Xiang Zhang

Motion-mediated trapped-ion interactions commonly coordinate state-dependent forces on both target ions. Sequential optical access reduces the number of concurrent target channels but makes the relative phase between disjoint force windows a control variable. We derive a complex near-resonant description in which each window generates a displacement vector and ordered symplectic products between vectors on different ions produce the ZZ phase. Only relative boundary phases affect this area; a common phase shift is a gauge transformation. Building on the experimental precedent for alternating single-ion addressing, we develop matched-envelope phase and contrast controls that isolate this boundary-phase dependence without target-window overlap or hidden force in the dark gaps. The analysis separates phase generation from differential closure, projector-common motion, deterministic local-Z phases, spectator coupling, and control-parameter transfer. A conditional-Ramsey sequence gives continuous and reset contrasts of 0.998 and 0.996, with a reset-induced phase separation of 0.581 rad modulo $π/2$. In the representative comparison, sequential control uses fewer concurrent target channels but greater normalized force action than independently calibrated simultaneous control. All results are model-level estimates within the stated Lamb-Dicke, rotating-wave, and apparatus-input limits.

Quantum systems promise to revolutionize information processing science and technology [1-3]. The preservation of quantum coherence, the defining property of qubits, fundamentally constrains the performance of quantum information processing with quantum memories [4]. While trapped atomic ions theoretically support million-year coherence based on spontaneous emission [5-7], experimental demonstrations have reached far less, only about an hour [8-13]. Here we combine clock-state qubits with decoherence-free subspace (DFS) encoding to achieve coherence exceeding ten hours. Using correlation-based phase tracking in 171Yb+ ion pairs sympathetically cooled by 138Ba+ ion, we demonstrate this without magnetic shielding or enhanced microwave phase stabilization that previously limited coherence times. DFS encoding references the qubit phase to the inter-ion energy difference to reject microwave phase noise and common-mode magnetic fluctuations, while clock states provide environmental insensitivity. Throughout measurements extended to 1600 seconds, we observe minimal coherence decay, with exponential fits yielding a coherence time of (3.77 +/- 1.09) x 10^4 seconds. Our results establish DFS encoding as a form of passive error correction that eliminates technical noise constraints, unlocking the million-year coherence potential of atomic ions for scalable quantum information processing.

We experimentally demonstrate an unambiguous quantum state discrimination of two qubit states under a non-Hermitian Hamiltonian with parity-time-reversal ($\mathcal{PT}$) symmetry in a single trapped $^{40}$Ca$^+$ ion. We show that any two non-orthogonal states can become orthogonal subjected to time evolution of a $\mathcal{PT}$-symmetric Hamiltonian in both the $\mathcal{PT}$-symmetry preserving and broken regimes, thus can be discriminated deterministically. For a given pair of candidate states, we show that the parameters of the Hamiltonian must be confined in a proper range, within which there exists an optimal choice to realize quantum brachistochrone for the fastest orthogonalization. Besides, we provide a clear geometric picture and some analytic results to understand the main conclusions. Our work shows a promising application of non-Hermitian physics in quantum information processing.

Whether the observables of a physical system admit real values is of fundamental importance to a deep understanding of nature. In this work, we report a device-independent experiment to confirm that the joint reality of two observables on a single two-level system is incompatible with the assumption of operational completeness, which is strictly weaker than that of preparation noncontextuality. We implement two observables on a trapped $^{171}{\rm Yb}^{+}$ ion to test this incompatibility via violation of certain inequalities derived from both linear and nonlinear criteria. Moreover, by introducing a highly controllable dephasing channel, we show that the nonlinear criterion is more robust against noise. Our results push the fundamental limit to delineate the quantum-classical boundary and pave the way for exploring relevant problems in other scenarios.

Non-Hermitian systems with parity-time reversal ($\mathcal{PT}$) or anti-$\mathcal{PT}$ symmetry have attracted a wide range of interest owing to their unique characteristics and counterintuitive phenomena. One of the most extraordinary features is the presence of an exception point (EP), across which a phase transition with spontaneously broken $\mathcal{PT}$ symmetry takes place. We implement a Floquet Hamiltonian of a single qubit with anti-$\mathcal{PT}$ symmetry by periodically driving a dissipative quantum system of a single trapped ion. With stroboscopic emission and quantum state tomography, we obtain the time evolution of density matrix for an arbitrary initial state, and directly demonstrate information retrieval, eigenstates coalescence, and topological energy spectra as unique features of non-Hermitian systems.

