T. R. Tan

The realisation of a universal quantum computer at scale promises to deliver a paradigm shift in information processing, providing the capability to solve problems that are intractable with conventional computers. A key limiting factor of realising fault-tolerant quantum information processing (QIP) is the large ratio of physical-to-logical qubits that outstrip device sizes available in the near future. An alternative approach proposed by Gottesman, Kitaev, and Preskill (GKP) encodes a single logical qubit into a single harmonic oscillator, alleviating this hardware overhead in exchange for a more complex encoding. Owing to this complexity, current experiments with GKP codes have been limited to single-qubit encodings and operations. Here, we report on the experimental demonstration of a universal gate set for the GKP code, which includes single-qubit gates and -- for the first time -- a two-qubit entangling gate between logical code words. Our scheme deterministically implements energy-preserving quantum gates on finite-energy GKP states encoded in the mechanical motion of a trapped ion. This is achieved by a novel optimal control strategy that dynamically modulates an interaction between the ion's spin and motion. We demonstrate single-qubit gates with a logical process fidelity as high as 0.960 and a two-qubit entangling gate with a logical process fidelity of 0.680. We also directly create a GKP Bell state from the oscillators' ground states in a single step with a logical state fidelity of 0.842. The overall scheme is compatible with existing hardware architectures, highlighting the opportunity to leverage optimal control strategies as a key accelerant towards fault tolerance.

Accurate simulation of dynamical processes in molecules and reactions is among the most challenging problems in quantum chemistry. Quantum computers promise efficient chemical simulation, but the existing quantum algorithms require many logical qubits and gates, placing practical applications beyond existing technology. Here, we carry out the first quantum simulations of chemical dynamics by employing a more hardware-efficient encoding scheme that uses both qubits and bosonic degrees of freedom. Our trapped-ion device accurately simulates the dynamics of non-adiabatic chemical processes, which are among the most difficult problems in computational chemistry because they involve strong coupling between electronic and nuclear motions. We demonstrate the programmability and versatility of our approach by simulating the dynamics of three different molecules as well as open-system dynamics in the condensed phase, all with the same quantum resources. Our approach requires orders of magnitude fewer resources than equivalent qubit-only quantum simulations, demonstrating the potential of using hybrid encoding schemes to accelerate quantum simulations of complex chemical processes, which could have applications in fields ranging from energy conversion and storage to biology and drug design.

Interactions of molecules with their environment influence the course and outcome of almost all chemical reactions. However, classical computers struggle to accurately simulate complicated molecule-environment interactions because of the steep growth of computational resources with both molecule size and environment complexity. Therefore, many quantum-chemical simulations are restricted to isolated molecules, whose dynamics can dramatically differ from what happens in an environment. Here, we show that analog quantum simulators can simulate open molecular systems by using the native dissipation of the simulator and injecting additional controllable dissipation. By exploiting the native dissipation to simulate the molecular dissipation -- rather than seeing it as a limitation -- our approach enables longer simulations of open systems than are possible for closed systems. In particular, we show that trapped-ion simulators using a mixed qudit-boson (MQB) encoding could simulate molecules in a wide range of condensed phases by implementing widely used dissipative processes within the Lindblad formalism, including pure dephasing and both electronic and vibrational relaxation. The MQB open-system simulations require significantly fewer additional quantum resources compared to both classical and digital quantum approaches.

Encoding logical qubits in bosonic modes provides a potentially hardware-efficient implementation of fault-tolerant quantum information processing. Here, we demonstrate high-fidelity and deterministic preparation of highly non-classical bosonic states in the mechanical motion of a trapped ion. Our approach implements error-suppressing pulses through optimized dynamical modulation of laser-driven spin-motion interactions to generate the target state in a single step. We demonstrate logical fidelities for the Gottesman-Kitaev-Preskill (GKP) state as high as $\bar{\mathcal{F}}=0.940(8)$, a distance-3 binomial state with an average fidelity of $\mathcal{F}=0.807(7)$, and a 12.91(5) dB squeezed vacuum state.

