P. Delahaye

Performance of the MORA Apparatus for Testing Time-Reversal Invariance in Nuclear Beta Decay

N. Goyal [1], A. Singh [1], S. Daumas-Tschopp [2], L. M. Motilla Martinez [1,3], G. Ban [2], V. Bosquet [2], J. F. Cam [2], P. Chauveau [1], S. Chinthakayala [1,3,4], G. Fremont, R. P. De Groote, F. de Oliveira Santos [1], T. Eronen [3], A. Falkowski [5,2], X. Flechard, Z. Ge [3,6,1], M. Gonzalez-Alonso, H. Guerin, L. Hayen [2], A. Jaries [3], M. Jbayli [1], A. Jokinen [3], A. Kankainen [3], B. Kootte [3], R. Kronholm [3], N. Lecesne [1], Y. Merrer [2], V. Morel [1], M. Mougeot [3], G. Neyens [4], J. Perronnel [2], M. Reponen [3], A. Raggio [3], S. Rinta-Antila [3], A. Rodriguez-Sanchez [6], N. Severijns [4], J. C. Thomas [1], C. Vandamme [2], S. Vanlangendonk [4], V. Virtanen [3,2], E. Lienard, I. D. Moore [3], P. Delahaye [1]

Abstract

The MORA experimental setup is designed to measure the triple-correlation D parameter in nuclear beta decay. The D coefficient is sensitive to possible violations of time-reversal invariance. The experimental configuration consists of a transparent Paul trap surrounded by a detection setup with alternating beta and recoil-ion detectors. The octagonal symmetry of the detection setup optimizes the sensitivity of positron-recoil-ion coincidence rates to the D correlation, while reducing systematic effects. MORA utilizes an innovative in-trap laser polarization technique. The design and performance of the ion trap, associated beamline elements, lasers and beta and recoil-ion detectors, are presented. Recent progress towards the polarization proof-of-principle is described.

High-precision mass measurements of the ground and isomeric states in $^{124,125}$Ag

J. Ruotsalainen [1], D. A. Nesterenko [1], M. Stryjczyk [1], A. Kankainen [1], L. Al Ayoubi [1,2], O. Beliuskina [1], L. Canete [1], P. Chauveau [3], R. P. de Groote [1], P. Delahaye [4], T. Eronen [1], M. Flayol [5], Z. Ge [6,1], S. Geldhof [1], W. Gins [1], M. Hukkanen [1,5], A. Jaries [1], D. Kahl, D. Kumar [6], I. D. Moore [1], S. Nikas [1], H. Penttilä, D. Pitman-Weymouth [8], A. Raggio [1], S. Rinta-Antila [1], A. de Roubin [1], M. Vilen [1], V. Virtanen, M. Winter [1]

Abstract

The masses of the ground and isomeric states in $^{124,125}$Ag have been measured using the phase-imaging ion-cyclotron-resonance technique at the JYFLTRAP double Penning trap mass spectrometer. The ground states of $^{124}$Ag and $^{125}$Ag were found to be 30(250) keV and 250(430) keV less bound but 36 and 110 times more precise than in the Atomic Mass Evaluation 2020, respectively. The excitation energy of $^{124}$Ag$^{m}$, ${E_x = 188.2(25)}$ keV, was determined for the first time. The new precise mass values have been utilised to study the evolution of nuclear structure via two-neutron separation energies. The impact on the astrophysical rapid neutron capture process has been investigated via neutron-capture reaction rate calculations. The precision measurements indicate a more linear trend in two-neutron separation energies and reduce the mass-related uncertainties for the neutron-capture rate of $^{124}$Ag$(n,γ)^{125}$Ag by a factor of around 100. The new mass values also improve the mass of $^{123}$Pd, previously measured using $^{124}$Ag as a reference.

