Tobias Schaetz

Understanding how strong coupling and memory effects influence the energy levels of open quantum systems is a complex and challenging problem. Here, we show these effects by probing the transition frequency of an open two-level system within the Jaynes-Cummings model, experimentally realised using Ramsey interferometry in a single trapped 25Mg+ ion. Measurements of the system, coupled to a single-mode environment, reveal a time-dependent shift in the system's energy levels of up to 15% of the bare system frequency. This shift, accurately predicted using an open system ansatz of minimal dissipation, results purely from ultra-strong system-mode interactions and the buildup of correlations. Time-averaged measurements converge to the dispersive Lamb shift predictions and match dressed-state energies, indicating that this observed shift represents a generalised Lamb shift applicable across all coupling and detuning regimes. Our findings provide direct evidence of dynamic energy level renormalisation in strongly coupled open quantum systems, although the total system-environment Hamiltonian is static; this underscores the significance of memory effects in shaping the reduced system's energy landscape. These results offer more profound insights into Hamiltonian renormalisation, essential for strong-coupling quantum thermodynamics and advancements in all quantum platforms.

In quantum technologies, it is essential to understand and exploit the interplay of light and matter. We introduce an approach, creating and maintaining the coherence of four oscillators: a global microwave reference field, a polarization-gradient traveling-wave pattern of light, and the spin and motional states of a single trapped ion. The features of our method are showcased by probing the 140-nm periodic light pattern and stroboscopically tracing dynamical variations in position and momentum observables with noise floors of $1.8(2)\,$nm and $8(2)~$zN$\,μ$s, respectively. The implications of our findings contribute to enhancing quantum control and metrological applications.

We report the optical trapping of multiple ions localized at individual lattice sites of a one-dimensional optical lattice. We observe a fivefold increase in robustness against axial DC-electric fields and an increase of the axial eigenfrequency by two orders of magnitude compared to an optical dipole trap without interference but similar intensity. Our findings motivate an alternative pathway to extend arrays of trapped ions in size and dimension, enabling quantum simulations with particles interacting at long range.

A variety of physical platforms are investigated for quantum control of many particles, and techniques are extended to access multiple dimensions. Here, we present our experimental study of shuttling single Mg$^+$ ions within a scalable trap-array architecture that contains up to thirteen trapping sites in a three-dimensional arrangement. We shuttle ions from a dedicated loading hub to multiple sites with a success rate of larger than $0.99999$. In a prototype application, we demonstrate the preservation of the coherence of superposition states of a hyperfine qubit during inter-site shuttling. Our findings highlight the potential of these techniques for use in future large-scale architectures.

Controlling physical systems and their dynamics on the level of individual quanta propels both fundamental science and quantum technologies. Trapped atomic and molecular systems, neutral and charged, are at the forefront of quantum science. Their extraordinary level of control is evidenced by numerous applications in quantum information processing and quantum metrology. Studying the long-range interactions between these systems when combined in a hybrid atom-ion trap has lead to landmark results. Reaching the ultracold regime, however, where quantum mechanics dominates the interaction, e.g., giving access to controllable scattering resonances, has been elusive so far. Here we demonstrate Feshbach resonances between ions and atoms, using magnetically tunable interactions between $^{138}$Ba$^{+}$ ions and $^{6}$Li atoms. We tune the experimental parameters to probe different interaction processes - first, enhancing three-body reactions and the related losses to identify the resonances, then making two-body interactions dominant to investigate the ion's sympathetic cooling in the ultracold atomic bath. Our results provide deeper insights into atom-ion interactions, giving access to complex many-body systems and applications in experimental quantum simulation.

Isolating neutral and charged particles from the environment is essential in precision experiments. For decades, this has been achieved by trapping ions with radio-frequency (rf) fields and neutral particles with optical fields. Recently, trapping of ions by interaction with light has been demonstrated. This might permit combining the advantages of optical trapping and ions. For example, by superimposing optical traps to investigate ensembles of ions and atoms in absence of any radiofrequency fields, as well as to benefit from the versatile and scalable trapping geometries featured by optical lattices. In particular, ions provide individual addressability, electronic and motional degrees of freedom that can be coherently controlled and detected via high fidelity, state-dependent operations. Their long-range Coulomb interaction is significantly larger compared to those of neutral atoms and molecules. This qualifies to study ultra-cold interaction and chemistry of trapped ions and atoms, as well as to provide a novel platform for higher-dimensional experimental quantum simulations. The aim of this topical review is to present the current state of the art and to discuss current challenges and the prospects of the emerging field.