Recent progresses on quantum control of cold atoms and trapped ions in both the scientific and technological aspects greatly advance the applications in precision measurement. Thanks to the exceptional controllability and versatility of these massive quantum systems, unprecedented sensitivity has been achieved in clocks, magnetometers and interferometers based on cold atoms and ions. Besides, these systems also feature many characteristics that can be employed to facilitate the applications in different scenarios. In this review, we briefly introduce the principles of optical clocks, cold atom magnetometers and atom interferometers used for precision measurement of time, magnetic field, and inertial forces. The main content is then devoted to summarize some recent experimental and theoretical progresses in these three applications, with special attention being paid to the new designs and possibilities towards better performance. The purpose of this review is by no means to give a complete overview of all important works in this fast developing field, but to draw a rough sketch about the frontiers and show the fascinating future lying ahead.

Ultraviolet (UV) diode lasers are widely used in many photonics applications. But their frequency stabilization schemes are not as mature as frequency-doubling lasers, mainly due to some limitations in the UV spectral region. Here we developed a high-performance UV frequency stabilization technique implemented directly on UV diode lasers by combining the dichroic atomic vapor laser lock and the resonant transfer cavity lock. As an example, we demonstrate a stable locking with frequency standard deviations of approximately 200 KHz and 300 KHz for 399nm and 370nm diode lasers in 20 minutes. We achieve a long-term frequency drift of no more than 1 MHz for the target 370nm laser within an hour, which was further verified with fluorescence counts rates of a single trapped $^{171}$Yb$^+$ ion. We also find strong linear correlations between lock points and environmental factors such as temperature and atmospheric pressure.

Modern computation relies crucially on modular architectures, breaking a complex algorithm into self-contained subroutines. A client can then call upon a remote server to implement parts of the computation independently via an application programming interface (API). Present APIs relay only classical information. Here we implement a quantum API that enables a client to estimate the absolute value of the trace of a server-provided unitary $U$. We demonstrate that the algorithm functions correctly irrespective of what unitary $U$ the server implements or how the server specifically realizes $U$. Our experiment involves pioneering techniques to coherently swap qubits encoded within the motional states of a trapped \Yb ion, controlled on its hyperfine state. This constitutes the first demonstration of modular computation in the quantum regime, providing a step towards scalable, parallelization of quantum computation.

The NOT gate that flips a classical bit is ubiquitous in classical information processing. However its quantum analogue, the universal NOT (UNOT) gate that flips a quantum spin in any alignment into its antipodal counterpart is strictly forbidden. Here we explore the connection between this discrepancy and how UNOT gates affect classical and quantum correlations. We show that while a UNOT gate always preserves classical correlations between two spins, it can non-locally increase or decrease their shared discord in ways that allow violation of the data processing inequality. We experimentally illustrate this using a multi-level trapped \Yb ion that allows simulation of anti-unitary operations.

Although nonequilibrium work and fluctuation relations have been studied in detail within classical statistical physics, extending these results to open quantum systems has proven to be conceptually difficult. For systems that undergo decoherence but not dissipation, we argue that it is natural to define quantum work exactly as for isolated quantum systems, using the two-point measurement protocol. Complementing previous theoretical analysis using quantum channels, we show that the nonequilibrium work relation remains valid in this situation, and we test this assertion experimentally using a system engineered from an optically trapped ion. Our experimental results reveal the work relation's validity over a variety of driving speeds, decoherence rates, and effective temperatures and represent the first confirmation of the work relation for non-unitary dynamics.

Quantum field theories describe a wide variety of fundamental phenomena in physics. However, their study often involves cumbersome numerical simulations. Quantum simulators, on the other hand, may outperform classical computational capacities due to their potential scalability. Here, we report an experimental realization of a quantum simulation of fermion-antifermion scattering mediated by bosonic modes, using a multilevel trapped ion, which is a simplified model of fermion scattering in both perturbative and nonperturbative quantum electrodynamics. The simulated model exhibits prototypical features in quantum field theory including particle pair creation and annihilation, as well as self-energy interactions. These are experimentally observed by manipulating four internal levels of a $^{171}\mathrm{Yb}^{+}$ trapped ion, where we encode the fermionic modes, and two motional degrees of freedom that simulate the bosonic modes. Our experiment establishes an avenue towards the efficient implementation of fermionic and bosonic quantum field modes, which may prove useful in scalable studies of quantum field theories in perturbative and nonperturbative regimes.

