M. Hennrich

The strong dipole-dipole interaction of trapped Rydberg ions offers the possibility of sub-microsecond entanglement gates. For example a two-qubit Control-Phase gate in 88 Sr + ions can be realized, by simultaneous excitation to the Rydberg states via stimulated Raman adiabatic passage (STIRAP) with simultaneous microwave induced dipole-dipole interaction. We show that this excitation protocol distorts the dark-state of the STIRAP stage and is prone to decay from the intermediate state. Here, we propose a novel pulse ordering, in which the STIRAP and the microwave dressing of the Rydberg states occurs in separate stages, preventing mutual interference effects that are detrimental to the gate fidelity. We show that, for experimentally feasible parameters, the proposed excitation scheme can achieve a fidelity of 99.93%, surpassing the experimentally demonstrated gate. In addition, we demonstrate a non-adiabatic speed-up to 400 ns by employing asymmetric pulse shapes in the STIRAP stage. The entangling phase is then controlled solely through the interaction strength by nonresonant asymmetric chirping of the microwave field.

We propose a quantum algorithm in an embedding ion-trap quantum simulator for the efficient computation of N-qubit entanglement monotones without the necessity of full tomography. Moreover, we discuss possible realistic scenarios and study the associated decoherence mechanisms.

Dynamical maps describe general transformations of the state of a physical system, and their iteration can be interpreted as generating a discrete time evolution. Prime examples include classical nonlinear systems undergoing transitions to chaos. Quantum mechanical counterparts show intriguing phenomena such as dynamical localization on the single particle level. Here we extend the concept of dynamical maps to an open-system, many-particle context: We experimentally explore the stroboscopic dynamics of a complex many-body spin model by means of a universal quantum simulator using up to five ions. In particular, we generate long-range phase coherence of spin by an iteration of purely dissipative quantum maps. We also demonstrate the characteristics of competition between combined coherent and dissipative non-equilibrium evolution. This opens the door for studying many-particle non-equilibrium physics and associated dynamical phase transitions with no immediate counterpart in equilibrium condensed matter systems. An error detection and reduction toolbox that facilitates the faithful quantum simulation of larger systems is developed as a first step in this direction.

A scheme for entangling distant atoms is realized, as proposed in the seminal paper by Cabrillo et al. [Phys. Rev. A 59, 1025 (1999)]. The protocol is based on quantum interference and detection of a single photon scattered from two effectively one meter distant laser-cooled and trapped atomic ions. The detection of a single photon heralds entanglement of two internal states of the trapped ions with high rate and with a fidelity limited mostly by atomic motion. Control of the entangled state phase is demonstrated by changing the path length of the single-photon interferometer.

A digital quantum simulator is an envisioned quantum device that can be pro- grammed to efficiently simulate any other local system. We demonstrate and investigate the digital approach to quantum simulation in a system of trapped ions. Using sequences of up to 100 gates and 6 qubits, the full time dynamics of a range of spin systems are digitally simulated. Interactions beyond those naturally present in our simulator are accurately reproduced and quantitative bounds are provided for the overall simulation quality. Our results demon- strate the key principles of digital quantum simulation and provide evidence that the level of control required for a full-scale device is within reach.

By tightly focussing a laser field onto a single cold ion trapped in front of a far-distant dielectric mirror, we could observe a quantum electrodynamic effect whereby the ion behaves as the optical mirror of a Fabry-Pérot cavity. We show that the amplitude of the laser field is significantly altered due to a modification of the electromagnetic mode structure around the atom in a novel regime in which the laser intensity is already changed by the atom alone. e propose a direct application of this system as a quantum memory for single photons.

Multiparticle entanglement leads to richer correlations than two-particle entanglement and gives rise to striking contradictions with local realism, inequivalent classes of entanglement, and applications such as one-way or topological quantum computing. When exposed to decohering or dissipative environments, multiparticle entanglement yields subtle dynamical features and access to new classes of states and applications. Here, using a string of trapped ions, we experimentally characterize the dynamics of entanglement of a multiparticle state under the influence of decoherence. By embedding an entangled state of four qubits in a decohering environment (via spontaneous decay), we observe a rich dynamics crossing distinctive domains: Bell-inequality violation, entanglement superactivation, bound entanglement, and full separability. We also develop new theoretical tools for characterizing entanglement in quantum states. Our techniques to control the environment can be used to enable novel quantum-computation, state-engineering, and simulation paradigms based on dissipation and decoherence.

We present a photoionization method to load single 40Ca ions in a linear Paul trap from an atomic beam. Neutral Ca I atoms are resonantly excited from the ground state to the intermediate 4s4p 1P_1-level using coherent 423nm radiation produced by single-pass second harmonic generation in a periodically poled KTiOPO_4 crystal pumped with an 120mW extended cavity diode laser. Ionization is then attained with a high-power light emitting diode imaged to the trap center, using an appropriately designed optical system composed of standard achromatic doublet lenses. The setup simplifies previous implementations at similar efficiency, and it hardly requires any maintenance at all.

Any residual coupling of a quantum computer to the environment results in computational errors. Encoding quantum information in a so-called decoherence-free subspace provides means to avoid these errors. Despite tremendous progress in employing this technique to extend memory storage times by orders of magnitude, computation within such subspaces has been scarce. Here, we demonstrate the realization of a universal set of quantum gates acting on decoherence-free ion qubits. We combine these gates to realize the first controlled-NOT gate within a decoherence-free, scalable quantum computer.

We observe the interaction of a single trapped calcium ion with single photons produced by a narrow-band, resonant down-conversion source [A. Haase et al., Opt. Lett. 34, 55 (2009)], employing a quantum jump scheme. Using the temperature dependence of the down-conversion spectrum and the tunability of the narrow source, absorption of the down-conversion photons is quantitatively characterized.

We report a tunable single-photon source based on a single trapped ion. Employing spontaneous Raman scattering and in-vacuum optics with large numerical aperture, single photons are efficiently created with controlled temporal shape and coherence time. These can be varied between 70 ns and 1.6 $μ$s, as characterized by operating two sources simultaneously in two remote ion traps which reveals mutual and individual coherence through two-photon interference.

We observe quantum interference of photons emitted by two continuously laser-excited single ions, independently trapped in distinct vacuum vessels. High contrast two-photon interference is observed in two experiments with different ion species, calcium and barium. Our experimental findings are quantitatively reproduced by Bloch equation calculations. In particular, we show that the coherence of the individual resonance fluorescence light field is determined from the observed interference.

Algorithms for quantum information processing are usually decomposed into sequences of quantum gate operations, most often realized with single- and two- qubit gates[1]. While such operations constitute a universal set for quantum computation, gates acting on more than two qubits can simplify the implementation of complex quantum algorithms[2]. Thus, a single three-qubit operation can replace a complex sequence of two-qubit gates, which in turn promises faster execution with potentially higher Fidelity. One important three-qubit operation is the quantum Toffoli gate which performs a NOT operation on a target qubit depending on the state of two control qubits. Here we present the first experimental realization of the quantum Toffoli gate in an ion trap quantum computer. Our implementation is particular effcient as we directly encode the relevant logic information in the motion of the ion string. [1] DiVincenzo, D. P. Two-bit gates are universal for quantum computation. cond-mat/9407022, Phys.Rev. A 51, 1015-1022 (1995). [2] Chiaverini, J. et al. Realization of quantum error correction. Nature 432, 602-605 (2004).