Philipp Müller

We present the implementation of a programmable atom-photon quantum interface, employing a single trapped $^{40}$Ca$^+$ ion and single photons. Depending on its mode of operation, the interface serves as a bi-directional atom-photon quantum-state converter, as a source of entangled atom-photon states, or as a quantum frequency converter of single photons. The interface lends itself particularly to interfacing ions with single or entangled photons in hybrid quantum networks.

We report on a single-photon-to-single-atom interface, where a single photon generated by Spontaneous Parametric Down Conversion (SPDC) is absorbed by a single trapped ion. The photon is heralded by its time-correlated partner generated in the SPDC process, while the absorption event is heralded by a single photon emitted in its course. Coincidence detection marks doubly-heralded absorption, enabling photon-to-atom quantum state transfer [1, 2]. Background in the coincidence measurement is strongly suppressed by a new method that discriminates real absorption events from dark count-induced coincidences.

We present, characterize, and apply a photonic quantum interface between the near infrared and telecom spectral regions. A singly resonant optical parametric oscillator (OPO) operated below threshold, in combination with external filters, generates high-rate ($>2.5\cdot10^6~{\rm s}^{-1}$) narrowband photon pairs ($\sim 7$ MHz bandwidth); the signal photons are tuned to resonance with an atomic transition in Ca$^+$, while the idler photons are at telecom wavelength. Quantum interface operation is demonstrated through high-rate absorption of single photons by a single trapped ion ($\sim 670~{\rm s}^{-1}$), heralded by coincident telecom photons.

We investigate quantum beats in the arrival-time distribution of single photons from a single trapped $^{40}$Ca$^+$ ion, revealing their fundamentally different physical origins in two distinct experimental situations: In a $Λ$-type level scheme the interference of two 854-nm absorption amplitudes suppresses and enhances the emission process of Raman-scattered 393-nm photons; in a V-type level scheme the interference of two 393-nm emission amplitudes causes a rotation of their dipole emission pattern resulting in a temporal modulation of the detected photons. For both cases we demonstrate coherent control over the quantum-beat phase through the phases of the atomic and photonic input states, which also allows controlled adjustment of the total photon detection efficiency.

We establish heralded interaction between two remotely trapped single 40Ca+ ions through the exchange of single photons. In the sender ion, we release single photons with controlled temporal shape on the P_3/2 to D_5/2 transition and transmit them to the distant receiver ion. Individual absorption events in the receiver ion are detected by quantum jumps. For continuously generated photons, the absorption reduces significantly the lifetime of the long-lived D_5/2 state. For triggered single-photon transmission, we observe coincidence between the emission at the sender and quantum jump events at the receiver.

We report on the efficient generation of single photons, making use of spontaneous Raman scattering in a single trapped ion. The photons are collected through in-vacuum high-NA objectives. Photon frequency, polarization and temporal shape are controlled through appropriate laser parameters, allowing for photons in a pure quantum state.