereby restoring Be$^+$ ions without the need for reloading. This technique facilitates longer experiment runtimes at a given background H$_2$ pressure, and may be adapted for removal of MgH$^+$ and AlH$^+$ impurities.

We employ spin-dependent optical dipole forces to characterize the transverse center-of-mass (COM) motional mode of a two-dimensional Wigner crystal of hundreds of $^9$Be$^+$. By comparing the measured spin dephasing produced by the spin-dependent force with the predictions of a semiclassical dephasing model, we obtain absolute mode temperatures in excellent agreement with both the Doppler laser cooling limit and measurements obtained from a previously published technique (B. C. Sawyer et al. Phys. Rev. Lett. \textbf{108}, 213003 (2012)). Furthermore, the structure of the dephasing histograms allows for discrimination between initial thermal and coherent states of motion. We also apply the techniques discussed here to measure, for the first time, the ambient heating rate of the COM mode of a 2D Coulomb crystal in a Penning trap. This measurement places an upper limit on the anomalous single-ion heating rate due to electric field noise from the trap electrode surfaces of $\frac{d\bar{n}}{dt}\sim 5$ s$^{-1}$ for our trap at a frequency of 795 kHz, where $\bar{n}$ is the mean occupation of quantized COM motion in the axial harmonic well.

Ising models, and the physical systems described by them, play a central role in generating entangled states for use in quantum metrology and quantum information. In particular, ultracold atomic gases, trapped ion systems, and Rydberg atoms realize long-ranged Ising models, which even in the absence of a transverse field can give rise to highly non-classical dynamics and long-range quantum correlations. In the first part of this paper, we present a detailed theoretical framework for studying the dynamics of such systems driven (at time t=0) into arbitrary unentangled non-equilibrium states, thus greatly extending and unifying the work of Ref. [1]. Specifically, we derive exact expressions for closed-time-path ordered correlation functions, and use these to study experimentally relevant observables, e.g. Bloch vector and spin-squeezing dynamics. In the second part, these correlation functions are then used to derive closed-form expressions for the dynamics of arbitrary spin-spin correlation functions in the presence of both T_1 (spontaneous spin relaxation/excitation) and T_2 (dephasing) type decoherence processes. Even though the decoherence is local, our solution reveals that the competition between Ising dynamics and T_1 decoherence gives rise to an emergent non-local dephasing effect, thereby drastically amplifying the degradation of quantum correlations. In addition to identifying the mechanism of this deleterious effect, our solution points toward a scheme to eliminate it via measurement-based coherent feedback.

By employing forces that depend on the internal electronic state (or spin) of an atomic ion, the Coulomb potential energy of a strongly coupled array of ions can be modified in a spin-dependent way to mimic effective quantum spin Hamiltonians. Both ferromagnetic and antiferromagnetic interactions can be implemented. We use simple models to explain how the effective spin interactions are engineered with trapped-ion crystals. We summarize the type of effective spin interactions that can be readily generated, and discuss an experimental implementation using single-plane ion crystals in a Penning trap.

We study the time evolution of correlation functions in long-range interacting quantum Ising models. For a large class of initial conditions, exact analytic results are obtained in arbitrary lattice dimension, both for ferromagnetic and antiferromagnetic coupling, and hence also in the presence of geometric frustration. In contrast to the nearest-neighbour case, we find that correlations decay like stretched or compressed exponentials in time. Provided the long-range character of the interactions is sufficiently strong, pronounced prethermalization plateaus are observed and relaxation timescales are widely separated. Specializing to a triangular lattice in two spatial dimensions, we propose to utilize these results for benchmarking of a recently developed ion-trap based quantum simulator.

The presence of long-range quantum spin correlations underlies a variety of physical phenomena in condensed matter systems, potentially including high-temperature superconductivity. However, many properties of exotic strongly correlated spin systems (e.g., spin liquids) have proved difficult to study, in part because calculations involving N-body entanglement become intractable for as few as N~30 particles. Feynman divined that a quantum simulator - a special-purpose "analog" processor built using quantum particles (qubits) - would be inherently adept at such problems. In the context of quantum magnetism, a number of experiments have demonstrated the feasibility of this approach. However, simulations of quantum magnetism allowing controlled, tunable interactions between spins localized on 2D and 3D lattices of more than a few 10's of qubits have yet to be demonstrated, owing in part to the technical challenge of realizing large-scale qubit arrays. Here we demonstrate a variable-range Ising-type spin-spin interaction J_ij on a naturally occurring 2D triangular crystal lattice of hundreds of spin-1/2 particles (9Be+ ions stored in a Penning trap), a computationally relevant scale more than an order of magnitude larger than existing experiments. We show that a spin-dependent optical dipole force can produce an antiferromagnetic interaction J_ij ~ 1/d_ij^a, where a is tunable over 0<a<3; d_ij is the distance between spin pairs. These power-laws correspond physically to infinite-range (a=0), Coulomb-like (a=1), monopole-dipole (a=2) and dipole-dipole (a=3) couplings. Experimentally, we demonstrate excellent agreement with theory for 0.05<a<1.4. This demonstration coupled with the high spin-count, excellent quantum control and low technical complexity of the Penning trap brings within reach simulation of interesting and otherwise computationally intractable problems in quantum magnetism.