Isomeric states of fission fragments explored via Penning trap mass spectrometry at IGISOL

A. Jaries [1], M. Stryjczyk [1], A. Kankainen [1], L. Al Ayoubi [1,2], O. Beliuskina [1], L. Canete [1], R. P. de Groote, C. Delafosse [1], P. Delahaye [3], T. Eronen [1], M. Flayol [4], Z. Ge [5,1], S. Geldhof [1], W. Gins [1], M. Hukkanen [1,4], P. Imgram [6], D. Kahl, J. Kostensalo [8,1], S. Kujanpää, D. Kumar [5,1], I. D. Moore, M. Mougeot [1], D. A. Nesterenko, S. Nikas [1], D. Patel [9,1], H. Penttilä, D. Pitman-Weymouth [10], I. Pohjalainen [1], A. Raggio [1], M. Ramalho [1], M. Reponen [1], S. Rinta-Antila [1], A. de Roubin [1,4], J. Ruotsalainen [1,9], P. C. Srivastava, J. Suhonen [1,11], M. Vilen [1], V. Virtanen [1], A. Zadvornaya [1]

Abstract

The masses of $^{84}$Br, $^{105}$Mo, $^{115,119,121}$Pd, $^{122}$Ag, $^{127,129}$In, $^{132}$Sb and their respective isomeric states have been measured with the JYFLTRAP Penning trap mass spectrometer using the phase-imaging ion-cyclotron-resonance technique. The excitation energies of the isomeric states in $^{132}$Sb and $^{119}$Pd were experimentally determined for the first time, while for $^{84}$Br, $^{115}$Pd and $^{127,129}$In, the precision of the mass values was substantially improved. In $^{105}$Mo and $^{121}$Pd there were no signs of a long-lived isomeric state. The ground-state measurements of $^{119}$Pd and $^{122}$Ag indicated that both are significantly more bound than the literature values. For $^{122}$Ag, there was no indication of a proposed third long-lived state. The results for the $N=49$ nucleus $^{84}$Br and isomers close to doubly magic $^{132}$Sn have been compared to the shell-model and the microscopic quasiparticle-phonon model calculations.

High-precision Penning-trap mass measurements of Cd and In isotopes at JYFLTRAP remove the fluctuations in the two-neutron separation energies

A. Jaries [1], M. Stryjczyk [1], A. Kankainen [1], L. Al Ayoubi [1,2], O. Beliuskina [1], P. Delahaye [3], T. Eronen [1], M. Flayol [4], Z. Ge [5,1], W. Gins [1], M. Hukkanen [1,4], D. Kahl [1], S. Kujanpää, D. Kumar [5,1], I. D. Moore, M. Mougeot [1], D. A. Nesterenko, S. Nikas [1], H. Penttilä, D. Pitman-Weymouth [7], I. Pohjalainen [1], A. Raggio [1], W. Rattanasakuldilok [1], A. de Roubin [4], J. Ruotsalainen [1], V. Virtanen [1]

Abstract

We report on the first direct mass measurements of the $^{118,119}$Cd and $^{117-119}$In isotopes performed at the Ion Guide Isotope Separator On-Line facility using the JYFLTRAP double Penning trap mass spectrometer. The masses of $^{117}$In and $^{118}$Cd isotopes are in agreement with the literature, while $^{118,119}$In and $^{119}$Cd differ from literature by 49, 13 and 85 keV (6.1, 1.9 and 2.1 standard deviations), respectively. The excitation energy of the $^{118}$In first isomeric state, $E_x = 40.3(25)$ keV, was determined for the first time. The updated mass values removed the fluctuations observed in the two-neutron separation energies and lead to a smoother linear decrease of both isotopic chains. The $\log(ft)$ value for the $^{118}$Cd decay is also found to increase from 3.93(6) to 4.089(8). The reported results indicate an absence of significant structural changes around $N=70$.

Geometry optimisation of a transparent axisymmetric ion trap for the MORA project

M. Benali [1], G. Quéméner, P. Delahaye [2,1], X. Fléchard, E. Liénard, B. M. Retailleau

Abstract

In the frame of the project MORA (Matter's Origin from the Radio Activity of trapped and oriented ions), a transparent axially symmetric radio-frequency ion trap (MORATrap) was designed in order to measure the triple correlation parameter $D$ in nuclear $β-$decay of laser-polarised ions. The trap design was inspired from the LPCTrap geometry, operated at GANIL from 2005 to 2013. In a real (non-ideal) Paul trap, the quadrupole electric potential is not perfect leading to instabilities in ion motion and therefore affecting the overall trapping efficiency. This paper presents a numerical method aiming to optimise the geometry of a trap. It is applied to MORATrap in order to improve the trapping efficiency and to enlarge the axial transparent solid angle compared to LPCTrap. In the whole optimisation process, numerical computation of electric potential and field was carried out using an electrostatic solver based on boundary element method (BEM). The optimisation consisted in minimising an objective function (fitness function) depending on higher order multipoles of the potential. Finally, systematic changes of trap dimensions and electrode displacements were applied to investigate geometrical effects on the potential quality.