For conventional ion traps, the trapping potential is close to independent of the electronic state, providing confinement for ions dependent primarily on their charge-to-mass ratio $Q/m$. In contrast, storing ions within an optical dipole trap results in state-dependent confinement. Here we experimentally study optical dipole potentials for $^{138}\mathrm{Ba}^+$ ions stored within two distinctive traps operating at 532 nm and 1064 nm. We prepare the ions in either the $6\mathrm{S}_{\mathrm{1/2}}$ electronic ground or the $5\mathrm{D}_{\mathrm{3/2}}$/ $5\mathrm{D}_{\mathrm{5/2}}$ metastable excited state and probe the relative strength and polarity of the potential. On the one hand, we apply our findings to selectively remove ions from a Coulomb crystal, despite all ions sharing the same $Q/m$. On the other hand, we deterministically purify the trapping volume from parasitic ions in higher-energy orbits, resulting in reliable isolation of Coulomb crystals down to a single ion within a radio-frequency trap.

We study a method for mass-selective removal of ions from a Paul trap by parametric excitation. This can be achieved by applying an oscillating electric quadrupole field at twice the secular frequency $ω_{\text{sec}}$ using pairs of opposing electrodes. While excitation near the resonance with the frequency $ω_{\text{sec}}$ only leads to a linear increase of the amplitude with excitation duration, parametric excitation near $2\, ω_{\text{sec}}$ results in an exponential increase of the amplitude. This enables efficient removal of ions from the trap with modest excitation voltages and narrow bandwidth, therefore substantially reducing the disturbance of ions with other charge-to-mass ratios. We numerically study and compare the mass selectivity of the two methods. In addition, we experimentally show that the barium isotopes with 136 and 137 nucleons can be removed from small ion crystals and ejected out of the trap while keeping $^{138}\text{Ba}^{+}$ ions Doppler cooled, corresponding to a mass selectivity of better than $Δm / m = 1/138$. This method can be widely applied to ion trapping experiments without major modifications, since it only requires modulating the potential of the ion trap.

A comprehensive description of molecular electron transfer reactions is essential for our understanding of fundamental phenomena in bio-energetics and molecular electronics. Experimental studies of molecular systems in condensed-phase environments, however, face difficulties to independently control the parameters that govern the transfer mechanism with high precision. We show that trapped-ion experiments instead allow to reproduce and continuously connect vastly different regimes of molecular charge transfer through precise tuning of, e.g., phonon temperature, electron-phonon interactions, and electronic couplings. Such a setting allows not only to reproduce widely-used transport models, such as Marcus theory. It also provides access to transfer regimes that are unattainable for molecular experiments, while controlling and measuring the relevant observables on the level of individual quanta. Our numerical simulations predict an unconventional quantum transfer regime, featuring a transition from quantum adiabatic- to resonance-assisted transfer as a function of the donor-acceptor energy gap, that can be reached by increasing the electronic coupling at low temperatures. Trapped ion-based quantum simulations thus promise to enhance our microscopic understanding of molecular electron transfer processes, and may help to reveal efficient design principles for synthetic devices.

We demonstrate Floquet engineering in a basic yet scalable 2D architecture of individually trapped and controlled ions. Local parametric modulations of detuned trapping potentials steer the strength of long-range inter-ion couplings and the related Peierls phase of the motional state. In our proof-of-principle, we initialize large coherent states and tune modulation parameters to control trajectories, directions and interferences of the phonon flow. Our findings open a new pathway for future Floquet-based trapped-ion quantum simulators targeting correlated topological phenomena and dynamical gauge fields.

The creation of matter and structure in our universe is currently described by an intricate interplay of quantum field theory and general relativity. Signatures of this process during an early inflationary period can be observed, while direct tests remain out of reach. Here, we study an experimental analog of the process based on trapped atomic ions. We create pairs of phonons by tearing apart quantum vacuum fluctuations. Thereby, we prepare ions in an entangled state of motion. Controlling timescales and the coupling to environments should permit optimizing efficiencies while keeping the effect robust via established tools in quantum information processing (QIP). This might also permit to cross-fertilize between concepts in cosmology and applications of QIP, such as, quantum metrology, experimental quantum simulations and quantum computing.

