J. J. Bollinger

We show experimentally that a broad class of interactions involving quantum harmonic oscillators can be made stronger (amplified) using a unitary squeezing protocol. While our demonstration uses the motional and spin states of a single trapped $^{25}$Mg$^{+}$ ion, the scheme applies generally to Hamiltonians involving just a single harmonic oscillator as well as Hamiltonians coupling the oscillator to another quantum degree of freedom such as a qubit, covering a large range of systems of interest in quantum information and metrology applications. Importantly, the protocol does not require knowledge of the parameters of the Hamiltonian to be amplified, nor does it require a well-defined phase relationship between the squeezing interaction and the rest of the system dynamics, making it potentially useful in instances where certain aspects of a signal or interaction may be unknown or uncontrolled.

We theoretically study the dynamical phase diagram of the Dicke model in both classical and quantum limits using large, experimentally relevant system sizes. Our analysis elucidates that the model features dynamical critical points that are distinct from previously investigated excited-state equilibrium transitions. Moreover, our numerical calculations demonstrate that mean-field features of the dynamics remain valid in the exact quantum dynamics, but we also find that in regimes where quantum effects dominate signatures of the dynamical phases and chaos can persist in purely quantum metrics such as entanglement and correlations. Our predictions can be verified in current quantum simulators of the Dicke model including arrays of trapped ions.

Strong and precisely-controlled interactions between quantum objects are essential for quantum information processing, simulation, and sensing, and for the formation of exotic quantum matter. A well-established paradigm for coupling otherwise weakly-interacting quantum objects is to use auxiliary bosonic quantum excitations to mediate the interactions. Important examples include photon-mediated interactions between atoms, superconducting qubits, and color centers in diamond, and phonon-mediated interactions between trapped ions and between optical and microwave photons. Boson-mediated interactions can in principle be amplified through parametric driving of the boson channel; the drive need not couple directly to the interacting quantum objects. This technique has been proposed for a variety of quantum platforms, but has not to date been realized in the laboratory. Here we experimentally demonstrate the amplification of a boson-mediated interaction between two trapped-ion qubits by parametric modulation of the trapping potential. The amplification provides up to a 3.25-fold increase in the interaction strength, validated by measuring the speedup of two-qubit entangling gates. This amplification technique can be used in any quantum platform where parametric modulation of the boson channel is possible, enabling exploration of new parameter regimes and enhanced quantum information processing.

Trapped ions are sensitive detectors of weak forces and electric fields that excite ion motion. Here measurements of the center-of-mass motion of a trapped-ion crystal that are phase-coherent with an applied weak external force are reported. These experiments are conducted far from the trap motional frequency on a two-dimensional trapped-ion crystal of approximately 100 ions, and determine the fundamental measurement imprecision of our protocol free from noise associated with the center-of-mass mode. The driven sinusoidal displacement of the crystal is detected by coupling the ion crystal motion to the internal spin-degree of freedom of the ions using an oscillating spin-dependent optical dipole force. The resulting induced spin-precession is proportional to the displacement amplitude of the crystal, and is measured with near-projection-noise-limited resolution. A $49\,$pm displacement is detected with a single measurement signal-to-noise ratio of 1, which is an order-of-magnitude improvement over prior phase-incoherent experiments. This displacement amplitude is $40$ times smaller than the zero-point fluctuations. With our repetition rate, a $8.4\,$pm$/\sqrt{\mathrm{Hz}}$ displacement sensitivity is achieved, which implies $12\,$yN$/\mathrm{ion}/\sqrt{\mathrm{Hz}}$ and $77\,μ$V$/$m$/\sqrt{\mathrm{Hz}}$ sensitivities to forces and electric fields, respectively. This displacement sensitivity, when applied on-resonance with the center-of-mass mode, indicates the possibility of weak force and electric field detection below $10^{-3}\,$yN/ion and $1\,$nV/m, respectively.

We introduce a bang-bang shortcut to adiabaticity for the Dicke model, which we implement via a 2-D array of trapped ions in a Penning trap with a spin-dependent force detuned close to the center-of-mass drumhead mode. Our focus is on employing this shortcut to create highly entangled states that can be used in high-precision metrology. We highlight that the performance of the bang-bang approach is comparable to standard preparation methods, but can be applied over a much shorter time frame. We compare these theoretical ideas with experimental data which serve as a first step towards realizing this theoretical procedure for generating multi-partite entanglement.

Detection of the weakest forces in nature and the search for new physics are aided by increasingly sensitive measurements of the motion of mechanical oscillators. However, the attainable knowledge of an oscillator's motion is limited by quantum fluctuations that exist even if the oscillator is in its lowest possible energy state. Here we demonstrate a widely applicable technique for amplifying coherent displacements of a mechanical oscillator with initial magnitudes well below these zero-point fluctuations. When applying two orthogonal "squeezing" interactions before and after a small displacement, the displacement is amplified, ideally with no added quantum noise. We implement this protocol with a trapped-ion mechanical oscillator and measure an increase of up to 17.5(3) decibels in sensitivity to small displacements.

