B. Liu

Offline Commissioning of the St. Benedict Gas Catcher

F. Rivero, D. Guillet, M. Brodeur, J. A. Clark, A. M. Houff, J. J. Kolata, B. Liu, J. McRae, P. D. O'Malley, W. S. Porter, C. Quick, G. Savard [1], A. A. Valverde, R. Zite [1]

Abstract

Precision measurements of $β$ decay transitions offer a promising channel through which the Standard Model (SM) can be probed. There is currently an ongoing effort to increase the precision on measurements of $\mathcal{F}t$-values for superallowed $β$ decay transitions between mirror nuclides. These allow for a determination of $V_{ud}$ which is complementary to that obtained from pure Fermi $0^+ \rightarrow 0^+$ transitions. The Superallowed Transition BEta-NEutrino Decay Ion Coincidence Trap (St. Benedict), under construction at the Nuclear Science Laboratory (NSL) at the University of Notre Dame, seeks to measure the Fermi-to-Gamow-Teller mixing ratio for transitions between mirror nuclei in order to expand the list of nuclides from which $V_{ud}$ can be extracted. Production and selection of the species of interest will be done in-flight, using the \textit{TwinSol} magnetic separator system. The first element of St. Benedict will be a large volume gas catcher which will thermalize radioactive ion beams for low energy delivery to the rest of the system. Offline commissioning of this gas catcher has been completed using an internal potassium source, and the device demonstrated a transport efficiency upwards of 95\% for pressures of 66 mbar and lower.

Precision Mass Measurements of \textsuperscript{130}Te, \textsuperscript{130}Sn, and Their Impact on Models for R-Process Nucleosynthesis

A. Cannon, W. S. Porter, A. A. Valverde, D. P. Burdette, A. M. Houff, B. Liu, A. Mitra, G. E. Morgan, C. Quick [1], D. Ray [1], L. Varriano [1], M. Brodeur [1], J. A. Clark, G. Savard [1], G. J. Mathews

Abstract

The astrophysical rapid neutron capture nucleosynthesis process (r-process) remains an active area of research due to the fact that it occurs in extreme conditions and involves reactions with exotic nuclei that are difficult to study experimentally. For the first time using the Phase-Imaging Ion Cyclotron Resonance (PI-ICR) technique, we measured the mass excesses of \textsuperscript{130}Te, \textsuperscript{130}Sn, and \textsuperscript{130}Sn\textsuperscript{m} with the Canadian Penning Trap (CPT). Our results show good agreement with previous Penning trap values obtained using the Time-of-Flight Ion Cyclotron Resonance (TOF-ICR) and the Fourier Transform Ion Cyclotron Resonance (FT-ICR) techniques, while being twice as precise for \textsuperscript{130}Sn. These new mass excesses were added to a SkyNet network calculation to determine their impact on r-process abundances and to find the best astrophysical conditions to reproduce the Solar System r-process abundance pattern. Finally, by treating lighter and heavier elements separately, we assess the relative frequency of events producing elements in a cold versus a hot r-process scenario.

Precise Mass Measurement of the $^{149}$La-$^{149}$Ce-$^{149}$Pr isobaric chain

B. Liu [1,2], M. Brodeur [1,2], J. A. Clark, D. Ray [3,2], G. Savard [2,4,3,1], A. A. Valverde, D. P. Burdette, A. M. Houff, A. Mitra [1,5,2], G. E. Morgan, R. Orford [6,1], W. S. Porter, C. Quick [1], F. Rivero [1,3], K. S. Sharma, L. Varriano [4,2]

Abstract

Penning trap mass measurements of $^{149}$La, $^{149}$Ce, and $^{149}$Pr were performed with the Canadian Penning Trap (CPT) at the CARIBU facility of Argonne National Laboratory using the phase-imaging ion-cyclotron-resonance technique. The resulting mass excess of $^{149}$La differs by 221 keV from a recent JYFLTRAP measurement, resulting in a significant change in the profile of the two-neutron separation energy for that isotopic chain. The mass excesses of $^{149}$Ce and $^{149}$Pr are determined with an eight-fold improvement in precision compared to previous time-of-flight ion-cyclotron-resonance measurements; the $^{149}$Ce value is consistent with AME2020, while the $^{149}$Pr mass excess is lower by 17.5 keV. The mass excesses of $^{149}$La and $^{149}$Pr reported in this work have been confirmed recently by a measurement with a multi-reflection time-of-flight mass spectrometer coupled to a $β$-time of flight detector at RIKEN, providing further validation of the present results.

Off-line Commissioning of the St. Benedict Radiofrequency Quadrupole Cooler-Buncher

D. P. Burdette, R. Zite, M. Brodeur, A. A. Valverde, O. Bruce, R. Bualuan, A. Cannon, J. A. Clark, C. Davis, T. Florenzo, A. T. Gallant, J. Harkin, A. M. Houff, J. Li, B. Liu, J. Long, P. D. O'Malley, W. S. Porter, C. Quick [1], R. Ringle [1], F. Rivero [1], G. Savard [1], M. A. Yeck

Abstract

The St. Benedict ion trapping system, which aims to measure the $β-ν$ angular correlation parameter in superallowed-mixed mirror transitions, is under construction at the University of Notre Dame. These measurements will provide much-needed data to improve the accuracy of the $V_{ud}$ element of the CKM matrix. One of the major components of this system is the radio frequency quadrupole cooler-buncher, which is necessary to create low-emittance ion bunches for injection into the measurement Paul trap. The off-line commissioning of the cooler-buncher, using a potassium ion source, determined that the device could produce cooled ion bunches characterized by a 50-ns full-width-half-maximum time width. The commissioning results also determined the trapping efficiency to be 93(1)$\%$ and the trapping half-life to be 20.0(5) s.

