Daniel H. Slichter

Controlled quantum mechanical motion of trapped atomic ions can be used to simulate and explore collective quantum phenomena and to process quantum information. Groups of cold atomic ions in an externally applied trapping potential self-organize into "Coulomb crystals" due to their mutual electrostatic repulsion. The motion of the ions in these crystals is strongly coupled, and the eigenmodes of motion all involve multiple ions. While this enables studies of many-body physics, it limits the flexibility and tunability of the system as a quantum platform. Here, we demonstrate an array of trapped ions in individual trapping sites whose motional modes can be controllably coupled and decoupled by tuning the local applied confining potential for each ion. We show that a single motional quantum, or phonon, can be coherently shared among two or three ions confined at the vertices of an equilateral triangle 30 $μ$m on a side. We can adiabatically tune the ion participation in the motional modes around a closed contour in configuration space, observing that the single-phonon wavefunction acquires a topological Berry phase if the contour encircles a conical intersection of motional eigenvalue surfaces. We observe this phase by single-phonon interference and study its breakdown as the motional mode tuning becomes non-adiabiatic. Our results show that precise, individual quantum control of ion motion in a two-dimensional array can provide unique access to quantum multi-body effects.

Rapid separation of linear crystals of trapped ions into different subsets is critical for realizing trapped ion quantum computing architectures where ions are rearranged in trap arrays to achieve all-to-all connectivity between qubits. We introduce a general theoretical framework that can be used to describe the separation of same-species and mixed-species crystals into smaller subsets. The framework relies on an efficient description of the evolution of Gaussian motional states under quadratic Hamiltonians that only requires a special solution of the classical equations of motion of the ions to describe their quantum evolution under the influence of a time-dependent applied potential and the ions' mutual Coulomb repulsion. We provide time-dependent applied potentials suitable for separation of a mixed species three-ion crystal on timescales similar to that of free expansion driven by Coulomb repulsion, with all modes along the crystal axis starting and ending close to their ground states. Three separately-confined mixed species ions can be combined into a crystal held in a single well without energy gain by time-reversal of this separation process.

Excess "micromotion" of trapped ions due to the residual radio-frequency (rf) trapping field at their location is often undesirable and is usually carefully minimized. Here, we induce precise amounts of excess micromotion on individual ions by adjusting the local static electric field they experience. Micromotion modulates the coupling of an ion to laser fields, ideally tuning it from its maximum value to zero as the ion is moved away from the trap's rf null. We use tunable micromotion to vary the Rabi frequency of stimulated Raman transitions over two orders of magnitude, and to individually control the rates of resonant fluorescence from three ions under global laser illumination without any changes to the driving light fields. The technique is amenable to situations where addressing individual ions with focused laser beams is challenging, such as tightly packed linear ion strings or two-dimensional ion arrays illuminated from the side.

Randomized benchmarking (RB) is a widely used strategy to assess the quality of available quantum gates in a computational context. RB involves applying known random sequences of gates to an initial state and using the statistics of a final measurement step to determine an effective depolarizing error per step of the sequence, which is a metric of gate quality. Here we investigate the advantages of fully randomized benchmarking, where a new random sequence is drawn for each experimental trial. The advantages of full randomization include smaller confidence intervals on the inferred step error, the ability to use maximum likelihood analysis without heuristics, straightforward optimization of the sequence lengths, and the ability to model and measure behaviors that go beyond the typical assumption of time-independent error rates. We discuss models of time-dependent or non-Markovian errors that generalize the basic RB model of a single exponential decay of the success probability. For any of these models, we implement a concrete protocol to minimize the uncertainty of the estimated parameters given a fixed time constraint on the complete experiment, and we implement a maximum likelihood analysis. We consider several previously published experiments and determine the potential for improvements with optimized full randomization. We experimentally observe such improvements in Clifford randomized benchmarking experiments on a single trapped ion qubit at the National Institute of Standards and Technology (NIST). For an experiment with uniform lengths and intentionally repeated sequences the step error was $2.42^{+0.30}_{-0.22}\times 10^{-5}$, and for an optimized fully randomized experiment of the same total duration the step error was $2.57^{+0.07}_{-0.06}\times 10^{-5}$. We find a substantial decrease in the uncertainty of the step error as a result of optimized fully randomized benchmarking.

Cooling the motion of trapped ions to near the quantum ground state is crucial for many applications in quantum information processing and quantum metrology. However, certain motional modes of trapped-ion crystals can be difficult to cool due to weak or zero interaction between the modes and the cooling radiation, typically laser beams. We overcome this challenge by coupling a mode with weak cooling radiation interaction to one with strong cooling radiation interaction using parametric modulation of the trapping potential, thereby enabling indirect cooling of the former. In this way, we demonstrate near-ground-state cooling of motional modes with weak or zero cooling radiation interaction in multi-ion crystals of the same and mixed ion species, specifically $^9$Be$^+$-$^9$Be$^+$, $^9$Be$^+$-$^{25}$Mg$^+$, and $^9$Be$^+$-$^{25}$Mg$^+$-$^9$Be$^+$ crystals. This approach can be generally applied to any Coulomb crystal where certain motional modes cannot be directly cooled efficiently, including crystals containing molecular ions, highly-charged ions, charged fundamental particles, or charged macroscopic objects.

