Julian Schmidt

We demonstrate a state-dependent Gaussian gate set on the motional modes of trapped $^{40}$Ca$^+$ ions, realized with an optical tweezer. Dynamic control of the tweezer intensity and position enables local displacement, squeezing, phase-space rotation, and beamsplitter operations, constituting a complete gate set. By varying the tweezer position relative to the ion, we show how the strength of each operation is set by the corresponding spatial derivative of the local optical potential. We further demonstrate the inherent dependence of each operation on the ion's internal state and use coherent spin-motion coupling provided by the tweezer to create a motional cat state. Our work establishes optical tweezers as a unified and local resource for continuous-variable quantum control in trapped ion systems.

We use quantum-logic spectroscopy (QLS) and interrogate rotational transitions of a single CaH+ ion with a highly coherent frequency comb, achieving a fractional statistical uncertainty for a transition line center of 4 x 10^-13. We also improve the resolution in measurement of the Stark effect due to the radio-frequency (rf) electric field experienced by a molecular ion in an rf Paul trap, which we characterize and model. This allows us to determine the electric dipole moment of CaH+ by systematically displacing the ion to sample different known rf electric fields and measuring the resultant shifts in transition frequency.

We report on the production of cold, state-selected H$_2^+$ molecular ions in a linear RF trap. The ions are produced by (3+1) resonance-enhanced multi-photon ionisation (REMPI) of H$_2$, and sympathetically cooled by laser-cooled Be$^+$ ions. After demonstrating and characterizing the REMPI process, we use photodissociation by a deep UV laser at 213~nm to verify the high vibrational purity of the produced H$_2^+$ ion samples. Moreover, the large difference between the photodissociation efficiencies of ions created in the $v=0$ and $v=1$ levels provides a way to detect a $v=0 \to 1$ transition. These results pave the way towards high-resolution vibrational spectroscopy of H$_2^+$ for fundamental metrology applications.

We study a method for mass-selective removal of ions from a Paul trap by parametric excitation. This can be achieved by applying an oscillating electric quadrupole field at twice the secular frequency $ω_{\text{sec}}$ using pairs of opposing electrodes. While excitation near the resonance with the frequency $ω_{\text{sec}}$ only leads to a linear increase of the amplitude with excitation duration, parametric excitation near $2\, ω_{\text{sec}}$ results in an exponential increase of the amplitude. This enables efficient removal of ions from the trap with modest excitation voltages and narrow bandwidth, therefore substantially reducing the disturbance of ions with other charge-to-mass ratios. We numerically study and compare the mass selectivity of the two methods. In addition, we experimentally show that the barium isotopes with 136 and 137 nucleons can be removed from small ion crystals and ejected out of the trap while keeping $^{138}\text{Ba}^{+}$ ions Doppler cooled, corresponding to a mass selectivity of better than $Δm / m = 1/138$. This method can be widely applied to ion trapping experiments without major modifications, since it only requires modulating the potential of the ion trap.

The electronic and motional degrees of freedom of trapped ions can be controlled and coherently coupled on the level of individual quanta. Assembling complex quantum systems ion by ion while keeping this unique level of control remains a challenging task. For many applications, linear chains of ions in conventional traps are ideally suited to address this problem. However, driven motion due to the magnetic or radio-frequency electric trapping fields sometimes limits the performance in one dimension and severely affects the extension to higher dimensional systems. Here, we report on the trapping of multiple Barium ions in a single-beam optical dipole trap without radio-frequency or additional magnetic fields. We study the persistence of order in ensembles of up to six ions within the optical trap, measure their temperature and conclude that the ions form a linear chain, commonly called a one-dimensional Coulomb crystal. As a proof-of-concept demonstration, we access the collective motion and perform spectrometry of the normal modes in the optical trap. Our system provides a platform which is free of driven motion and combines advantages of optical trapping, such as state-dependent confinement and nano-scale potentials, with the desirable properties of crystals of trapped ions, such as long-range interactions featuring collective motion. Starting with small numbers of ions, it has been proposed that these properties would allow the experimental study of many-body physics and the onset of structural quantum phase transitions between one- and two-dimensional crystals.

We report on single Barium ions confined in a near-infrared optical dipole trap for up to three seconds in absence of any radio-frequency fields. Additionally, the lifetime in a visible optical dipole trap is increased by two orders of magnitude as compared to the state-of-the-art using an efficient repumping method. We characterize the state-dependent potentials and measure an upper bound for the heating rate in the near-infrared trap. These findings are beneficial for entering the regime of ultracold interaction in atom-ion ensembles exploiting bichromatic optical dipole traps. Long lifetimes and low scattering rates are essential to reach long coherence times for quantum simulations in optical lattices employing many ions, or ions and atoms.

Optical trapping and ions combine unique advantages of independently striving fields of research. Light fields can form versatile potential landscapes, such as optical lattices, for neutral and charged atoms, avoiding detrimental implications of established radiofrequency (rf) traps while mediating interaction via long range Coulomb forces, controlling and detecting motional and electronic states on the quantum level. Here we show optical trapping of $^{138}$Ba$^{+}$ ions in the absence of rf fields in a far-detuned dipole trap, suppressing photon scattering by three and the related recoil heating by four orders of magnitude. To enhance the prospects for optical as well as hybrid traps, we demonstrate a novel method for stray electric field compensation to a level below 9 mV/m. Our results will be relevant, for example, for ion-atom ensembles, to enable four to five orders of magnitude lower common temperatures, accessing the regime of ultracold interaction and chemistry, where quantum effects are predicted to dominate.