Spontaneous symmetry breaking is a universal concept throughout science. For instance, the Landau-Ginzburg paradigm of translational symmetry breaking underlies the classification of nearly all quantum phases of matter and explains the emergence of crystals, insulators, and superconductors. Usually, the consequences of translational invariance are studied in large systems to suppress edge effects which cause undesired symmetry breaking. While this approach works for investigating global properties, studies of local observables and their correlations require access and control of the individual constituents. Periodic boundary conditions, on the other hand, could allow for translational symmetry in small systems where single particle control is achievable. Here, we crystallize up to fifteen 40Ca+ ions in a microscopic ring with inherent periodic boundary conditions. We show the ring's translational symmetry is preserved at millikelvin temperatures by delocalizing the Doppler laser cooled ions. This establishes an upper bound for undesired symmetry breaking at a level where quantum control becomes feasible. These findings pave the way towards studying quantum many-body physics with translational symmetry at the single particle level in a variety of disciplines from simulation of Hawking radiation to exploration of quantum phase transitions.

In classical computational chemistry, the coupled-cluster ansatz is one of the most commonly used $ab~initio$ methods, which is critically limited by its non-unitary nature. The unitary modification as an ideal solution to the problem is, however, extremely inefficient in classical conventional computation. Here, we provide the first experimental evidence that indeed the unitary version of the coupled cluster ansatz can be reliably performed in physical quantum system, a trapped ion system. We perform a simulation on the electronic structure of a molecular ion (HeH$^+$), where the ground-state energy surface curve is probed, energies of excited-states are studied and the bond-dissociation is simulated non-perturbatively. Our simulation takes advantages from quantum computation to overcome the intrinsic limitations in classical computation and our experimental results indicate that the method is promising for preparing molecular ground-states for quantum simulation.

We present a design of an r.f. trap using planar electrodes with the goal to trap on the order of 100 ions in a small ring structure of diameters ranging between 100 $μ$m and 200 $μ$m. In order to minimize the influence of trap electrode imperfections due to the fabrication, we aim at trapping the ions around 400 $μ$m above the trap electrodes. In view of experiments to create freely rotating crystals near the ground state, we numerically study factors breaking the rotational symmetry such as external stray electric fields, local charging of the trap electrodes, and fabrication imperfections. We conclude that these imperfections can be controlled sufficiently well under state-of-the-art experimental conditions to allow for freely rotating ion rings even at energies comparable to the ground state energy of the rotational degree-of-freedom.

The understanding of symmetry operations has brought enormous advancements in physics, ranging from elementary particle to condensed matter systems. In quantum mechanics, symmetry operations are described by either unitary or antiunitary operators, where the latter are unphysical transformations that cannot be realized in physical systems. So far, quantum simulators of unitary and dissipative processes, the only allowed physical dynamics, have been realized in key experiments. Here, we present an embedding quantum simulator able to encode unphysical operations in a multilevel single trapped ion. In this sense, we experimentally observe phenomena associated with the nonunitary Majorana dynamics and implement antiunitary symmetry operations, i.e., time reversal and charge conjugation, at arbitrary evolution times. These experiments enhance the toolbox of quantum simulations towards applications involving unphysical operations.

We report the first experimental realization of the geometric Landau-Zener-Stückelberg (LZS) interferometry proposed by [Phys. Rev. Lett. 107, 207002 (2011)] in a single trapped ion system. Different from a conventional LZS interferometer, the interference fringes of our geometric interferometer originate solely from geometric phase. We also observe the robustness of the interference contrast against noise or fluctuation in the experimental parameters. Our scheme can be applied to other complex systems subject to relatively large errors in system control.

This is a reply to the comment from Patrick Bruno (arXiv:1211.4792) on our paper (Phys. Rev. Lett. 109, 163001 (2012)).

We experimentally observed state-independent violations of Kochen-Specker inequalities for the simplest indivisible quantum system manifesting quantum contextuality, a three-level (qutrit) system. We performed the experiment with a single trapped ^{171}Yb^{+} ion, by mapping three ground states of the ^{171}Yb^{+} ion to a qutrit system and carrying out quantum operatations by applying microwaves resonant to the qutrit transition frequencies. Our results are free from the detection loophole and cannot be explained by the non-contextual hidden variable models.

Spontaneous symmetry breaking can lead to the formation of time crystals, as well as spatial crystals. Here we propose a space-time crystal of trapped ions and a method to realize it experimentally by confining ions in a ring-shaped trapping potential with a static magnetic field. The ions spontaneously form a spatial ring crystal due to Coulomb repulsion. This ion crystal can rotate persistently at the lowest quantum energy state in magnetic fields with fractional fluxes. The persistent rotation of trapped ions produces the temporal order, leading to the formation of a space-time crystal. We show that these space-time crystals are robust for direct experimental observation. We also study the effects of finite temperatures on the persistent rotation. The proposed space-time crystals of trapped ions provide a new dimension for exploring many-body physics and emerging properties of matter.