State readout of trapped-ion qubits with trap-integrated detectors can address important challenges for scalable quantum computing, but the strong rf electric fields used for trapping can impact detector performance. Here, we report on NbTiN superconducting nanowire single-photon detectors (SNSPDs) employing grounded aluminum mirrors as electrical shielding that are integrated into linear surface-electrode rf ion traps. The shielded SNSPDs can be successfully operated at applied rf trapping potentials of up to $\mathrm{54\,V_{peak}}$ at $\mathrm{70\,MHz}$ and temperatures of up to $\mathrm{6\,K}$, with a maximum system detection efficiency of $\mathrm{68\,\%}$. This performance should be sufficient to enable parallel high-fidelity state readout of a wide range of trapped ion species in typical cryogenic apparatus.

Precise quantum control and measurement of several harmonic oscillators, such as the modes of the electromagnetic field in a cavity or of mechanical motion, are key for their use as quantum platforms. The motional modes of trapped ions can be individually controlled and have good coherence properties. However, achieving high-fidelity two-mode operations and nondestructive measurements of the motional state has been challenging. Here we demonstrate the coherent exchange of single motional quanta between spectrally separated harmonic motional modes of a trapped-ion crystal. The timing, strength, and phase of the coupling are controlled through an oscillating electric potential with suitable spatial variation. Coupling rates that are much larger than decoherence rates enable demonstrations of high fidelity quantum state transfer and beamsplitter operations, entanglement of motional modes, and Hong-Ou-Mandel-type interference. Additionally, we use the motional coupling to enable repeated non-destructive projective measurement of a trapped-ion motional state. Our work enhances the suitability of trapped-ion motion for continuous-variable quantum computing and error correction and may provide opportunities to improve the performance of motional cooling and motion-mediated entangling interactions.

We propose and demonstrate a protocol for high-fidelity indirect readout of trapped ion hyperfine qubits, where the state of a $^9\text{Be}^+$ qubit ion is mapped to a $^{25}\text{Mg}^+$ readout ion using laser-driven Raman transitions. By partitioning the $^9\text{Be}^+$ ground state hyperfine manifold into two subspaces representing the two qubit states and choosing appropriate laser parameters, the protocol can be made robust to spontaneous photon scattering errors on the Raman transitions, enabling repetition for increased readout fidelity. We demonstrate combined readout and back-action errors for the two subspaces of $1.2^{+1.1}_{-0.6} \times 10^{-4}$ and $0^{+1.9}_{-0} \times 10^{-5}$ with 68% confidence while avoiding decoherence of spectator qubits due to stray resonant light that is inherent to direct fluorescence detection.

We demonstrate a simplified method for dissipative generation of an entangled state of two trapped-ion qubits. Our implementation produces its target state faster and with higher fidelity than previous demonstrations of dissipative entanglement generation and eliminates the need for auxiliary ions. The entangled singlet state is generated in $\sim$7 ms with a fidelity of 0.949(4). The dominant source of infidelity is photon scattering. We discuss this error source and strategies for its mitigation.

We demonstrate the use of a single trapped ion as a sensor to probe electric-field noise from interchangeable test surfaces. As proof of principle, we measure the magnitude and distance dependence of electric-field noise from two ion-trap-like samples with patterned Au electrodes. This trapped-ion sensor could be combined with other surface characterization tools to help elucidate the mechanisms that give rise to electric-field noise from ion-trap surfaces. Such noise presents a significant hurdle for performing large-scale trapped-ion quantum computations.

Quantum information processing systems rely on a broad range of microwave technologies and have spurred development of microwave devices and methods in new operating regimes. Here we review the use of microwave signals and systems in quantum computing, with specific reference to three leading quantum computing platforms: trapped atomic ion qubits, spin qubits in semiconductors, and superconducting qubits. We highlight some key results and progress in quantum computing achieved through the use of microwave systems, and discuss how quantum computing applications have pushed the frontiers of microwave technology in some areas. We also describe open microwave engineering challenges for the construction of large-scale, fault-tolerant quantum computers.

Experiments in atomic, molecular, and optical (AMO) physics rely on lasers at many different wavelengths and with varying requirements on spectral linewidth, power, and intensity stability. Vertical external-cavity surface-emitting lasers (VECSELs), when combined with nonlinear frequency conversion, can potentially replace many of the laser systems currently in use. Here we present and characterize VECSEL systems that can perform all laser-based tasks for quantum information processing experiments with trapped magnesium ions. For photoionization of neutral magnesium, 570.6$\,$nm light is generated with an intracavity frequency-doubled VECSEL containing a lithium triborate (LBO) crystal for second harmonic generation. External frequency doubling produces 285.3$\,$nm light for resonant interaction with the $^{1}S_{0}\leftrightarrow$ $^{1}P_{1}$ transition of neutral Mg. Using an externally frequency-quadrupled VECSEL, we implement Doppler cooling of $^{25}$Mg$^{+}$ on the 279.6$\,$nm $^{2}S_{1/2}\leftrightarrow$ $^{2}P_{3/2}$ cycling transition, repumping on the 280.4$\,$nm $^{2}S_{1/2}\leftrightarrow$ $^{2}P_{1/2}$ transition, coherent state manipulation, and resolved sideband cooling close to the motional ground state. Our systems serve as prototypes for applications in AMO requiring single-frequency, power-scalable laser sources at multiple wavelengths.