J. P. Home

We demonstrate a trapped-ion system with two competing dissipation channels, implemented independently on two ion species co-trapped in a Paul trap. By controlling coherent spin-oscillator couplings and optical pumping rates we explore the phase diagram of this system, which exhibits a regime analogous to that of a (phonon) laser but operates close to the quantum ground state with an average phonon number of $\bar{n}<10$. We demonstrate phase locking of the oscillator to an additional resonant drive, and also observe the phase diffusion of the resulting state under dissipation by reconstructing the quantum state from a measurement of the characteristic function.

We demonstrate co-trapping and sideband cooling of a H$_2^+$ - $^9$Be$^+$ ion pair in a cryogenic Paul trap. We study the chemical lifetime of H$_2^+$ and its dependence on the apparatus temperature, achieving lifetimes of up to $11^{+6}_{-3}$ h at 10 K. We demonstrate cooling of two of the modes of translational motion to an average phonon number of 0.07(1) and 0.05(1), corresponding to a temperature of 22(1) $μ$K and 55(3) $μ$K respectively. Our results provide a basis for quantum logic spectroscopy experiments of H$_2^+$, as well as other light ions such as HD$^+$, H$_3^+$, and He$^+$.

We propose and implement a novel scheme for dissipatively pumping two qubits into a singlet Bell state. The method relies on a process of collective optical pumping to an excited level, to which all states apart from the singlet are coupled. We apply the method to deterministically entangle two trapped ${}^{40}\text{Ca}^+$ ions with a fidelity of $93(1)\%$. We theoretically analyze the performance and error susceptibility of the scheme and find it to be insensitive to a large class of experimentally relevant noise sources.

We employ a trapped ion to study quantum contextual correlations in a single qutrit using the 5-observable KCBS inequality, which is arguably the most fundamental non-contextuality inequality for testing Quantum Mechanics (QM). We quantify the effect of systematics in our experiment by purposely scanning the degree of signaling between measurements, which allows us to place realistic bounds on the non-classicality of the observed correlations. Our results violate the classical bound for this experiment by up to 25 standard deviations, while being in agreement with the QM limit. In order to test the prediction of QM that the contextual fraction increases with the number of observables, we gradually increase the complexity of our measurements from 5 up to 121 observables. We find stronger-than-classical correlations in all prepared scenarios up to 101 observables, beyond which experimental imperfections blur the quantum-classical divide.

The non-commutativity of position and momentum observables is a hallmark feature of quantum physics. However this incompatibility does not extend to observables which are periodic in these base variables. Such modular-variable observables have been suggested as tools for fault-tolerant quantum computing and enhanced quantum sensing. Here we implement sequential measurements of modular variables in the oscillatory motion of a single trapped ion, using state-dependent displacements and a heralded non-destructive readout. We investigate the commutative nature of modular variable observables by demonstrating no-signaling-in-time between successive measurements, using a variety of input states. In the presence of quantum interference, which we enhance using squeezed input states, measurements of different periodicity show signaling-in-time. The sequential measurements allow us to extract two-time correlators for modular variables, which we use to violate a Leggett-Garg inequality. The experiments involve control and coherence of multi-component superpositions of up to 8 coherent, squeezed or Fock state wave-packets. Signaling-in-time as well as Leggett-Garg inequalities serve as efficient quantum witnesses which we probe here with a mechanical oscillator, a system which has a natural crossover from the quantum to the classical regime.

We use a single trapped-ion qutrit to demonstrate the violation of an input-state-independent non-contextuality inequality using a sequence of randomly chosen quantum non-demolition projective measurements. We concatenate 54 million sequential measurements of 13 observables, and violate an optimal non-contextual bound by 214 standard deviations. We use the same dataset to characterize imperfections including signaling and repeatability of the measurements. The experimental sequence was generated in real time with a quantum random number generator integrated into our control system to select the subsequent observable with a latency below 50 μs, which can be used to constrain hidden-variable models that might describe our results. The state-recycling experimental procedure is resilient to noise, self-correcting and independent of the qutrit state, substantiating the fact that quantumness is connected to measurements as opposed to designated states.