Quantum mechanics dominates various effects in modern research from miniaturizing electronics, up to potentially ruling solid-state physics, quantum chemistry and biology. To study these effects experimental quantum systems may provide the only effective access. Seminal progress has been achieved in a variety of physical platforms, highlighted by recent applications. Atomic ions are known for their unique controllability and are identical by nature, as evidenced, e.g., by performing among the most precise atomic clocks and providing the basis for one-dimensional simulators. However, controllable, scalable systems of more than one dimension are required to address problems of interest and to reach beyond classical numerics with its powerful approximative methods. Here we show, tunable, coherent couplings and interference in a two-dimensional ion microtrap array, completing the toolbox for a reconfigurable quantum simulator. Previously, couplings and entangling interactions between sites in one-dimensional traps have been realized, while coupling remained elusive in microtrap approaches. Our architecture is based on well isolatable ions as identical quantum entities hovering above scalable CMOS chips. In contrast to other multi-dimensional approaches, it allows individual control in arbitrary, even non-periodic, lattice structures. Embedded control structures can exploit the long-range Coulomb interaction to configure synthetic, fully connected many-body systems to address multi-dimensional problems.

The electronic and motional degrees of freedom of trapped ions can be controlled and coherently coupled on the level of individual quanta. Assembling complex quantum systems ion by ion while keeping this unique level of control remains a challenging task. For many applications, linear chains of ions in conventional traps are ideally suited to address this problem. However, driven motion due to the magnetic or radio-frequency electric trapping fields sometimes limits the performance in one dimension and severely affects the extension to higher dimensional systems. Here, we report on the trapping of multiple Barium ions in a single-beam optical dipole trap without radio-frequency or additional magnetic fields. We study the persistence of order in ensembles of up to six ions within the optical trap, measure their temperature and conclude that the ions form a linear chain, commonly called a one-dimensional Coulomb crystal. As a proof-of-concept demonstration, we access the collective motion and perform spectrometry of the normal modes in the optical trap. Our system provides a platform which is free of driven motion and combines advantages of optical trapping, such as state-dependent confinement and nano-scale potentials, with the desirable properties of crystals of trapped ions, such as long-range interactions featuring collective motion. Starting with small numbers of ions, it has been proposed that these properties would allow the experimental study of many-body physics and the onset of structural quantum phase transitions between one- and two-dimensional crystals.

We propose a method to simulate the dynamics of spin-boson models with small crystals of trapped ions where the electronic degree of freedom of one ion is used to encode the spin while the collective vibrational degrees of freedom are employed to form an effective harmonic environment. The key idea of our approach is that a single damped mode can be used to provide a harmonic environment with Lorentzian spectral density. More complex spectral functions can be tailored by combining several individually damped modes. We propose to work with mixed-species crystals such that one species serves to encode the spin while the other species is used to cool the vibrational degrees of freedom to engineer the environment. The strength of the dissipation on the spin can be controlled by tuning the coupling between spin and vibrational degrees of freedom. In this way the dynamics of spin-boson models with macroscopic and non-Markovian environments can be simulated using only a few ions. We illustrate the approach by simulating an experiment with realistic parameters and show by computing quantitative measures that the dynamics is genuinely non-Markovian.

Trapped atomic ions enable a precise quantification of the flow of information between internal and external degrees of freedom by employing a non-Markovianity measure [H.-P. Breuer et al., Phys. Rev. Lett. 103, 210401 (2009)]. We reveal that the nature of projective measurements in quantum mechanics leads to a fundamental, nontrivial bias in this measure. We observe and study the functional dependence of this bias to permit a demonstration of applications of local quantum probing. An extension of our approach can act as a versatile reference, relevant for understanding complex systems.

We report on single Barium ions confined in a near-infrared optical dipole trap for up to three seconds in absence of any radio-frequency fields. Additionally, the lifetime in a visible optical dipole trap is increased by two orders of magnitude as compared to the state-of-the-art using an efficient repumping method. We characterize the state-dependent potentials and measure an upper bound for the heating rate in the near-infrared trap. These findings are beneficial for entering the regime of ultracold interaction in atom-ion ensembles exploiting bichromatic optical dipole traps. Long lifetimes and low scattering rates are essential to reach long coherence times for quantum simulations in optical lattices employing many ions, or ions and atoms.