We demonstrate spectroscopy and thermometry of individual motional modes in a mesoscopic 2D ion array using entanglement-induced decoherence as a method of transduction. Our system is a $\sim$400 $μ$m-diameter planar crystal of several hundred $^9$Be$^+$ ions exhibiting complex drumhead modes in the confining potential of a Penning trap. Exploiting precise control over the $^9$Be$^+$ valence electron spins, we apply a homogeneous spin-dependent optical dipole force to excite arbitrary transverse modes with an effective wavelength approaching the interparticle spacing ($\sim$20 \nolinebreak$μ$m). Center-of-mass displacements below 1 nm are detected via entanglement of spin and motional degrees of freedom.

Building robust instruments capable of making interferometric measurements with precision beyond the standard quantum limit remains an important goal in many metrology laboratories. We describe here the basic concepts underlying spin squeezing experiments that allow one to surpass this limit. In priniciple it is possible to reach the so-called Heisenberg limit, which constitutes an improvement in precision by a factor $\sqrt{N}$, where $N$ is the number of particles on which the measurement is carried out. In particular, we focus on recent progress toward implementing spin squeezing with a cloud of beryllium ions in a Penning ion trap, via the geometric phase gate used more commonly for performing two-qubit entangling operations in quantum computing experiments.

We discuss the use of two-dimensional $^{9}$Be$^{+}$ ion crystals for experimental tests of quantum control techniques. Our primary qubit is the 124 GHz ground-state electron spin flip transition, which we drive using microwaves. An ion crystal represents a spatial ensemble of qubits, but the effects of inhomogeneities across a typical crystal are small, and as such we treat the ensemble as a single effective spin. We are able to initialize the qubits in a simple state and perform a projective measurement on the system. We demonstrate full control of the qubit Bloch vector, performing arbitrary high-fidelity rotations ($τ_π\sim$200 $μ$s). Randomized Benchmarking demonstrates an error per gate (a Pauli-randomized $π/2$ and $π$ pulse pair) of $8\pm1\times10^{-4}$. Ramsey interferometry and spin-locking measurements are used to elucidate the limits of qubit coherence in the system, yielding a typical free-induction decay coherence time of $T_{2}\sim$2 ms, and a limiting $T_{1ρ}\sim$688 ms. These experimental specifications make ion crystals in a Penning trap ideal candidates for novel experiments in quantum control. As such, we briefly describe recent efforts aimed at studying the error-suppressing capabilities of dynamical decoupling pulse sequences, demonstrating an ability to extend qubit coherence and suppress phase errors. We conclude with a discussion of future avenues for experimental exploration, including the use of additional nuclear-spin-flip transitions for effective multiqubit protocols, and the potential for Coulomb crystals to form a useful testbed for studies of large-scale entanglement.

One approach to maintaining phase coherence of qubits through dynamical decoupling consists of applying a sequence of Hahn spin-echo pulses. Recent studies have shown that, in certain noise environments, judicious choice of the delay times between these pulses can greatly improve the suppression of phase errors compared to traditional approaches. By enforcing a simple analytical condition, we obtain sets of dynamical decoupling sequences that are designed for optimized noise filtration and are spectrum-independent up to a single scaling factor set by the coherence time of the system. We demonstrate the efficacy of these sequences in suppressing phase errors through measurements on a model qubit system, $^{9}$Be$^{+}$ ions in a Penning trap. Our combined theoretical and experimental studies show that in high-frequency-dominated noise environments this approach may suppress phase errors orders of magnitude more efficiently than comparable techniques can.

We present a detailed experimental study of the Uhrig Dynamical Decoupling (UDD) sequence in a variety of noise environments. Our qubit system consists of a crystalline array of $^{9}$Be$^{+}$ ions confined in a Penning trap. We use an electron-spin-flip transition as our qubit manifold and drive qubit rotations using a 124 GHz microwave system. We study the effect of the UDD sequence in mitigating phase errors and compare against the well known CPMG-style multipulse spin echo as a function of pulse number, rotation axis, noise spectrum, and noise strength. Our results agree well with theoretical predictions for qubit decoherence in the presence of classical phase noise, accounting for the effect of finite-duration $π$ pulses. Finally, we demonstrate that the Uhrig sequence is more robust against systematic over/underrotation and detuning errors than is multipulse spin echo, despite the precise prescription for pulse-timing in UDD.