We demonstrate control of a trapped-ion quantum harmonic oscillator in a squeezed Fock state basis, using engineered Hamiltonians analogous to the Jaynes-Cummings and anti-Jaynes-Cummings forms. We demonstrate that for squeezed Fock states with low $n$ the engineered Hamiltonians reproduce the $\sqrt{n}$ scaling of the matrix elements which is typical of Jaynes-Cummings physics, and also examine deviations due to the finite wavelength of our control fields. Starting from a squeezed vacuum state, we apply sequences of alternating transfer pulses which allow us to climb the squeezed Fock state ladder, creating states up to excitations of $n = 6$ with up to 8.7 dB of squeezing, as well as demonstrating superpositions of these states. These techniques offer access to new sets of states of the harmonic oscillator which may be applicable for precision metrology or quantum information science.

We demonstrate the ability to load, cool and detect singly-charged calcium ions in a surface electrode trap using only visible and infrared lasers for the trapped-ion control. As opposed to the standard methods of cooling using dipole-allowed transitions, we combine power broadening of a quadrupole transition at 729 nm with quenching of the upper level using a dipole allowed transition at 854 nm. By observing the resulting 393 nm fluorescence we are able to perform background-free detection of the ion. We show that this system can be used to smoothly transition between the Doppler cooling and sideband cooling regimes, and verify theoretical predictions throughout this range. We achieve scattering rates which reliably allow recooling after collision events and allow ions to be loaded from a thermal atomic beam. This work is compatible with recent advances in optical waveguides, and thus opens a path in current technologies for large-scale quantum information processing. In situations where dielectric materials are placed close to trapped ions, it carries the additional advantage of using wavelengths which do not lead to significant charging, which should facilitate high rate optical interfaces between remotely held ions.

The ability of matter to be superposed at two different locations while being intrinsically connected by a quantum phase is among the most counterintuitive predictions of quantum physics. While such superpositions have been created for a variety of systems, the in-situ observation of the phase coherence has remained out of reach. Using a heralding measurement on a spin-oscillator entangled state, we project a mechanical trapped-ion oscillator into a superposition of two spatially separated states, a situation analogous to Schrödinger's cat. Quantum interference is clearly observed by extracting the occupations of the energy levels. For larger states, we encounter problems in measuring the energy distribution, which we overcome by performing the analogous measurement in a squeezed Fock basis with each basis element stretched along the separation axis. Using 8 dB of squeezing we observe quantum interference for cat states with phase space separations of $Δα= 15.6$, corresponding to wavepackets with a root-mean-square extent of 7.8 nm separated by over 240 nm. We also introduce a method for reconstructing the Wigner phase-space quasi-probability distribution using both squeezed and non-squeezed Fock bases. We apply this to a range of negative parity cats, observing the expected interference fringes and negative values at the center of phase space. Alongside the fundamental nature of these large state superpositions, our reconstruction methods facilitate access to the large Hilbert spaces required to work with mesoscopic quantum superpositions, and may be realized in a wide range of experimental platforms.

The time evolution of a closed quantum system is connected to its Hamiltonian through Schroedinger's equation. The ability to estimate the Hamiltonian is critical to our understanding of quantum systems, and allows optimization of control. Though spectroscopic methods allow time-independent Hamiltonians to be recovered, for time-dependent Hamiltonians this task is more challenging. Here, using a single trapped ion, we experimentally demonstrate a method for estimating a time-dependent Hamiltonian of a single qubit. The method involves measuring the time evolution of the qubit in a fixed basis as a function of a time-independent offset term added to the Hamiltonian. In our system the initially unknown Hamiltonian arises from transporting an ion through a static, near-resonant laser beam. Hamiltonian estimation allows us to estimate the spatial dependence of the laser beam intensity and the ion's velocity as a function of time. This work is of direct value in optimizing transport operations and transport-based gates in scalable trapped ion quantum information processing, while the estimation technique is general enough that it can be applied to other quantum systems, aiding the pursuit of high operational fidelities in quantum control.

