Roman Schmied

Controlled quantum mechanical motion of trapped atomic ions can be used to simulate and explore collective quantum phenomena and to process quantum information. Groups of cold atomic ions in an externally applied trapping potential self-organize into "Coulomb crystals" due to their mutual electrostatic repulsion. The motion of the ions in these crystals is strongly coupled, and the eigenmodes of motion all involve multiple ions. While this enables studies of many-body physics, it limits the flexibility and tunability of the system as a quantum platform. Here, we demonstrate an array of trapped ions in individual trapping sites whose motional modes can be controllably coupled and decoupled by tuning the local applied confining potential for each ion. We show that a single motional quantum, or phonon, can be coherently shared among two or three ions confined at the vertices of an equilateral triangle 30 $μ$m on a side. We can adiabatically tune the ion participation in the motional modes around a closed contour in configuration space, observing that the single-phonon wavefunction acquires a topological Berry phase if the contour encircles a conical intersection of motional eigenvalue surfaces. We observe this phase by single-phonon interference and study its breakdown as the motional mode tuning becomes non-adiabiatic. Our results show that precise, individual quantum control of ion motion in a two-dimensional array can provide unique access to quantum multi-body effects.

We discuss the design and optimisation of two types of junctions between surface-electrode radiofrequency ion-trap arrays that enable the integration of experiments with sympathetically cooled molecular ions on a monolithic chip device. A detailed description of a multi-objective optimisation procedure applicable to an arbitrary planar junction is presented, and the results for a cross junction between four quadrupoles as well as a quadrupole-to-octupole junction are discussed. Based on these optimised functional elements, we propose a multi-functional ion-trap chip for experiments with translationally cold molecular ions at temperatures in the millikelvin range. This study opens the door to extending complex chip-based trapping techniques to Coulomb-crystallised molecular ions with potential applications in mass spectrometry, spectroscopy, controlled chemistry and quantum technology.

Quantum technologies exploit entanglement to revolutionize computing, measurements, and communications. This has stimulated the research in different areas of physics to engineer and manipulate fragile many-particle entangled states. Progress has been particularly rapid for atoms. Thanks to the large and tunable nonlinearities and the well developed techniques for trapping, controlling and counting, many groundbreaking experiments have demonstrated the generation of entangled states of trapped ions, cold and ultracold gases of neutral atoms. Moreover, atoms can couple strongly to external forces and light fields, which makes them ideal for ultra-precise sensing and time keeping. All these factors call for generating non-classical atomic states designed for phase estimation in atomic clocks and atom interferometers, exploiting many-body entanglement to increase the sensitivity of precision measurements. The goal of this article is to review and illustrate the theory and the experiments with atomic ensembles that have demonstrated many-particle entanglement and quantum-enhanced metrology.

A custom-built and precisely controlled quantum system may offer access to a fundamental understanding of another, less accessible system of interest. A universal quantum computer is currently out of reach, but an analog quantum simulator that makes the relevant observables, interactions, and states of a quantum model accessible could permit experimental insight into complex quantum dynamics that are intractable on conventional computers. Several platforms have been suggested and proof-of-principle experiments have been conducted. Here we characterise two-dimensional arrays of three ions trapped by radio-frequency fields in individually controlled harmonic wells forming equilateral triangles with side lengths 40 and 80 micrometer. In our approach, which is scalable to arbitrary two dimensional lattices, we demonstrate individual control of the electronic and motional degrees of freedom, preparation of a fiducial initial state with ion motion close to the ground state, as well as tuning of crucial couplings between ions within experimental sequences. Our work paves the way towards an analog quantum simulator of two-dimensional systems designed at will.

We present a detailed study of quantum simulations of coupled spin systems in surface-electrode ion-trap arrays, and illustrate our findings with a proposed implementation of the hexagonal Kitaev model [A. Kitaev, Annals of Physics 321,2 (2006)]. The effective (pseudo)spin interactions making up such quantum simulators are found to be proportional to the dipole-dipole interaction between the trapped ions, and are mediated by motion which can be driven by state-dependent forces. The precise forms of the trapping potentials and the interactions are derived in the presence of a surface electrode and a cover electrode. These results are the starting point to derive an optimized surface-electrode geometry for trapping ions in the desired honeycomb lattice of Kitaev's model, where we design the dipole-dipole interactions in a way that allows for coupling all three bond types of the model simultaneously, without the need for time discretization. Finally we propose a simple wire structure that can be incorporated in a microfabricated chip to generate localized state-dependent forces which drive the couplings prescribed by this particular model; such a wire structure should be adaptable to many other situations.

We present approximate methods for calculating the three-dimensional electric potentials of finite surface electrodes including gaps between electrodes, and estimate the effects of finite electrode thickness and an underlying dielectric substrate. As an example we optimize a radio-frequency surface-electrode ring ion trap, and find that each of these factors reduces the trapping secular frequencies by less than 5% in realistic situations. This small magnitude validates the usual assumption of neglecting the influences of gaps between electrodes and finite electrode extent.

Trapped ions offer long internal state (spin) coherence times and strong inter-particle interactions mediated by the Coulomb force. This makes them interesting candidates for quantum simulation of coupled lattices. To this end it is desirable to be able to trap ions in arbitrary conformations with precisely controlled local potentials. We provide a general method for optimizing periodic planar radio-frequency electrodes for generating ion trapping potentials with specified trap locations and curvatures above the electrode plane. A linear-programming algorithm guarantees globally optimal electrode shapes that require only a single radio-frequency voltage source for operation. The optimization method produces final electrode shapes that are smooth and exhibit low fragmentation. Such characteristics are desirable for practical fabrication of surface-electrode trap lattices.

We propose loading trapped ions into microtraps formed by an optical lattice. For harmonic microtraps, the Coulomb coupling of the spatial motions of neighboring ions can be used to construct a broad class of effective short-range Hamiltonians acting on an internal degree of freedom of the ions. For large anharmonicities, on the other hand, the spatial motion of the ions itself represents a spin-1/2 model with frustrated dipolar XY interactions. We illustrate the latter setup with three systems: the linear chain, the zig-zag ladder, and the triangular lattice. In the frustrated zig-zag ladder with dipolar interactions we find chiral ordering beyond what was predicted previously for a next-nearest-neighbor model. In the frustrated anisotropic triangular lattice with nearest-neighbor interactions we find that the transition from the one-dimensional gapless spin-liquid phase to the two-dimensional spiraling ordered phase passes through a gapped spin-liquid phase, similar to what has been predicted for the same model with Heisenberg interactions. Further, a second gapped spin-liquid phase marks the transition to the two-dimensional Neel-ordered phase.