Dylan J Gorman

Many important chemical and biochemical processes in the condensed phase are notoriously difficult to simulate numerically. Often this difficulty arises from the complexity of simulating dynamics resulting from coupling to structured, mesoscopic baths, for which no separation of time scales exists and statistical treatments fail. A prime example of such a process is vibrationally assisted charge or energy transfer. A quantum simulator, capable of implementing a realistic model of the system of interest, could provide insight into these processes in regimes where numerical treatments fail. We take a first step towards modeling such transfer processes using an ion trap quantum simulator. By implementing a minimal model, we observe vibrationally assisted energy transport between the electronic states of a donor and an acceptor ion augmented by coupling the donor ion to its vibration. We tune our simulator into several parameter regimes and, in particular, investigate the transfer dynamics in the nonperturbative regime often found in biochemical situations.

The detailed characterization of non-trivial coherence properties of composite quantum systems of increasing size is an indispensable prerequisite for scalable quantum computation, as well as for understanding of nonequilibrium many-body physics. Here we show how autocorrelation functions in an interacting system of phonons as well as the quantum discord between distinct degrees of freedoms can be extracted from a small controllable part of the system. As a benchmark, we show this in chains of up to 42 trapped ions, by tracing a single phonon excitation through interferometric measurements of only a single ion in the chain. We observe the spreading and partial refocusing of the excitation in the chain, even on a background of thermal excitations. We further show how this local observable reflects the dynamical evolution of quantum discord between the electronic state and the vibrational degrees of freedom of the probe ion.

Electric field noise in proximity to metallic surfaces is a poorly understood phenomenon that appears in different areas of physics. Trapped ion quantum information processors are particular susceptible to this noise, leading to motional decoherence which ultimately limits the fidelity of quantum operations. On the other hand they present an ideal tool to study this effect, opening new possibilities in surface science. In this work we analyze and measure the polarization of the noise field in a micro-fabricated ion trap for various noise sources. We find that technical noise sources and noise emanating directly from the surface give rise to different degrees of polarization which allows us to differentiate between the two noise sources. Based on this, we demonstrate a method to infer the magnitude of surface noise in the presence of technical noise.

Atomic ions, confined in radio-frequency Paul ion traps, are a promising candidate to host a future quantum information processor. In this letter, we demonstrate a method to couple two motional modes of a single trapped ion, where the coupling mechanism is based on applying electric fields rather than coupling the ion's motion to a light field. This reduces the design constraints on the experimental apparatus considerably. As an application of this mechanism, we cool a motional mode close to its ground state without accessing it optically. As a next step, we apply this technique to measure the mode's heating rate, a crucial parameter determining the trap quality. In principle, this method can be used to realize a two-mode quantum parametric amplifier.