Fast control of quantum systems is essential in order to make use of quantum properties before they are degraded by decoherence. This is important for quantum-enhanced information processing, as well as for pushing quantum systems into macroscopic regimes at the boundary between quantum and classical physics. Bang-bang control attains the ultimate speed limit by making large changes to control fields on timescales much faster than the system can respond, however these methods are often challenging to implement experimentally. Here we demonstrate bang-bang control of a trapped-ion oscillator using nano-second switching of the trapping potentials. We perform controlled displacements which allow us to realize quantum states with up to 10,000 quanta of energy. We use these displaced states to verify the form of the ion-light interaction at high excitations which are far outside the usual regime of operation. These methods provide new possibilities for quantum-state manipulation and generation, alongside the potential for a significant increase in operational clock speed for ion-trap quantum information processing.

Entanglement is one of the most fundamental properties of quantum mechanics, and is the key resource for quantum information processing. Bipartite entangled states of identical particles have been generated and studied in several experiments, and post-selected or heralded entangled states involving pairs of photons, single photons and single atoms, or different nuclei in the solid state, have also been produced. Here, we use a deterministic quantum logic gate to generate a "hybrid" entangled state of two trapped-ion qubits held in different isotopes of calcium, perform full tomography of the state produced, and make a test of Bell's inequality with non-identical atoms. We use a laser-driven two-qubit gate, whose mechanism is insensitive to the qubits' energy splittings, to produce a maximally-entangled state of one Ca-40 qubit and one Ca-43 qubit, held 3.5 microns apart in the same ion trap, with 99.8(6)% fidelity. We test the Clauser-Horne-Shimony-Holt (CHSH) version of Bell's inequality for this novel entangled state and find that it is violated by 15 standard deviations; in this test, we close the detection loophole but not the locality loophole. Mixed-species quantum logic is a powerful technique for the construction of a quantum computer based on trapped ions, as it allows protection of memory qubits while other qubits undergo logic operations, or are used as photonic interfaces to other processing units. The entangling gate mechanism used here can also be applied to qubits stored in different atomic elements; this would allow both memory and logic gate errors due to photon scattering to be reduced below the levels required for fault-tolerant quantum error correction, which is an essential pre-requisite for general-purpose quantum computing.

We investigate the dynamics under diabatic expansions/compressions of linear ion chains.Combining a dynamical normal-mode harmonic approximation with the invariant-based inverse-engineering technique, we design protocols that minimize the final motional excitation of the ions. This can substantially reduce the transition time between high and low trap-frequency operations, potentially contributing to the development of scalable quantum information processing.

We demonstrate a surface-electrode ion trap fabricated using techniques transferred from the manufacture of photonic-crystal fibres. This provides a relatively straightforward route for realizing traps with an electrode structure on the 100 micron scale with high optical access. We demonstrate the basic functionality of the trap by cooling a single ion to the quantum ground state, allowing us to measure a heating rate from the ground state of 787(24) quanta/s. Variation of the fabrication procedure used here may provide access to traps in this geometry with trap scales between 100 um and 10 um.

The robust generation of quantum states in the presence of decoherence is a primary challenge for explorations of quantum mechanics at larger scales. Using the mechanical motion of a single trapped ion, we utilize reservoir engineering to generate squeezed, coherent and displaced-squeezed states as steady states in the presence of noise. We verify the created state by generating two-state correlated spin-motion Rabi oscillations resulting in high contrast measurements. For both cooling and measurement, we use spin-oscillator couplings that provide transitions between oscillator states in an engineered Fock state basis. Our approach should facilitate studies of entanglement, quantum computation, and open-system quantum simulations in a wide range of physical systems.