We present two methods for characterization of motional-mode configurations that are generally applicable to the weak and strong-binding limit of single or multiple trapped atomic ions. Our methods are essential to realize control of the individual as well as the common motional degrees of freedom. In particular, when implementing scalable radio-frequency trap architectures with decreasing ion-electrode distances, local curvatures of electric potentials need to be measured and adjusted precisely, e.g., to tune phonon tunneling and control effective spin-spin interaction. We demonstrate both methods using single $^{25}$Mg$^+$ ions that are individually confined $40\,μ$m above a surface-electrode trap array and prepared close to the ground state of motion in three dimensions.

We consider the transversal modes of ions in a linear radio frequency (rf) trap where we control the time dependent axial confinement to show that we can excite quanta of motion via a two-mode squeezing process. This effect is analogous to phenomena predicted to occur during the evaporation of black holes and cosmological particle creation, in general out of reach for experimental investigation. As substantial advantage of this proposal in comparison to previous ones we propose to exploit radial and axial modes simultaneously to permit experimental access of these effects based on state-of-the-art technology. In addition, we propose to create and explore entanglement, starting with two ions, and relate the results to fundamental aspects of the entropy of black holes.

A custom-built and precisely controlled quantum system may offer access to a fundamental understanding of another, less accessible system of interest. A universal quantum computer is currently out of reach, but an analog quantum simulator that makes the relevant observables, interactions, and states of a quantum model accessible could permit experimental insight into complex quantum dynamics that are intractable on conventional computers. Several platforms have been suggested and proof-of-principle experiments have been conducted. Here we characterise two-dimensional arrays of three ions trapped by radio-frequency fields in individually controlled harmonic wells forming equilateral triangles with side lengths 40 and 80 micrometer. In our approach, which is scalable to arbitrary two dimensional lattices, we demonstrate individual control of the electronic and motional degrees of freedom, preparation of a fiducial initial state with ion motion close to the ground state, as well as tuning of crucial couplings between ions within experimental sequences. Our work paves the way towards an analog quantum simulator of two-dimensional systems designed at will.

We introduce a scheme that exploits laser cooling and phonon-mediated spin-spin interactions in crystals of trapped atomic ions to explore the transport of energy through a quantum magnet. We show how to implement an effective transport window to control the flow of energy through the magnet even in the absence of fermionic statistics for the carriers. This is achieved by shaping the density of states of the effective thermal reservoirs that arise from the interaction with the external bath of the modes of the electromagnetic field, and can be experimentally controlled by tuning the laser frequencies and intensities appropriately. The interplay of this transport window with the spin-spin interactions is exploited to build an analogue of the Coulomb-blockade effect in nano-scale electronic devices, and opens new possibilities to study quantum effects in energy transport.

We use trapped atomic ions forming a hybrid Coulomb crystal, and exploit its phonons to study an isolated quantum system composed of a single spin coupled to an engineered bosonic environment. We increase the complexity of the system by adding ions and controlling coherent couplings and, thereby, we observe the emergence of thermalization: Time averages of spin observables approach microcanonical averages while related fluctuations decay. Our platform features precise control of system size, coupling strength, and isolation from the external world to explore the dynamics of equilibration and thermalization.

Optical trapping and ions combine unique advantages of independently striving fields of research. Light fields can form versatile potential landscapes, such as optical lattices, for neutral and charged atoms, avoiding detrimental implications of established radiofrequency (rf) traps while mediating interaction via long range Coulomb forces, controlling and detecting motional and electronic states on the quantum level. Here we show optical trapping of $^{138}$Ba$^{+}$ ions in the absence of rf fields in a far-detuned dipole trap, suppressing photon scattering by three and the related recoil heating by four orders of magnitude. To enhance the prospects for optical as well as hybrid traps, we demonstrate a novel method for stray electric field compensation to a level below 9 mV/m. Our results will be relevant, for example, for ion-atom ensembles, to enable four to five orders of magnitude lower common temperatures, accessing the regime of ultracold interaction and chemistry, where quantum effects are predicted to dominate.

