P. C. Haljan

An array of ions in a linear radio-frequency (RF) Paul trap is a good candidate for investigating structural phase transitions, such as the linear-to-zigzag (LZ) transition, due to the convenient control provided by modification of the trap confinement strength. In such studies, the trap secular frequencies are a key factor that limits the stability of the critical point (CP). In this paper, we implement secular-frequency stabilization, including active feedback stabilization of the RF voltage near the trap electrodes, and achieve a stability of better than 5~ppm over 200~s for both transverse and axial potentials. To evaluate the combined long-term stability of the trap potential in both directions, we measure the zigzag (ZZ) mode frequency near the CP, where the effect of instability in both trap directions is substantially amplified. The short-term noise within a limited spectral window is also suppressed by this scheme, as inferred from decoherence rates of the ZZ mode measured at different frequencies with Ramsey fringes. We also identify that the limitation of the secular frequency stability is mainly from the imperfect temperature insensitivity of voltage dividers and RF detectors, and as a result improvement of lab temperature stability is of great help for stabilizing the trap frequency.

While engineered quantum systems are a general route to the manipulation of multipartite quantum states, access in a physical system to a continuous quantum phase transition under sufficient control offers the possibility of an intrinsic source of entangled states. To this end we realize the quantum version of the linear-zigzag structural transition for arrays of up to five ground state-cooled ions held in a linear Paul trap and we demonstrate several of the control requirements towards entangled-state interferometry near the critical point. Using in-situ spectroscopy we probe the energy level structure and occupation of the soft mode associated with the structural transition, and show a stable critical point and majority ground state occupation crossing the transition. We resolve biases arising from trap electrode asymmetries that change the nature of the transition, show that they can be suppressed by varying the ion number, and demonstrate control of the transition bias using optical dipole forces.

Using a laser polarization gradient, we realize 3D Sisyphus cooling of $^{171}$Yb$^+$ ions confined in and near the Lamb-Dicke regime in a linear Paul trap. The cooling rate and final mean motional energy of a single ion are characterized as a function of laser intensity and compared to semiclassical and quantum simulations. Sisyphus cooling is also applied to a linear string of four ions to obtain a mean energy of 1-3 quanta for all vibrational modes, an approximately order-of-magnitude reduction below Doppler cooled energies. This is used to enable subsequent, efficient sideband laser cooling.

The spontaneous nucleation and dynamics of topological kink defects have been studied in trapped arrays of 41-43 Yb ions. The number of kinks formed as a function of quench rate across the linear-zigzag transition is measured in the under-damped regime of the inhomogeneous Kibble-Zurek theory. The experimental results agree well with molecular dynamics simulations, which show how losses mask the intrinsic nucleation rate. Simulations indicate that doubling the ion number and optimization of laser cooling can help reduce the effect of losses. A range of kink dynamics is observed including configural change, motion and lifetime, and behavioral sensitivity to ion number.

We report the laser-cooling and confinement of Cd atoms in a magneto-optical trap, and characterize the loading process from the background Cd vapor. The trapping laser drives the 1S0-1P1 transition at 229 nm in this two-electron atom and also photoionizes atoms directly from the 1P1 state. This photoionization overwhelms the other loss mechanisms and allows a direct measurement of the photoionization cross section, which we measure to be 2(1)x10^(-16)cm^(2) from the 1P1 state. When combined with nearby laser-cooled and trapped Cd^(+) ions, this apparatus could facilitate studies in ultracold interactions between atoms and ions.

Atomic cadmium ions are loaded into radiofrequency ion traps by photoionization of atoms in a cadmium vapor with ultrafast laser pulses. The photoionization is driven through an intermediate atomic resonance with a frequency-quadrupled mode-locked Ti:Sapphire laser that produces pulses of either 100 fsec or 1 psec duration at a central wavelength of 229 nm. The large bandwidth of the pulses photoionizes all velocity classes of the Cd vapor, resulting in high loading efficiencies compared to previous ion trap loading techniques. Measured loading rates are compared with a simple theoretical model, and we conclude that this technique can potentially ionize every atom traversing the laser beam within the trapping volume. This may allow the operation of ion traps with lower levels of background pressures and less trap electrode surface contamination. The technique and laser system reported here should be applicable to loading most laser-cooled ion species.

Simultaneous measurement of multiple qubits stored in hyperfine levels of trapped 111Cd+ ions is realized with an intensified charge-coupled device (CCD) imager. A general theory of fluorescence detection for hyperfine qubits is presented and applied to experimental data. The use of an imager for photon detection allows for multiple qubit state measurement with detection fidelities of greater than 98%. Improvements in readout speed and fidelity are discussed in the context of scalable quantum computation architectures.

We report the implementation of Grover's quantum search algorithm in the scalable system of trapped atomic ion quantum bits. Any one of four possible states of a two-qubit memory is marked, and following a single query of the search space, the marked element is successfully recovered with an average probability of 60(2)%. This exceeds the performance of any possible classical search algorithm, which can only succeed with a maximum average probability of 50%.

A Mølmer-Sørensen entangling gate is realized for pairs of trapped $^{111}$Cd$^+$ ions using magnetic-field insensitive "clock" states and an implementation offering reduced sensitivity to optical phase drifts. The gate is used to generate the complete set of four entangled states, which are reconstructed and evaluated with quantum-state tomography. An average target-state fidelity of 0.79 is achieved, limited by available laser power and technical noise. The tomographic reconstruction of entangled states demonstrates universal quantum control of two ion-qubits, which through multiplexing can provide a route to scalable architectures for trapped-ion quantum computing.

There are several known schemes for entangling trapped ion quantum bits for large-scale quantum computation. Most are based on an interaction between the ions and external optical fields, coupling internal qubit states of trapped-ions to their Coulomb-coupled motion. In this paper, we examine the sensitivity of these motional gate schemes to phase fluctuations introduced through noisy external control fields, and suggest techniques to suppress the resulting phase decoherence.

Favored schemes for trapped-ion quantum logic gates use bichromatic laser fields to couple internal qubit states with external motion through a "spin-dependent force." We introduce a new degree of freedom in this coupling that reduces its sensitivity to phase decoherence. We demonstrate bichromatic spin-dependent forces on a single trapped $^{111}$Cd$^+$ ion, and show that phase coherence of the resulting "Schrödinger-cat" states of motion depends critically upon the spectral arrangement of the optical fields. This applies directly to the operation of entangling gates on multiple ions.

We report on ground state laser cooling of single 111Cd+ ions confined in radio-frequency (Paul) traps. Heating rates of trapped ion motion are measured for two different trapping geometries and electrode materials, where no effort was made to shield the electrodes from the atomic Cd source. The low measured heating rates suggest that trapped 111Cd+ ions may be well-suited for experiments involving quantum control of atomic motion, including applications in quantum information science.