J. Eschner

We perform high-resolution real-time read-out of the motion of a single trapped and laser-cooled Ba ion. By using an interferometric setup we demonstrate shot-noise limited measurement of thermal oscillations with resolution of 4 times the standard quantum limit. We apply the real-time monitoring for phase control of the ion motion through a feedback loop, suppressing the photon recoil-induced phase diffusion. Due to the spectral narrowing in phase-locked mode, the coherent ion oscillation is measured with resolution of about 0.3 times the standard quantum limit.

We use a single trapped 40Ca+ ion as a resonant, polarization-sensitive absorber to detect and characterize the entanglement of tunable narrowband photon pairs from a spontaneous parametric down-conversion source. Single-photon absorption is marked by a quantum jump in the ion and heralded by coincident detection of the partner photon. For three polarization basis settings of absorption and detection of the herald, we find maximum coincidences always for orthogonal polarizations. The polarization entanglement is further evidenced by tomographic reconstruction of the biphoton quantum state.

In the fluorescence light of a single atom, the probability for emission of a photon with certain polarization depends on the polarization of the photon emitted immediately before it. Here correlations of such kind are investigated with a single trapped calcium ion by means of second order correlation functions. A theoretical model is developed and fitted to the experimental data, which show 91% probability for the emission of polarization-correlated photon pairs within 24 ns.

We present a photoionization method to load single 40Ca ions in a linear Paul trap from an atomic beam. Neutral Ca I atoms are resonantly excited from the ground state to the intermediate 4s4p 1P_1-level using coherent 423nm radiation produced by single-pass second harmonic generation in a periodically poled KTiOPO_4 crystal pumped with an 120mW extended cavity diode laser. Ionization is then attained with a high-power light emitting diode imaged to the trap center, using an appropriately designed optical system composed of standard achromatic doublet lenses. The setup simplifies previous implementations at similar efficiency, and it hardly requires any maintenance at all.

We observe the interaction of a single trapped calcium ion with single photons produced by a narrow-band, resonant down-conversion source [A. Haase et al., Opt. Lett. 34, 55 (2009)], employing a quantum jump scheme. Using the temperature dependence of the down-conversion spectrum and the tunability of the narrow source, absorption of the down-conversion photons is quantitatively characterized.

We report a tunable single-photon source based on a single trapped ion. Employing spontaneous Raman scattering and in-vacuum optics with large numerical aperture, single photons are efficiently created with controlled temporal shape and coherence time. These can be varied between 70 ns and 1.6 $μ$s, as characterized by operating two sources simultaneously in two remote ion traps which reveals mutual and individual coherence through two-photon interference.

We report measurements of an intensity-field correlation function of the resonance fluorescence of a single trapped Ba+ ion. Detection of a photon prepares the atom in its ground state and we observe its subsequent evolution under interaction with a laser field of well defined phase. We record the regression of the resonance fluorescence source field. This provides a direct measurement of the field of the radiating dipole of a single atom and exhibits its strong non-classical behavior. In the experimental setup an interference measurement is conditioned on a fluorescence photon detection. The third-order correlation function thus recorded demonstrates an aspect of wave-particle duality at the single-atom, single-photon level.

We observe quantum interference of photons emitted by two continuously laser-excited single ions, independently trapped in distinct vacuum vessels. High contrast two-photon interference is observed in two experiments with different ion species, calcium and barium. Our experimental findings are quantitatively reproduced by Bloch equation calculations. In particular, we show that the coherence of the individual resonance fluorescence light field is determined from the observed interference.

When trapped atoms are illuminated by weak lasers, off-resonant transitions cause shifts in the frequencies of the vibrational-sideband resonances. These frequency shifts may be understood in terms of Stark-shifts of the individual levels or, as proposed here, as a vibrational Bloch-Siegert shift, an effect closely related to the usual (radio-frequency or optical) Bloch-Siegert shift and associated with rapidly oscillating terms when the Rotating Wave Approximation is not made. Explicit analytic expressions are derived and compared to numerical results, and the similarities and differences between the usual and the vibrational Bloch-Siegert shifts are also spelled out.