We report on three-dimensional optical trapping of single ions in an optical lattice formed by two counter-propagating laser beams. We characterize the trapping parameters of the standing wave using the ion as a sensor stored in a hybrid trap consisting of a radio-frequency (rf), a dc, and the optical potential. When loading ions directly from the rf into the standing-wave trap, we observe a dominant heating rate. Monte Carlo simulations confirm rf-induced parametric excitations within the deep optical lattice as the main source. We demonstrate a way around this effect by an alternative transfer protocol which involves an intermediate step of optical confinement in a single-beam trap avoiding the temporal overlap of the standing wave and the rf field. Implications arise for hybrid (rf/optical) and pure optical traps as platforms for ultra-cold chemistry experiments exploring atom--ion collisions or quantum simulation experiments with ions, or combinations of ions and atoms.

We describe a versatile toolbox for the quantum simulation of many-body lattice models, capable of exploring the combined effects of background Abelian and non-Abelian gauge fields, bond and site disorder, and strong on-site interactions. We show how to control the quantum dynamics of particles trapped in lattice potentials by the photon-assisted tunneling induced by periodic drivings. This scheme is general enough to be applied to either bosons or fermions with the additional advantage of being non-perturbative. It finds an ideal application in microfabricated ion trap arrays, where the quantized vibrational modes of the ions can be described by a quantum lattice model. We present a detailed theoretical proposal for a quantum simulator in that experimental setup, and show that it is possible to explore phases of matter that range from the fractional quantum Hall effect, to exotic strongly-correlated glasses, or flux-lattice models decorated with arbitrary patterns of localized defects.

We recently reported on a proof-of-principle experiment demonstrating optical trapping of an ion in a single-beam dipole trap superimposed by a static electric potential [Nat. Photonics 4, 772--775 (2010)]. Here, we first discuss the experimental procedures focussing on the influence and consequences of the static electric potential. These potentials can easily prevent successful optical trapping, if their configuration is not chosen carefully. Afterwards, we analyse the dipole trap experiments with different analytic models, in which different approximations are applied. According to these models the experimental results agree with recoil heating as the relevant heating effect. In addition, a Monte-Carlo simulation has been developed to refine the analysis. It reveals a large impact of the static electric potential on the dipole trap experiments in general. While it supports the results of the analytic models for the parameters used in the experiments, the analytic models cease their validity for significantly different parameters. Finally, we propose technical improvements for future realizations of experiments with optically trapped ions.

We examine the prospects of discrete quantum walks (QWs) with trapped ions. In particular, we analyze in detail the limitations of the protocol of Travaglione and Milburn (PRA 2002) that has been implemented by several experimental groups in recent years. Based on the first realization in our group (PRL 2009), we investigate the consequences of leaving the scope of the approximations originally made, such as the Lamb--Dicke approximation. We explain the consequential deviations from the idealized QW for different experimental realizations and an increasing number of steps by taking into account higher-order terms of the quantum evolution. It turns out that these become dominant after a few steps already, which is confirmed by experimental results and is currently limiting the scalability of this approach. Finally, we propose a new scheme using short laser pulses, derived from a protocol from the field of quantum computation. We show that the new scheme is not subject to the above-mentioned restrictions, and analytically and numerically evaluate its limitations, based on a realistic implementation with our specific setup. Implementing the protocol with state-of-the-art techniques should allow for substantially increasing the number of steps to 100 and beyond and should be extendable to higher-dimensional QWs.

Direct experimental access to some of the most intriguing quantum phenomena is not granted due to the lack of precise control of the relevant parameters in their naturally intricate environment. Their simulation on conventional computers is impossible, since quantum behaviour arising with superposition states or entanglement is not efficiently translatable into the classical language. However, one could gain deeper insight into complex quantum dynamics by experimentally simulating the quantum behaviour of interest in another quantum system, where the relevant parameters and interactions can be controlled and robust effects detected sufficiently well. We report on the progress in experimentally simulating quantum many-body physics with trapped ions.

This work theoretically addresses the trapping an ionized atom with a single valence electron by means of lasers, analyzing qualitatively and quantitatively the consequences of the net charge of the particle. In our model, the coupling between the ion and the electromagnetic field includes the charge monopole and the internal dipole, within a multipolar expansion of the interaction Hamiltonian. Specifically, we perform a Power-Zienau-Woolley transformation, taking into account the motion of the center of mass. The net charge produces a correction in the atomic dipole which is of order $m_e/M$ with $m_e$ the electron mass and $M$ the total mass of the ion. With respect to neutral atoms, there is also an extra coupling to the laser field which can be approximated by that of the monopole located at the position of the center of mass. These additional effects, however, are shown to be very small compared to the dominant dipolar trapping term.