Daniel J. Blumenthal

Trapped ions are a leading technology for quantum computing, but their reliance on bespoke tabletop laser and optical systems remains a major obstacle to scaling and robustness. Integrated silicon nitride lasers, compatible with future monolithic integration with surface electrode ion traps, have recently demonstrated frequency-selective qubit state preparation and measurement as well as interrogation of an optical clock transition. However, coherent qubit gates driven by integrated laser sources have not yet been demonstrated because coherent quantum logic imposes substantially more stringent performance requirements on the laser. Here, we use a visible-wavelength integrated Brillouin laser stabilized to an integrated coil resonator to drive coherent single- and two-qubit gates with $^{88}$Sr$^+$ optical qubits. We measure an average single-qubit fidelity of 99.61% $\pm$ 0.03% per Clifford gate with randomized benchmarking and use a two-qubit Mølmer-Sørensen interaction to generate an entangled Bell state with a fidelity of 92.35% $\pm$ 1.50%. The qubit exhibits a bare Ramsey coherence time of 660 $\pm$ 9 $μ$s, extended to 1.750 $\pm$ 0.033 ms by spin echo. These results demonstrate that integrated visible-wavelength narrow-linewidth photonic lasers can meet the phase-noise requirements for coherent trapped ion quantum logic, providing a path for scalable optical systems integrated within trapped ion quantum processors.

Modulation and control of lasers and optical signals is necessary for trapped-ion and cold neutral atom quantum systems. Given the diversity of atomic species, experimental modalities, and architectures, integrated optical modulators designed to operate across the visible to near-infrared spectrum are a key step towards portable, robust, and compact quantum computers, clocks, and sensors. Integrated optical modulators that are wavelength-independent, CMOS-compatible, and capable of maintaining low waveguide losses and a high resonator quality factor, DC-coupled broadband frequency response, and low power consumption, are essential for scalable photonic integration. Yet progress towards these goals has remained limited. Here we demonstrate four types of integrated stress-optic lead zirconate titanate (PZT) silicon nitride modulators: a coil Mach-Zehnder modulator, a coil pure phase modulator, and bus-coupled and add-drop ring resonator modulators, with operation from 493 nm to 780 nm. The coil MZM operates at 532 nm with a V$π$ of 2.8V, a 0.4 MHz 3-dB bandwidth, and an extinction ratio of 21.5dB. The coil phase modulator operates at 493 nm with a V$π$ of 2.8V and low residual amplitude modulation of -34 dB at a 1kHz offset. The bus-coupled ring resonator modulator operates at 493 nm and the add-drop ring resonator modulator operates at 780 nm. The ring-based modulators have an intrinsic quality factor of 3.4 million and 1.9 million, a linear tuning strength of 0.9 GHz/V and 1 GHz/V, and a 3-dB bandwidth of 2.6 MHz and 10 MHz, respectively. All four modulator designs maintain the low optical waveguide loss of SiN, are DC coupled with broadband frequency response, operate independent of wavelength, and consume only tens of nW per actuator. Such solutions unlock the potential for further integration with other precision SiN components to realize chip-scale atomic and quantum systems.

Precision atomic and quantum experiments rely on ultra-stable narrow linewidth lasers constructed using table-top ultra-low expansion reference cavities. These experiments often require multiple lasers, operating at different wavelengths, to perform key steps used in state preparation and measurement required in quantum sensing and computing. This is traditionally achieved by disciplining a cavity-stabilized laser to a key atomic transition and then transferring the transition linewidth and stability to other lasers using the same reference cavity in combination with bulk-optic frequency shifting such as acousto-optic modulators. Transitioning such capabilities to a low cost photonic-integrated platform will enable a wide range of portable, low power, scalable quantum experiments and applications. Yet, today's bulk optic approaches pose challenges related to lack of cavity tunability, large free spectral range, and limited photonic integration potential. Here, we address these challenges with demonstration of an agile photonic-integrated 780 nm ultra-high-Q tunable silicon nitride reference cavity that performs multiple critical experimental steps including laser linewidth narrowing, high resolution rubidium spectroscopy, dual-stage stabilization to a rubidium transition, and stability transfer to other lasers. We achieve up to 20 dB of frequency noise reduction at 10 kHz offset, precision spectroscopy over a 250 MHz range, and dual-stage locking to rubidium with an Allan deviation of $8.5 \times 10^{-12}$ at 1 s and up to 40 dB reduction at 100 Hz. We further demonstrate the transfer of this atomic stability to a second laser, via the rubidium-disciplined cavity, and demonstrate multi-wavelength Rydberg electrometry quantum sensing. These results pave the path for integrated, compact, and scalable solutions for quantum sensing, computing and other atomic and trapped ion applications.