Qubits encoded in hyperfine states of trapped ions are ideal for quantum computation given their long lifetimes and low sensitivity to magnetic fields, yet they suffer from off-resonant scattering during detection often limiting their measurement fidelity. In ${}^{171}$Yb$^{+}$ this is exacerbated by a low fluorescence yield, which leads to a need for complex and expensive hardware - a problematic bottleneck especially when scaling up the number of qubits. We demonstrate a detection routine based on electron shelving to address this issue in ${}^{171}$Yb$^{+}$ and achieve a 5.6$\times$ reduction in single-ion detection error on an avalanche photodiode to $1.8(2)\times10^{-3}$ in a 100 $μ$s detection period, and a 4.3$\times$ error reduction on an electron multiplying CCD camera, with $7.7(2)\times10^{-3}$ error in 400 $μ$s. We further improve the characterization of a repump transition at 760 nm to enable a more rapid reset of the auxiliary $^2$F$_{7/2}$ states populated after shelving. Finally, we examine the detection fidelity limit using the long-lived $^2$F$_{7/2}$ state, achieving a further 300$\times$ and 12$\times$ reduction in error to $6(7)\times10^{-6}$ and $6.3(3)\times10^{-4}$ in 1 ms on the respective detectors. While shelving-rate limited in our setup, we suggest various techniques to realize this detection method at speeds compatible with quantum information processing, providing a pathway to ultra-high fidelity detection in ${}^{171}$Yb$^{+}$.

Scaling quantum information processors is a challenging task, requiring manipulation of a large number of qubits with high fidelity and a high degree of connectivity. For trapped ions, this could be realized in a two-dimensional array of interconnected traps in which ions are separated, transported and recombined to carry out quantum operations on small subsets of ions. Here, we use a junction connecting orthogonal linear segments in a two-dimensional (2D) trap array to reorder a two-ion crystal. The secular motion of the ions experiences low energy gain and the internal qubit levels maintain coherence during the reordering process, therefore demonstrating a promising method for providing all-to-all connectivity in a large-scale, two- or three-dimensional trapped-ion quantum information processor.

Entangled states are a crucial resource for quantum-based technologies such as quantum computers and quantum communication systems (1,2). Exploring new methods for entanglement generation is important for diversifying and eventually improving current approaches. Here, we create entanglement in atomic ions by applying laser fields to constrain the evolution to a restricted number of states, in an approach that has become known as "quantum Zeno dynamics" (3-5). With two trapped $^9\rm{Be}^+$ ions, we obtain Bell state fidelities up to $0.990^{+2}_{-5}$, with three ions, a W-state (6) fidelity of $0.910^{+4}_{-7}$ is obtained. Compared to other methods of producing entanglement in trapped ions, this procedure is relatively insensitive to certain imperfections such as fluctuations in laser intensity, laser frequency, and ion-motion frequencies.

Precision control over hybrid physical systems at the quantum level is important for the realization of many quantum-based technologies. In the field of quantum information processing (QIP) and quantum networking, various proposals discuss the possibility of hybrid architectures where specific tasks are delegated to the most suitable subsystem. For example, in quantum networks, it may be advantageous to transfer information from a subsystem that has good memory properties to another subsystem that is more efficient at transporting information between nodes in the network. For trapped-ions, a hybrid system formed of different species introduces extra degrees of freedom that can be exploited to expand and refine the control of the system. Ions of different elements have previously been used in QIP experiments for sympathetic cooling, creation of entanglement through dissipation, and quantum non-demolition (QND) measurement of one species with another. Here, we demonstrate an entangling quantum gate between ions of different elements which can serve as an important building block of QIP, quantum networking, precision spectroscopy, metrology, and quantum simulation. A geometric phase gate between a $^9$Be$^+$ ion and a $^{25}$Mg$^+$ ion is realized through an effective spin-spin interaction generated by state-dependent forces induced with laser beams. Combined with single-qubit gates and same-species entangling gates, this mixed-element entangling gate provides a complete set of gates over such a hybrid system for universal QIP. Using a sequence of such gates, we demonstrate a Controlled-NOT (CNOT) gate and a SWAP gate. We further demonstrate the robustness of these gates against thermal excitation and show improved detection in quantum logic spectroscopy (QLS). We also observe a strong violation of a CHSH-type Bell inequality on entangled states composed of different ion species.