We investigate electrode geometries required to produce periodic 2-dimensional ion-trap arrays with the ions placed between two planes of electrodes. We present a generalization of previous methods for traps containing a single electrode plane to this new geometry, and show that for a given ion-electrode distance and applied voltages, the inter-ion distance can be reduced by a factor of up to 3 relative to single-plane traps. This represents an increase by a factor of 9 in the trap density and a factor of 27 in the exchange coupling between the oscillatory motion of neighboring ions. The resulting traps are also considerably deeper for bi-layer structures than for single-plane traps. These results could offer a useful path towards 2-dimensional ion arrays for quantum simulation. We also discuss issues with the fabrication of such traps.

We show how to create quantum gates of arbitrary speed between trapped ions, using a laser walking wave, with complete insensitivity to drift of the optical phase, and requiring cooling only to the Lamb-Dicke regime. We present pulse sequences that satisfy the requirements and are easy to produce in the laboratory.

We describe laser systems for photoionization, Doppler cooling and quantum state manipulation of beryllium ions. For photoionization of neutral beryllium, we have developed a continuous-wave 235 nm source obtained by two stages of frequency doubling from a diode laser at 940 nm. The system delivers up to 400 mW at 470 nm and 28 mW at 235 nm. For control of the beryllium ion, three laser wavelengths at 313 nm are produced by sum-frequency generation and second-harmonic generation from four infrared fiber lasers. Up to 7.2 W at 626 nm and 1.9 W at 313 nm are obtained using two pump beams at 1051 and 1551 nm. Intensity fluctuations below 0.5 % per hour (during 8 hours of operation) have been measured at a 313 nm power of 1 W. These systems are used to load beryllium ions into a segmented ion trap.

We propose a new scheme for supplying voltages to the electrodes of microfabricated ion traps, enabling access to a regime in which changes to the trapping potential are made on timescales much shorter than the period of the secular oscillation frequencies of the trapped ions. This opens up possibilities for speeding up the transport of ions in segmented ion traps and also provides access to control of multiple ions in a string faster than the Coulomb interaction between them. We perform a theoretical study of ion transport using these methods in a surface-electrode trap, characterizing the precision required for a number of important control parameters. We also consider the possibilities and limitations for generating motional state squeezing using these techniques, which could be used as a basis for investigations of Gaussian-state entanglement.

We investigate the motional dynamics of single and multiple ions during transport between and separation into spatially distinct locations in a multi-zone linear Paul trap. A single 9Be+ ion in a 2 MHz harmonic well located in one zone was laser-cooled to near its ground state of motion and transported 370 micrometers by moving the well to another zone. This was accomplished in 8 microseconds, corresponding to 16 periods of oscillation. Starting from a state with n=0.1 quanta, during transport the ion was excited to a displaced coherent state with n=1.6 quanta but on completion was returned close to its motional ground state with n=0.2. Similar results were achieved for the transport of two ions. We also separated chains of up to 9 ions from one potential well to two distinct potential wells. With two ions this was accomplished in 55 microseconds, with final excitations of about 2 quanta for each ion. Fast coherent transport and separation can significantly reduce the time overhead in certain architectures for scalable quantum information processing with trapped ions.

As experimental platforms for quantum information processing continue to mature, characterization of the quality of unitary gates that can be applied to their quantum bits (qubits) becomes essential. Eventually, the quality must be sufficiently high to support arbitrarily long quantum computations. Randomized benchmarking already provides a platform-independent method for assessing the quality of one-qubit rotations. Here we describe an extension of this method to multi-qubit gates. We provide a platform-independent protocol for evaluating the performance of experimental Clifford unitaries, which form the basis of fault-tolerant quantum computing. We implemented the benchmarking protocol with trapped-ion two-qubit phase gates and one-qubit gates and found an error per random two-qubit Clifford unitary of $0.162 \pm 0.008$, thus setting the first benchmark for such unitaries. By implementing a second set of sequences with an extra two-qubit phase gate at each step, we extracted an error per phase gate of $0.069 \pm 0.017$. We conducted these experiments with movable, sympathetically cooled ions in a multi-zone Paul trap - a system that can in principle be scaled to larger numbers of ions.