Narrow linewidth stabilized lasers are central to precision applications that operate across the visible to short-wave infrared wavelengths, including optical clocks, quantum sensing and computing, ultra-low noise microwave generation, and fiber sensing. Today, these spectrally pure sources are realized using multiple external cavity tabletop lasers locked to bulk-optic free-space reference cavities. Integration of this technology will enable portable precision applications with improved reliability and robustness. Here, we report wavelength-flexible design and operation, over more than an octave span, of an integrated coil-resonator-stabilized Brillouin laser architecture. Leveraging a versatile two-stage noise reduction approach, we achieve low linewidths and high stability with chip-scale laser designs based on the ultra-low-loss, CMOS-compatible silicon nitride platform. We report operation at 674 and 698 nm for applications to strontium neutral and trapped-ion clocks, quantum sensing and computing, and at 1550 nm for applications to fiber sensing and ultra-low phase noise microwave generation. Over this range we demonstrate frequency noise reduction from 1 Hz to 10 MHz resulting in 1.0 Hz -17 Hz fundamental and 181 Hz - 630 Hz integral linewidths and an Allan deviation of 6.5 x 10-13 at 1 ms for 674 nm, 6.0 x 10-13 at 15 ms for 698 nm, and 2.6 x10-13 at 15 ms for 1550 nm. This represents the lowest achieved linewidths and highest stability for integrated stabilized Brillouin lasers over an order of magnitude improvement in operating wavelength range. These results unlock the potential of integrated, ultra-low-phase-noise stabilized lasers for precision applications and further integration in systems-on-chip solutions.

Integrating precise, stable, ultra-low noise visible light lasers into atomic systems is critical for advancing quantum information sciences and improving scalability and portability. Trapped ions are a leading approach for high-fidelity quantum computing, high-accuracy optical clocks, and precision quantum sensors. However, current ion-based systems rely on bulky, lab-scale precision lasers and optical stabilization cavities for optical clock and qubit operations, constraining the size, weight, scalability, and portability of atomic systems. Chip-scale integration of ultra-low noise lasers and reference cavities operating directly at optical clock transitions and capable of qubit and clock operations will represent a major transformation in atom and trapped ion-based quantum technologies. However, this goal has remained elusive. Here we report the first demonstration of chip-scale optical clock and qubit operations on a trapped ion using a photonic integrated direct-drive visible wavelength Brillouin laser stabilized to an integrated 3-meter coil-resonator reference cavity and the optical clock transition of a $^{88}$Sr$^+$ ion trapped on a surface electrode chip. We also demonstrate for the first time, to the best of our knowledge, trapped-ion spectroscopy and qubit operations such as Rabi oscillations and high fidelity (99%) qubit state preparation and measurement (SPAM) using direct drive integrated photonic technologies without bulk optic stabilization cavities or second harmonic generation. Our chip-scale stabilized Brillouin laser exhibits a 6 kHz linewidth with the 0.4 Hz quadrupole transition of $^{88}$Sr$^+$ and a self-consistent coherence time of 60 $μ$s via Ramsey interferometry on the trapped ion qubit. Furthermore, we demonstrate the stability of the locked Brillouin laser to 5$\times10^{-13}/ \sqrtτ$ at 1 second using dual optical clocks.