The MORA project

P. Delahaye [1,2], E. Liénard, I. Moore [3], M. Benali [2], M. L. Bissell [4], L. Canete [3], T. Eronen [3], A. Falkowski [5,2], X. Fléchard, M. Gonzalez-Alonso [6], W. Gins [7], R. P. De Groote [3], A. Jokinen [3], A. Kankainen [3], M. Kowalska [6], N. Lecesne [1], R. Leroy [1], Y. Merrer [2], G. Neyens [6,7], F. De Oliveira Santos [1], G. Quemener [2], A. De Roubin [3], B. -M. Retailleau [1], T. Roger [1], N. Severijns [7], J. C. Thomas [1], K. Turzo [1], P. Ujic [1]

Abstract

The MORA (Matter's Origin from the RadioActivity of trapped and oriented ions) project aims at measuring with unprecedented precision the D correlation in the nuclear beta decay of trapped and oriented ions. The D correlation offers the possibility to search for new CP-violating interactions, complementary to searches done at the LHC and with Electric Dipole Moments. Technically, MORA uses an innovative in-trap orientation method which combines the high trapping efficiency of a transparent Paul trap with laser orientation techniques. The trapping, detection, and laser setups are under development, for first tests at the Accelerator laboratory, JYFL, in the coming years.

The open LPC Paul trap for precision measurements in beta decay

P. Delahaye [1,2], G. Ban [2], M. Benali [2], D. Durand [2], X. Fabian [3,2], X. Fléchard, M. Herbane [2], E. Liénard, F. Mauger [2,4], A. Méry, Y. Merrer [2], O. Naviliat-Cuncic [2,5], G. Quéméner, B. M. Retailleau [1], D. Rodriguez [6], J. C. Thomas [1], P. Ujic [1]

Abstract

The LPCTrap experiment uses an open Paul trap which was built to enable precision measurements in the beta decay of radioactive ions. The initial goal was the precise measurement of the beta-neutrino angular correlation coefficient in the decay of 6He. Its geometry results from a careful optimization of the harmonic potential created by cylindrical electrodes. It supersedes previously considered geometries that presented a smaller detection solid angle to the beta particle and the recoiling ion. We describe here the methods which were used for the potential optimization, and we present the measured performances in terms of trapping time, cloud size and temperature, and space charge related limits. The properties of the ion cloud at equilibrium are well reproduced by a simple numerical simulation using hard sphere collisions, which additionally gives insights on the trapping loss mechanism. The interpretation for the observed trapping liftetimes is further corroborated by a model recently developed for ion clouds in Paul traps. The open trap shall serve other projects. It is currently used for commissioning purpose in the TRAPSENSOR experiment and is also considered in tests of the Standard Model involving the beta decay of polarized $^{23}$Mg and $^{39}$Ca ion in the frame of the MORA experiment. The latter tests require in-trap polarization of the ions and further optimization of the trapping and detection setup. Based on the results of the simulations and of their interpretations given by the model, different improvements of the trapping setup are discussed.

Electron shakeoff following the \b{eta}+ decay of 19Ne+ and 35Ar+ trapped ions

X. Fabian [1], X. Fléchard, B. Pons [2,1], E. Liénard, G. Ban [1], M. Breitenfeldt [3], C. Couratin [1], P. Delahaye [4], D. Durand [1], P. Finlay [3], B. Guillon [1], Y. Lemière, F. Mauger [1,5], A. Méry, O. Naviliat-Cuncic [1,6], T. Porobic [3,1], G. Quéméner, N. Severijns [3,4], J. -C. Thomas

Abstract

The electron shakeoff of 19F and 35Cl atoms resulting from the \b{eta}+ decay of 19Ne+ and 35Ar+ ions has been investigated using a Paul trap coupled to a time of flight recoil-ion spectrometer. The charge-state distributions of the recoiling daughter nuclei were compared to theoretical calculations based on the sudden approximation and accounting for subsequent Auger processes. The excellent agreement obtained for 35Cl is not reproduced in 19F. The shortcoming is attributed to the inaccuracy of the independent particle model employed to calculate the primary shakeoff probabilities in systems with rather low atomic numbers. This calls for more elaborate calculations, including explicitly the electron-electron correlations.

