R. N. Wolf

Mass spectrometry of $^{75}$Zn ground and isomeric states from in-trap decay of $^{75}$Cu

M. Müller, N. A. Althubiti [2,3], D. Atanasov [1], K. Blaum [1], R. B. Cakirli [1], T. E. Cocolios [4], F. Herfurth [5], S. Kreim [1], D. Lunney [6], V. Manea [1,7], N. Minkov [1,8], D. Neidherr [5], M. Rosenbusch [9], L. Schweikhard [9], A. Welker [7,10], F. Wienholtz [7,9], R. N. Wolf [1]

Abstract

We report on high-precision mass measurements of the ground and first isomeric state of $^{75}$Zn, performed using the time-of-flight ion-cyclotron-resonance technique at the ISOLTRAP Penning-trap mass spectrometer at ISOLDE/CERN. The isomeric state was produced using in-trap decay of $^{75}$Cu. This marks the first direct investigation of the isomeric state of $^{75}$Zn via mass spectrometry. The isomer was observed at an excitation energy of 123.7(20) keV, in 2$\,σ$ agreement with the value previously determined through decay spectroscopy. In addition, our measurements correct a misassignment of the ground-state mass excess based on a previous measurement by Baruah et al., revising the value to -62681.0(21) keV. To further investigate the earlier discrepancy, we explored the spin-parity assignments of the ground and isomeric states in $^{75}$Zn using Skyrme Hartree-Fock plus Bardeen-Cooper-Schrieffer theoretical calculations, given the absence of definitive experimental data. In light of the laser spectroscopy results from Wraith et al., our results add strong evidence for a spin-1/2 ground state, which would agree with large-scale shell-model predictions as well as explaining disagreements with the Monte Carlo Shell Model.

Charge radii, moments and masses of mercury isotopes across the N = 126 shell closure

T. Day Goodacre [1,2,3,4,5], A. V. Afanasjev, A. E. Barzakh, L. Nies [2,6], B. A. Marsh, S. Sels [2,7,4], U. C. Perera, P. Ring [8], F. Wienholtz [2,6,9,10], A. N. Andreyev, P. Van Duppen [7,1,11], N. A. Althubiti, B. Andel [7,12], D. Atanasov [13,3], R. S. Augusto, J. Billowes [1], K. Blaum [13,1,7,9,5,2,14,15], T. E. Cocolios, J. G. Cubiss, G. J. Farooq-Smith, D. V. Fedorov, V. N. Fedosseev, K. T. Flanagan, L. P. Gaffney, L. Ghys [7,16], A. Gottberg [3,17], M. Huyse [7], S. Kreim [13,2], P. Kunz [3,18], D. Lunney [19,1,2], K. M. Lynch, V. Manea [13], Y. Martinez Palenzuela [7,2,5], T. M. Medonca, P. L. Molkanov, M. Mougeot [2], J. P. Ramos, M. Rosenbusch [6,2,20], R. E. Rossel, S. Rothe [2], L. Schweikhard [6,5], M. D. Seliverstov, P. Spagnoletti [15], C. Van Beveren [7], M. Veinhard [2], E. Verstraelen [7], A. Welker [2,21], K. Wendt [20,13,6], R. N. Wolf, A. Zadvornaya [7], K. Zuber [21]

Abstract

Combining laser spectroscopy in a Versatile Arc Discharge and Laser Ion Source, with Penning-trap mass spectrometry at the CERN-ISOLDE facility, this work reports on mean-square charge radii of neutron-rich mercury isotopes across the $N = 126$ shell closure, the electromagnetic moments of $^{207}$Hg and more precise mass values of $^{206-208}$Hg. The odd-even staggering (OES) of the mean square charge radii and the kink at $N = 126$ are analyzed within the framework of covariant density functional theory (CDFT), with comparisons between different functionals to investigate the dependence of the results on the underlying single-particle structure. The observed features are defined predominantly in the particle-hole channel in CDFT, since both are present in the calculations without pairing. However, the magnitude of the kink is still affected by the occupation of the $1i_{11/2}$ and $2g_{9/2}$ orbitals with a dependence on the relative energies as well as pairing.

The Heidelberg compact electron beam ion traps

P. Micke [1,2], S. Kühn, L. Buchauer [1], J. R. Harries [3,1], T. M. Bücking, K. Blaum [1], A. Cieluch [1], A. Egl [1], D. Hollain [1], S. Kraemer [1], T. Pfeifer [1], P. O. Schmidt [2,4,1], R. X. Schüssler, Ch. Schweiger [1,5,6,7], T. Stöhlker, S. Sturm [1], R. N. Wolf [1], S. Bernitt [1,7], J. R. Crespo López-Urrutia

Abstract

Electron beam ion traps (EBIT) are ideal tools for both production and study of highly charged ions (HCI). In order to reduce their construction, maintenance, and operation costs we have developed a novel, compact, room-temperature design, the Heidelberg Compact EBIT (HC-EBIT). Four already commissioned devices operate at the strongest fields (up to 0.86 T) reported for such EBITs using permanent magnets, run electron beam currents up to 80 mA and energies up to 10 keV. They demonstrate HCI production, trapping, and extraction of pulsed Ar$^{16+}$ bunches and continuous 100 pA ion beams of highly charged Xe up to charge state 29+, already with a 4 mA, 2 keV electron beam. Moreover, HC-EBITs offer large solid-angle ports and thus high photon count rates, e. g., in x-ray spectroscopy of dielectronic recombination in HCIs up to Fe$^{24+}$, achieving an electron-energy resolving power of $E/ΔE > 1500$ at 5 keV. Besides traditional on-axis electron guns, we have also implemented a novel off-axis gun for laser, synchrotron, and free-electron laser applications, offering clear optical access along the trap axis. We report on its first operation at a synchrotron radiation facility demonstrating resonant photoexcitation of highly charged oxygen.