Entangled states are a key resource in fundamental quantum physics, quantum cryp-tography, and quantum computation [1].To date, controlled unitary interactions applied to a quantum system, so-called "quantum gates", have been the most widely used method to deterministically create entanglement [2]. These processes require high-fidelity state preparation as well as minimizing the decoherence that inevitably arises from coupling between the system and the environment and imperfect control of the system parameters. Here, on the contrary, we combine unitary processes with engineered dissipation to deterministically produce and stabilize an approximate Bell state of two trapped-ion qubits independent of their initial state. While previous works along this line involved the application of sequences of multiple time-dependent gates [3] or generated entanglement of atomic ensembles dissipatively but relied on a measurement record for steady-state entanglement [4], we implement the process in a continuous time-independent fashion, analogous to optical pumping of atomic states. By continuously driving the system towards steady-state, the entanglement is stabilized even in the presence of experimental noise and decoherence. Our demonstration of an entangled steady state of two qubits represents a step towards dissipative state engineering, dissipative quantum computation, and dissipative phase transitions [5-7]. Following this approach, engineered coupling to the environment may be applied to a broad range of experimental systems to achieve desired quantum dynamics or steady states. Indeed, concurrently with this work, an entangled steady state of two superconducting qubits was demonstrated using dissipation [8].

We demonstrate a trapped-ion entangling-gate scheme proposed by Bermudez et al. [Phys. Rev. A 85, 040302 (2012)]. Simultaneous excitation of a strong carrier and a single-sideband transition enables deterministic creation of entangled states. The method works for magnetic field-insensitive states, is robust against thermal excitations, includes dynamical decoupling from qubit dephasing errors, and provides simplifications in experimental implementation compared to some other entangling gates with trapped ions. We achieve a Bell state fidelity of 0.974(4) and identify the main sources of error.

We investigate the motional dynamics of single and multiple ions during transport between and separation into spatially distinct locations in a multi-zone linear Paul trap. A single 9Be+ ion in a 2 MHz harmonic well located in one zone was laser-cooled to near its ground state of motion and transported 370 micrometers by moving the well to another zone. This was accomplished in 8 microseconds, corresponding to 16 periods of oscillation. Starting from a state with n=0.1 quanta, during transport the ion was excited to a displaced coherent state with n=1.6 quanta but on completion was returned close to its motional ground state with n=0.2. Similar results were achieved for the transport of two ions. We also separated chains of up to 9 ions from one potential well to two distinct potential wells. With two ions this was accomplished in 55 microseconds, with final excitations of about 2 quanta for each ion. Fast coherent transport and separation can significantly reduce the time overhead in certain architectures for scalable quantum information processing with trapped ions.

As experimental platforms for quantum information processing continue to mature, characterization of the quality of unitary gates that can be applied to their quantum bits (qubits) becomes essential. Eventually, the quality must be sufficiently high to support arbitrarily long quantum computations. Randomized benchmarking already provides a platform-independent method for assessing the quality of one-qubit rotations. Here we describe an extension of this method to multi-qubit gates. We provide a platform-independent protocol for evaluating the performance of experimental Clifford unitaries, which form the basis of fault-tolerant quantum computing. We implemented the benchmarking protocol with trapped-ion two-qubit phase gates and one-qubit gates and found an error per random two-qubit Clifford unitary of $0.162 \pm 0.008$, thus setting the first benchmark for such unitaries. By implementing a second set of sequences with an extra two-qubit phase gate at each step, we extracted an error per phase gate of $0.069 \pm 0.017$. We conducted these experiments with movable, sympathetically cooled ions in a multi-zone Paul trap - a system that can in principle be scaled to larger numbers of ions.