First order Doppler effects are usually ignored in laser driven trapped ions when the recoil frequency is much smaller than the trapping frequency (Lamb-Dicke regime). This means that the central, carrier excitation band is supposed to be unaffected by vibronic transitions in which the vibrational number changes. While this is strictly true in the Lamb-Dicke limit (infinitely tight confinement), the vibronic transitions do play a role in the Lamb-Dicke regime. In this paper we quantify the asymptotic behaviour of their effect with respect to the Lamb-Dicke parameter. In particular, we give analytical expressions for the frequency shift, ``pulling'' or ``pushing'', produced in the carrier absorption band by the vibronic transitions both for Rabi and Ramsey schemes. This shift is shown to be independent of the initial vibrational state.

We report the realization of an elementary quantum processor based on a linear crystal of trapped ions. Each ion serves as a quantum bit (qubit) to store the quantum information in long lived electronic states. We present the realization of single-qubit and of universal two-qubit logic gates. The qwo-qubit operation relies on the coupling of the ions through their collective quantized motion. A detailed description of the setup and the methods is included.

A single 40Ca+ ion is trapped and laser cooled to its motional ground state. Laser radiation which couples off-resonantly to a motional sideband of the ion's S1/2 to D5/2 transition causes a phase shift proportional to the ion's motional quantum state |n>. As the phase shift is conditional upon the ion's motion, we are able to demonstrate a universal 2-qubit quantum gate operation where the electronic target state {S,D} is flipped depending on the motional qubit state |n>={|0>,|1>}. Finally, we discuss scaling properties of this universal quantum gate for linear ion crystals and present numerical simulations for the generation of a maximally entangled state of five ions.

We report on tomographic means to study the stability of a qubit register based on a string of trapped ions. In our experiment, two ions are held in a linear Paul trap and are entangled deterministically by laser pulses that couple their electronic and motional states. We reconstruct the density matrix using single qubit rotations and subsequent measurements with near-unity detection efficiency. This way, we characterize the created Bell states, the states into which they subsequently decay, and we derive their entanglement, applying different entanglement measures.

A distant mirror leads to a vacuum-induced level shift in a laser-excited atom. This effect has been measured with a single mirror 25 cm away from a single, trapped barium ion. This dispersive action is the counterpart to the mirror's dissipative effect, which has been shown earlier to effect a change in the ion's spontaneous decay [J. Eschner et al., Nature 413, 495-498 (2001)]. The experimental data are well described by 8-level optical Bloch equations which are amended to take into account the presence of the mirror according to the model in [U. Dorner and P. Zoller, Phys. Rev. A 66, 023816 (2002)]. Observed deviations from simple dispersive behavior are attributed to multi-level effects.

Using optical Ramsey interferometry, we precisely measure the laser-induced AC-stark shift on the $S_{1/2}$ -- $D_{5/2}$ "quantum bit" transition near 729 nm in a single trapped $^{40}$Ca$^+$ ion. We cancel this shift using an additional laser field. This technique is of particular importance for the implementation of quantum information processing with cold trapped ions. As a simple application we measure the atomic phase evolution during a $n \times 2π$ rotation of the quantum bit.

Two-level ionic systems, where quantum information is encoded in long lived states (qubits), are discussed extensively for quantum information processing. We present a collection of measurements which characterize the stability of a qubit based on the $S_{1/2}$--$D_{5/2}$ transition of single $^{40}$Ca$^+$ ions in a linear Paul trap. We find coherence times of $\simeq$1 ms, discuss the main technical limitations and outline possible improvements.

The quadrupole S$_{1/2}$ -- D$_{5/2}$ optical transition of a single trapped Ca$^+$ ion, well suited for encoding a quantum bit of information, is coherently coupled to the standing wave field of a high finesse cavity. The coupling is verified by observing the ion's response to both spatial and temporal variations of the intracavity field. We also achieve deterministic coupling of the cavity mode to the ion's vibrational state by selectively exciting vibrational state-changing transitions and by controlling the position of the ion in the standing wave field with nanometer-precision.

A novel method of ground state laser cooling of trapped atoms utilizes the absorption profile of a three (or multi-) level system which is tailored by a quantum interference. With cooling rates comparable to conventional sideband cooling, lower final temperatures may be achieved. The method was experimentally implemented to cool a single Ca$^+$ ion to its vibrational ground state. Since a broad band of vibrational frequencies can be cooled simultaneously, the technique will be particularly useful for the cooling of larger ion strings, thereby being of great practical importance for initializing a quantum register based on trapped ions. We also discuss its application to different level schemes and for ground state cooling of neutral atoms trapped by a far detuned standing wave laser field.