Scrambling of quantum information is the process by which information initially stored in the local degrees of freedom of a quantum many-body system spreads over its many-body degrees of freedom, becoming inaccessible to local probes and thus apparently lost. Scrambling and entanglement are key concepts reconciling seemingly unrelated behaviors including thermalization of isolated quantum systems and information loss in black holes, and have revolutionized our understanding of non-equilibrium phenomena. Here, we demonstrate that a family of fidelity out-of-time-order correlators (FOTOCs), recently measured in a trapped-ion quantum simulator via time reversal of the many-body dynamics followed by a fidelity measurement, can serve as a unifying diagnostic tool that elucidates the intrinsic connection between fast scrambling, volume law entanglement, ergodicity, quantum chaos, and the associated butterfly effect in the semiclassical dynamics of the system. We demonstrate the utility of FOTOCs by computing them in the Dicke model, an iconic model in quantum optics, recently implemented in atomic and trapped-ion setups. This model describes the coupling of a large spin to an oscillator and features rich behaviors, including a quantum phase transition and chaos. Here, we show that FOTOCs provide a direct measure of the spin-phonon Renyi entropy and quantum thermalization. Moreover, we connect the FOTOCs to the variance of simple operators, allowing us to observe fast scrambling in the parameter regime where the system's classical trajectories are chaotic, and to explicitly relate the quantum and classical Lyapunov exponents in a truly quantum many-body system. Our results open a path for the experimental use of FOTOCs to quantify fast scrambling, determine bounds on quantum information processing and to identify possible candidates of black hole analogs in controllable quantum systems.

We use a self-assembled two-dimensional Coulomb crystal of $\sim 70$ ions in the presence of an external transverse field to engineer a simulator of the Dicke Hamiltonian, an iconic model in quantum optics which features a quantum phase transition between a superradiant/ferromagnetic and a normal/paramagnetic phase. We experimentally implement slow quenches across the quantum critical point and benchmark the dynamics and the performance of the simulator through extensive theory-experiment comparisons which show excellent agreement. The implementation of the Dicke model in fully controllable trapped ion arrays can open a path for the generation of highly entangled states useful for enhanced metrology and the observation of scrambling and quantum chaos in a many-body system.

We use a self-assembled two-dimensional Coulomb crystal of $\sim 70$ ions in the presence of an external transverse field to engineer a quantum simulator of the Dicke Hamiltonian. This Hamiltonian has spin and bosonic degrees of freedom which are encoded by two hyperfine states in each ion and the center of mass motional mode of the crystal, respectively. The Dicke model features a quantum critical point separating two distinct phases: the superradiant (ferromagnetic) and normal (paramagnetic) phases. We experimentally explore protocols that aim to adiabatically prepare the superradiant ground state, a spin-boson cat state with macroscopic phonon occupation, which is well-suited for enhanced metrology and quantum information processing. We start in the normal phase, with all spins aligned along a large transverse field and ramp down the field across the critical point following various protocols. We measure the spin observables, both experimentally and in our simulations to characterize the state of the system at the end of the ramp. We find that under current operating conditions an optimally designed ramp is not sufficient to achieve significant fidelity with the superradiant ground state. However, our theoretical investigation shows that slight modifications of experimental parameters, together with modest reductions in decoherence rates and thermal noise can increase the cat-state fidelity to $\sim 75\%$ for $N \sim 20$ spins. Our results open a path for the use of large ensembles of trapped ions as powerful quantum sensors and quantum computers.

We present a technique to measure the amplitude of a center-of-mass (COM) motion of a two-dimensional ion crystal of $\sim$100 ions. By sensing motion at frequencies far from the COM resonance frequency, we experimentally determine the technique's measurement imprecision. We resolve amplitudes as small as 50 pm, 40 times smaller than the COM mode zero-point fluctuations. The technique employs a spin-dependent, optical-dipole force to couple the mechanical oscillation to the electron spins of the trapped ions, enabling a measurement of one quadrature of the COM motion through a readout of the spin state. We demonstrate sensitivity limits set by spin projection noise and spin decoherence due to off-resonant light scattering. When performed on resonance with the COM mode frequency, the technique demonstrated here can enable the detection of extremely weak forces ($< \,$1 yN) and electric fields ($< \,$1 nV/m), providing an opportunity to probe quantum sensing limits and search for physics beyond the standard model.

We report phase-coherent Doppler detection of optical dipole forces using large ion crystals in a Penning trap. The technique is based on laser Doppler velocimetry using a cycling transition in $^{9}$Be$^{+}$ near 313 nm and the center-of-mass (COM) ion motional mode. The optical dipole force is tuned to excite the COM mode, and measurements of photon arrival times synchronized with the excitation potential show oscillations with a period commensurate with the COM motional frequency. Experimental results compare well with a quantitative model for a driven harmonic oscillator. This technique permits characterization of motional modes in ion crystals; the measurement of both frequency and phase information relative to the driving force is a key enabling capability -- comparable to lockin detection -- providing access to a parameter that is typically not available in time-averaged measurements. This additional information facilitates discrimination of nearly degenerate motional modes.