Astrophysical significance of the isomer $^{119m}$Ag demonstrated through direct mass measurement

F. Rivero [1], M. Brodeur [1,2], J. A. Clark, B. Liu [1,2,3,4], G. W. Misch, M. R. Mumpower, W. S. Porter, D. Ray [5,2], G. Savard [2,6,3,5], T. M. Sprouse, A. A. Valverde, D. P. Burdette, A. Cannon [7,8,1], A. T. Gallant, A. M. Houff, K. Kolos [8,2], F. G. Kondev, R. Orford [9], C. Quick [1,5], K. S. Sharma, L. Varriano [10]

Abstract

The abundance of elements heavier than iron produced via the astrophysical rapid-neutron capture process depends sensitively on the atomic mass of the involved nuclei as well as the behavior of a few special types of nuclear isomers called astromers. High-precision mass measurements of $^{119}$Cd, $^{119}$Ag and their respective isomeric states have been performed with the Phase Imaging-Ion Cyclotron Resonance (PI-ICR) method with a precision of $δm/m \approx 10^{-8}$ using the Canadian Penning Trap (CPT). The ground state mass excess, as well as the excitation energy, agrees with recent Penning Trap measurements from JYFLTRAP. Network calculations using these new measurements revealed that, contrary to previous expectations, $^{119m}$Ag behaves as an astromer which significantly affects the population of $^{119}$Ag.

Mass measurements of neutron-rich nuclides using the Canadian Penning Trap to inform predictions in the $r$-process rare-earth peak region

D. Ray [1,2], N. Vassh [3], B. Liu [4,2,1], A. A. Valverde, M. Brodeur [4,2,1,5,6], J. A. Clark, G. C. McLaughlin, M. R. Mumpower, R. Orford [7,4], W. S. Porter, G. Savard [2,8], K. S. Sharma [1], R. Surman [4], F. Buchinger [9,2], D. P. Burdette, N. Callahan [2,10], A. T. Gallant, D. E. M. Hoff, K. Kolos [10,2], F. G. Kondev, G. E. Morgan [2,11], F. Rivero [4], D. Santiago-Gonzalez [2,10], N. D. Scielzo, L. Varriano [2,8,12], C. M. Weber, G. E. Wilson [11,2,13], X. L. Yan

Abstract

Studies aiming to determine the astrophysical origins of nuclei produced by the rapid neutron capture process ($r$ process) rely on nuclear properties as inputs for simulations. The solar abundances can be used as a benchmark for such calculations, with the $r$-process rare-earth peak (REP) around mass number ($A$) 164 being of special interest due to its presently unknown origin. With the advancement of rare isotope beam production over the last decade and improvement in experimental sensitivities, many of these REP nuclides have become accessible for measurement. Masses are one of the most critical inputs as they impact multiple nuclear properties, namely the neutron-separation energies, neutron capture rates, $β$-decay rates, and $β$-delayed neutron emission probabilities. In this work, we report masses of 20 neutron-rich nuclides (along the Ba, La, Ce, Pr, Nd, Pm, Gd, Dy and Ho isotopic chains) produced at the CAlifornium Rare Isotope Breeder Upgrade (CARIBU) facility at Argonne National Laboratory. The masses were measured with the Canadian Penning trap (CPT) mass spectrometer using the Phase-Imaging Ion-Cyclotron-Resonance (PI-ICR) technique. We then use these new masses along with previously published CPT masses to inform predictions for a Markov Chain Monte Carlo (MCMC) procedure aiming to identify the astrophysical conditions consistent with both solar data and mass measurements. We show that the MCMC responds to this updated mass information, producing refined results for both mass predictions and REP abundances.

Phase-Imaging Ion-Cyclotron-Resonance Mass Spectrometry with the Canadian Penning Trap at CARIBU

D. Ray, A. A. Valverde, M. Brodeur, F. Buchinger, J. A. Clark, B. Liu, G. E. Morgan, R. Orford [1], W. S. Porter, G. Savard [1], K. S. Sharma, X. L. Yan

Abstract

The Canadian Penning Trap mass spectrometer (CPT) has conducted precision mass measurements of neutron-rich nuclides from the CAlifornium Rare Isotope Breeder Upgrade (CARIBU) of the Argonne Tandem Linac Accelerator System (ATLAS) facility at Argonne National Laboratory using the Phase-Imaging Ion-Cyclotron-Resonance (PIICR) technique for over half a decade. Here we discuss the CPT system, and methods to improve accuracy and precision in mass measurement using PI-ICR including some optimization techniques and recently studied systematic effects.

Self-trapping and acceleration of ions in laser-driven relativistically transparent plasma

B. Liu [1], J. Meyer-ter-Vehn [2], H. Ruhl [1]

Abstract

Self-trapping and acceleration of ions in laser-driven relativistically transparent plasma are investigated with the help of particle-in-cell simulations. A theoretical model based on ion wave breaking is established in describing ion evolution and ion trapping. The threshold for ion trapping is identified. Near the threshold ion trapping is self-regulating and stops when the number of trapped ions is large enough. The model is applied to ion trapping in three-dimensional geometry. Longitudinal distributions of ions and the electric field near the wave breaking point are derived analytically in terms of power-law scalings. The areal density of trapped charge is obtained as a function of the strength of ion wave breaking, which scales with target density for fixed laser intensity. The results of the model are confirmed by the simulations.