Extending the applicability of an open-ring trap to perform experiments with a single laser-cooled ion

J. M. Cornejo, M. Colombano [1], J. Doménech, M. Block [2,3,4], P. Delahaye [5,1], D. Rodríguez

Abstract

An open-ring ion trap, also referred to as transparent trap was initially built up to perform $β$-$ν$ correlation experiments with radioactive ions. This trap geometry is also well suited to perform experiments with laser-cooled ions, serving for the development of a new type of Penning trap, in the framework of the project TRAPSENSOR at the University of Granada. The goal of this project is to use a single $^{40}$Ca$^+$ ion as detector for single-ion mass spectrometry. Within this project and without any modification to the initial electrode configuration, it was possible to perform Doppler cooling on $^{40}$Ca$^+$ ions, starting from large clouds and reaching single ion sensitivity. This new feature of the trap might be important also for other experiments with ions produced at Radioactive Ion Beam (RIB) facilities. In this publication, the trap and the laser system will be described, together with their performance with respect to laser cooling applied to large ion clouds down to a single ion.

Electron shakeoff following the ?+ decay of trapped 35Ar+ ions

C. Couratin [1], X. Fabian [1], B. Fabre [2], B. Pons [2,1], X. Fléchard, E. Liénard, G. Ban [1], M. Breitenfeldt [3], P. Delahaye [4], D. Durand [1,5], A. Méry, O. Naviliat-Cuncic [1,6], T. Porobic [3,1,7], G. Quéméner, D. Rodriguez, N. Severijns [3,4], J. C. Thomas, S. Van Gorp [8]

Abstract

The electron shakeoff of $^{35}$Cl atoms resulting from the $β$$^+$ decay of $^{35}$Ar$^+$ ions has been investigated using a Paul trap coupled to a recoil-ion spectrometer. The charge-state distribution of the recoiling daughter nuclei is compared to theoretical calculations accounting for shakeoff and Auger processes. The calculations are in excellent agreement with the experimental results and enable to identify the ionization reaction routes leading to the formation of all charge states.

First detection and energy measurement of recoil ions following beta decay in a Penning trap with the WITCH experiment

M. Beck [1], S. Coeck [2], V. Yu. Kozlov, M. Breitenfeld [2], P. Delahaye [3], P. Friedag [1], M. Herbane [2], A. Herlert [3,2], I. S. Kraev, J. Mader [1], M. Tandecki [2], S. Van Gorp [2], F. Wauters [2], Ch. Weinheimer [1], F. Wenander [3], N. Severijns [2]

Abstract

The WITCH experiment (Weak Interaction Trap for CHarged particles) will search for exotic interactions by investigating the beta-neutrino angular correlation via the measurement of the recoil energy spectrum after beta decay. As a first step the recoil ions from the beta-minus decay of 124In stored in a Penning trap have been detected. The evidence for the detection of recoil ions is shown and the properties of the ion cloud that forms the radioactive source for the experiment in the Penning trap are presented.

Electric and magnetic field optimization procedure for Penning trap mass spectrometers

D. Beck, K. Blaum, G. Bollen, P. Delahaye, S. George, C. Guenaut, F. Herfurth, A. Herlert, D. Lunney, L. Schweikhard [1], C. Yazidjian [1]

Abstract

Significant systematic errors in high-precision Penning trap mass spectrometry can result from electric and magnetic field imperfections. An experimental procedure to minimize these uncertainties is presented for the on-line Penning trap mass spectrometer ISOLTRAP, located at ISOLDE/CERN. The deviations from the ideal magnetic and electric fields are probed by measuring the cyclotron frequency and the reduced cyclotron frequency, respectively, of stored ions as a function of the time between the ejection of ions from the preparation trap and their capture in the precision trap, which influences the energy of their axial motion. The correction parameters are adjusted to minimize the frequency shifts.

The WITCH Experiment: towards weak interactions studies. Status and prospects

V. Yu. Kozlov, M. Beck, S. Coeck, M. Herbane, I. S. Kraev, N. Severijns, F. Wauters, P. Delahaye, A. Herlert, F. Wenander, D. Zakoucky

Abstract

Primary goal of the WITCH experiment is to test the Standard Model for a possible ad-mixture of a scalar or tensor type interaction in beta-decay. This information will be inferred from the shape of the recoil energy spectrum. The experimental set-up was completed and is under intensive commissioning at ISOLDE (CERN). It combines a Penning trap to store the ions and a retardation spectrometer to probe the recoil ion energy. A brief overview of the WITCH set-up and the results of commissioning tests performed until now are presented. Finally, perspectives of the physics program are reviewed.