We theoretically and experimentally examine the effects of anharmonic terms in the trapping potential for linear chains of trapped ions. We concentrate on two different effects that become significant at different levels of anharmonicity. The first is a modification of the oscillation frequencies and amplitudes of the ions' normal modes of vibration for multi-ion crystals, resulting from each ion experiencing a different curvature in the potential. In the second effect, which occurs with increased anharmonicity or higher excitation amplitude, amplitude-dependent shifts of the normal-mode frequencies become important. We evaluate normal-mode frequency and amplitude shifts, and comment on the implications for quantum information processing and quantum state engineering. Since the ratio of the anharmonic to harmonic terms typically increases as the ion--electrode distance decreases, anharmonic effects will become more significant as ion trap sizes are reduced. To avoid unwanted problems, anharmonicities should therefore be taken into account at the design stage of trap development.

The universal quantum computer is a device capable of simulating any physical system and represents a major goal for the field of quantum information science. Algorithms performed on such a device are predicted to offer significant gains for some important computational tasks. In the context of quantum information, "universal" refers to the ability to perform arbitrary unitary transformations in the system's computational space. The combination of arbitrary single-quantum-bit (qubit) gates with an entangling two-qubit gate is a gate set capable of achieving universal control of any number of qubits, provided that these gates can be performed repeatedly and between arbitrary pairs of qubits. Although gate sets have been demonstrated in several technologies, they have as yet been tailored toward specific tasks, forming a small subset of all unitary operators. Here we demonstrate a programmable quantum processor that realises arbitrary unitary transformations on two qubits, which are stored in trapped atomic ions. Using quantum state and process tomography, we characterise the fidelity of our implementation for 160 randomly chosen operations. This universal control is equivalent to simulating any pairwise interaction between spin-1/2 systems. A programmable multi-qubit register could form a core component of a large-scale quantum processor, and the methods used here are suitable for such a device.

Large-scale quantum information processors must be able to transport and maintain quantum information, and repeatedly perform logical operations. Here we demonstrate a combination of all the fundamental elements required to perform scalable quantum computing using qubits stored in the internal states of trapped atomic ions. We quantify the repeatability of a multi-qubit operation, observing no loss of performance despite qubit transport over macroscopic distances. Key to these results is the use of different pairs of beryllium ion hyperfine states for robust qubit storage, readout and gates, and simultaneous trapping of magnesium re-cooling ions along with the qubit ions.

We demonstrate sympathetic cooling of a 43Ca+ trapped-ion "memory" qubit by a 40Ca+ "coolant" ion near the ground state of both axial motional modes, whilst maintaining coherence of the qubit. This is an essential ingredient in trapped-ion quantum computers. The isotope shifts are sufficient to suppress decoherence and phase shifts of the memory qubit due to the cooling light which illuminates both ions. We measure the qubit coherence during 10 cycles of sideband cooling, finding a coherence loss of 3.3% per cooling cycle. The natural limit of the method is O(0.01%) infidelity per cooling cycle.

We demonstrate long-lived coherence in internal hyperfine states of a single \Ca{43} trapped-ion qubit $[T_2=1.2(2)\s]$, and in external motional states of a single \Ca{40} trapped-ion qubit $[T_2'=0.18(4)\s]$, in the same apparatus. The motional decoherence rate is consistent with the heating rate, which was measured to be 3(1) quanta/sec. Long coherence times in the external motional states are essential for performing high-fidelity quantum logic gates between trapped-ion qubits. The internal-state $T_2$ time that we observe in \Ca{43}, which has not previously been used as a trapped-ion qubit, is about one thousand times longer than that of physical qubits based on \Ca{40} ions. Using a single spin-echo pulse to ``re-phase'' the internal state, we can detect no decoherence after 1\s, implying an effective coherence time $T_2^{\mbox{\tiny SE}} \gtish 45\s$. This compares with timescales in this trap for single-qubit operations of \ish 1\us, and for two-qubit operations of \ish 10\us.