Ground state cooling and coherent manipulation of ions in an rf-(Paul) trap is the prerequisite for quantum information experiments with trapped ions. With resolved sideband cooling on the optical S1/2 - D5/2 quadrupole transition we have cooled one and two 40Ca+ ions to the ground state of vibration with up to 99.9% probability. With a novel cooling scheme utilizing electromagnetically induced transparency on the S1/2 - P1/2 manifold we have achieved simultaneous ground state cooling of two motional sidebands 1.7 MHz apart. Starting from the motional ground state we have demonstrated coherent quantum state manipulation on the S1/2 - D5/2 quadrupole transition at 729 nm. Up to 30 Rabi oscillations within 1.4 ms have been observed in the motional ground state and in the n=1 Fock state. In the linear quadrupole rf-trap with 700 kHz trap frequency along the symmetry axis (2 MHz in radial direction) the minimum ion spacing is more than 5 micron for up to 4 ions. We are able to cool two ions to the ground state in the trap and individually address the ions with laser pulses through a special optical addressing channel.

Ground state laser cooling of a single trapped ion is achieved using a technique which tailors the absorption profile for the cooling laser by exploiting electromagnetically induced transparency in the Zeeman structure of a dipole transition. This new method is robust, easy to implement and proves particularly useful for cooling several motional degrees of freedom simultaneously, which is of great practical importance for the implementation of quantum logic schemes with trapped ions.

We have cooled a two-ion-crystal to the ground state of its collective modes of motion. Laser cooling, more specific resolved sideband cooling is performed sympathetically by illuminating only one of the two $^{40}$Ca$^+$ ions in the crystal. The heating rates of the motional modes of the crystal in our linear trap have been measured, and we found them considerably smaller than those previously reported by Q. Turchette {\em et. al.} Phys. Rev. A 61, 063418 (2000) in the case of trapped $^9$Be$^+$ ions. After the ground state is prepared, coherent quantum state manipulation of the atomic population can be performed. Within the coherence time, up to 12 Rabi oscillations are observed, showing that many coherent manipulations can be achieved. Coherent excitation of each ion individually and ground state cooling are important tools for the realization of quantum information processing in ion traps.

We investigate single ions of $^{40}Ca^+$ in Paul traps for quantum information processing. Superpositions of the S$_{1/2}$ electronic ground state and the metastable D$_{5/2}$ state are used to implement a qubit. Laser light on the S$_{1/2} \leftrightarrow$ D$_{5/2}$ transition is used for the manipulation of the ion's quantum state. We apply sideband cooling to the ion and reach the ground state of vibration with up to 99.9% probability. Starting from this Fock state $|n=0>$, we demonstrate coherent quantum state manipulation. A large number of Rabi oscillations and a ms-coherence time is observed. Motional heating is measured to be as low as one vibrational quantum in 190 ms. We also report on ground state cooling of two ions.

Resonance fluorescence of a single trapped ion is spectrally analyzed using a heterodyne technique. Motional sidebands due to the oscillation of the ion in the harmonic trap potential are observed in the fluorescence spectrum. From the width of the sidebands the cooling rate is obtained and found to be in agreement with the theoretical prediction.

A single Ca+ ion in a Paul trap has been cooled to the ground state of vibration with up to 99.9% probability. Starting from this Fock state |n=0> we have demonstrated coherent quantum state manipulation on an optical transition. Up to 30 Rabi oscillations within 1.4 ms have been observed. We find a similar number of Rabi oscillations after preparation of the ion in the |n=1> Fock state. The coherence of optical state manipulation is only limited by laser and ambient magnetic field fluctuations. Motional heating has been measured to be as low as one vibrational quantum in 190 ms.

We study laser cooling of two ions that are trapped in a harmonic potential and interact by Coulomb repulsion. Sideband cooling in the Lamb-Dicke regime is shown to work analogously to sideband cooling of a single ion. Outside the Lamb-Dicke regime, the incommensurable frequencies of the two vibrational modes result in a quasi-continuous energy spectrum that significantly alters the cooling dynamics. The cooling time decreases nonlinearly with the linewidth of the cooling transition, and the effect of trapping states which may slow down the cooling is considerably reduced. We show that cooling to the ground state is possible also outside the Lamb-Dicke regime. We develop the model and use Quantum Monte Carlo calculations for specific examples. We show that a rate equation treatment is a good approximation in all cases.