The ability to detect extremely small forces is vital for a variety of disciplines including precision spin-resonance imaging, microscopy, and tests of fundamental physical phenomena. Current force-detection sensitivity limits have surpassed 1 $aN/\sqrt{Hz}$ (atto $=10^{-18}$) through coupling of micro or nanofabricated mechanical resonators to a variety of physical systems including single-electron transistors, superconducting microwave cavities, and individual spins. These experiments have allowed for probing studies of a variety of phenomena, but sensitivity requirements are ever-increasing as new regimes of physical interactions are considered. Here we show that trapped atomic ions are exquisitely sensitive force detectors, with a measured sensitivity more than three orders of magnitude better than existing reports. We demonstrate detection of forces as small as 174 $yN$ (yocto $=10^{-24}$), with a sensitivity 390$\pm150$ $yN/\sqrt{Hz}$ using crystals of $n=60$ $^{9}$Be$^{+}$ ions in a Penning trap. Our technique is based on the excitation of normal motional modes in an ion trap by externally applied electric fields, detection via and phase-coherent Doppler velocimetry, which allows for the discrimination of ion motion with amplitudes on the scale of nanometers. These experimental results and extracted force-detection sensitivities in the single-ion limit validate proposals suggesting that trapped atomic ions are capable of detecting of forces with sensitivity approaching 1 $yN/\sqrt{Hz}$. We anticipate that this demonstration will be strongly motivational for the development of a new class of deployable trapped-ion-based sensors, and will permit scientists to access new regimes in materials science.

We report on the design, fabrication, and preliminary testing of a 150 zone array built in a `surface-electrode' geometry microfabricated on a single substrate. We demonstrate transport of atomic ions between legs of a `Y'-type junction and measure the in-situ heating rates for the ions. The trap design demonstrates use of a basic component design library that can be quickly assembled to form structures optimized for a particular experiment.

A scalable, multiplexed ion trap for quantum information processing is fabricated and tested. The trap design and fabrication process are optimized for scalability to small trap size and large numbers of interconnected traps, and for integration of control electronics and optics. Multiple traps with similar designs are tested with Cd+, Mg+, and Sr+ ions at room temperature and with Sr+ at 6 K, with respective ion lifetimes of 90 s, 300 +/- 30 s, 56 +/- 6 s, and 4.5 +/- 1.1 hours. The motional heating rate for Mg+ at room temperature and a trap frequency of 1.6 MHz is measured to be 7 +/- 3 quanta per millisecond. For Sr+ at 6 K and 540 kHz the heating rate is measured to be 220 +/- 30 quanta per second.

We have measured motional heating rates of trapped atomic ions, a factor that can influence multi-ion quantum logic gate fidelities. Two simplified techniques were developed for this purpose: one relies on Raman sideband detection implemented with a single laser source, while the second is even simpler and is based on time-resolved fluorescence detection during Doppler recooling. We applied these methods to determine heating rates in a microfrabricated surface-electrode trap made of gold on fused quartz, which traps ions 40 microns above its surface. Heating rates obtained from the two techniques were found to be in reasonable agreement. In addition, the trap gives rise to a heating rate of 300 plus or minus 30 per second for a motional frequency of 5.25 MHz, substantially below the trend observed in other traps.

The prospect of building a quantum information processor underlies many recent advances ion trap fabrication techniques. Potentially, a quantum computer could be constructed from a large array of interconnected ion traps. We report on a micrometer-scale ion trap, fabricated from bulk silicon using micro-electromechanical systems (MEMS) techniques. The trap geometry is relatively simple in that the electrodes lie in a single plane beneath the ions. In such a trap we confine laser-cooled 24Mg+ ions approximately 40 microns above the surface. The fabrication technique and planar electrode geometry together make this approach amenable to scaling up to large trap arrays. In addition we observe that little laser cooling light is scattered by the electrodes.

We demonstrate confinement of individual atomic ions in a radio-frequency Paul trap with a novel geometry where the electrodes are located in a single plane and the ions confined above this plane. This device is realized with a relatively simple fabrication procedure and has important implications for quantum state manipulation and quantum information processing using large numbers of ions. We confine laser-cooled Mg-24 ions approximately 40 micrometer above planar gold electrodes. We measure the ions' motional frequencies and compare them to simulations. From measurements of the escape time of ions from the trap, we also determine a heating rate of approximately five motional quanta per millisecond for a trap frequency of 5.3 MHz.

We briefly discuss recent experiments on quantum information processing using trapped ions at NIST. A central theme of this work has been to increase our capabilities in terms of quantum computing protocols, but we have also applied the same concepts to improved metrology, particularly in the area of frequency standards and atomic clocks. Such work may eventually shed light on more fundamental issues, such as the quantum measurement problem.

A single laser-cooled and trapped 9Be+ ion is used to investigate methods of coherent quantum-state synthesis and quantum logic. We create and characterize nonclassical states of motion including "Schroedinger-cat" states. A fundamental quantum logic gate is realized which uses two states of the quantized ion motion and two ion internal states as qubits. We explore some of the applications for, and problems in realizing, quantum computation based on multiple trapped ions.