We have measured motional heating rates of trapped atomic ions, a factor that can influence multi-ion quantum logic gate fidelities. Two simplified techniques were developed for this purpose: one relies on Raman sideband detection implemented with a single laser source, while the second is even simpler and is based on time-resolved fluorescence detection during Doppler recooling. We applied these methods to determine heating rates in a microfrabricated surface-electrode trap made of gold on fused quartz, which traps ions 40 microns above its surface. Heating rates obtained from the two techniques were found to be in reasonable agreement. In addition, the trap gives rise to a heating rate of 300 plus or minus 30 per second for a motional frequency of 5.25 MHz, substantially below the trend observed in other traps.

We investigate the temporal dynamics of Doppler cooling of an initially hot single trapped atom in the weak binding regime using a semiclassical approach. We develop an analytical model for the simplest case of a single vibrational mode for a harmonic trap, and show how this model allows us to estimate the initial energy of the trapped particle by observing the fluorescence rate during the cooling process. The experimental implementation of this temperature measurement provides a way to measure atom heating rates by observing the temperature rise in the absence of cooling. This method is technically relatively simple compared to conventional sideband detection methods, and the two methods are in reasonable agreement. We also discuss the effects of RF micromotion, relevant for a trapped atomic ion, and the effect of coupling between the vibrational modes on the cooling dynamics.

We create entangled states of the spin and motion of a single $^{40}$Ca$^+$ ion in a linear ion trap. The motional part consists of coherent states of large separation and long coherence time. The states are created by driving the motion using counterpropagating laser beams. We theoretically study and experimentally observe the behaviour outside the Lamb-Dicke regime, where the trajectory in phase space is modified and the coherent states become squeezed. We directly observe the modification of the return time of the trajectory, and infer the squeezing. The mesoscopic entanglement is observed up to $Δα= 5.1$ with coherence time 170 microseconds and mean phonon excitation $\nbar = 16$.

We have implemented a universal quantum logic gate between qubits stored in the spin state of a pair of trapped calcium 40 ions. An initial product state was driven to a maximally entangled state deterministically, with 83% fidelity. We present a general approach to quantum state tomography which achieves good robustness to experimental noise and drift, and use it to measure the spin state of the ions. We find the entanglement of formation is 0.54.

We study the problem of designing electrode structures that allow pairs of ions to be brought together and separated rapidly in an array of linear Paul traps. We show that it is desirable for the electrode structure to produce a d.c. octupole moment with an a.c. radial quadrupole. For the case where electrical breakdown limits the voltages that can be applied, we show that the octupole is more demanding than the quadrupole when the characteristic distance scale of the structure is larger than 1 to 10 microns (for typical materials). We present a variety of approaches and optimizations of structures consisting of one to three layers of electrodes. The three-layer structures allow the fastest operation at given distance r from the trap centres to the nearest electrode surface, but when the total thickness w of the structure is constrained, leading to w < r, then two-layer structures may be preferable.

We present studies of resonance-enhanced photo-ionization for isotope-selective loading of Ca+ into a Paul trap. The 4s^2 ^1S_0 <-> 4s4p ^1P_1 transition of neutral calcium is driven by a 423nm laser and the atoms are photo-ionized by a second laser at 389nm. Isotope-selectivity is achieved by using crossed atomic and laser beams to reduce the Doppler width significantly below the isotope shifts in the 423nm transition. The loading rate of ions into the trap is studied under a range of experimental parameters for the abundant isotope 40Ca+. Using the fluorescence of the atomic beam at 423nm as a measure of the Ca number density, we estimate a lower limit for the absolute photo-ionization cross-section. We achieve loading and laser-cooling of all the naturally occurring isotopes, without the need for enriched sources. Laser-heating/cooling is observed to enhance the isotope-selectivity. In the case of the rare species 43Ca+ and 46Ca+, which have not previously been laser-cooled, the loading is not fully isotope-selective but we show that pure crystals of 43Ca+ may nevertheless be obtained. We find that for loading 40Ca+ the 389nm laser may be replaced by an incoherent source.